Inhibition, enhancement, and control of spontaneous emission in photonic nanowires.

We experimentally investigate the spontaneous emission (SE) rates of single InAs quantum dots embedded in GaAs photonic nanowires. For a diameter leading to the optimal confinement of the fundamental guided mode HE11, the coupling to HE11 dominates the SE process and an increase of the SE rate by a factor of 1.5 is achieved. When the diameter is decreased, the coupling to this mode vanishes rapidly, thus allowing the coupling to the other radiation modes to be probed. In these conditions, a SE inhibition factor of 16, equivalent to the one obtained in state-of-the-art photonic crystals, is measured. These results, which are supported by fully vectorial calculations, confirm the potential of photonic nanowires for a nearly perfect, broadband SE control.

[1]  V. Klimov Spontaneous emission rate of an excited atom placed near a nanofiber (17 pages) , 2004 .

[2]  E. Yablonovitch,et al.  Inhibited spontaneous emission in solid-state physics and electronics. , 1987, Physical review letters.

[3]  Willem L. Vos,et al.  Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals , 2004, Nature.

[4]  H Germany,et al.  Experimental realization of highly efficient broadband coupling of single quantum dots to a photonic crystal waveguide. , 2008, Physical review letters.

[5]  S. Hughes,et al.  Single quantum-dot Purcell factor and β factor in a photonic crystal waveguide , 2007 .

[6]  Jean-Paul Hugonin,et al.  Very Large Spontaneous-Emission β Factors in Photonic-Crystal Waveguides , 2007 .

[7]  A. Forchel,et al.  Inhibition and enhancement of the spontaneous emission of quantum dots in structured microresonators. , 2001, Physical review letters.

[8]  Jean-Paul Hugonin,et al.  The electromagnetic properties of light emission into semiconductor waveguides , 2006, SPIE Photonics Europe.

[9]  Kenichi Iga,et al.  Spontaneous emission factor of a microcavity DBR surface-emitting laser , 1991 .

[10]  D. Englund,et al.  Controlling the spontaneous emission rate of single quantum dots in a two-dimensional photonic crystal. , 2005, Physical review letters.

[11]  P. Hemmer,et al.  A diamond nanowire single-photon source. , 2009, Nature nanotechnology.

[12]  Willem L. Vos,et al.  Size dependence of the wavefunction of self-assembled InAs quantum dots from time-resolved optical measurements , 2008 .

[13]  N. Gregersen,et al.  A highly efficient single-photon source based on a quantum dot in a photonic nanowire , 2010 .

[14]  J. Mørk,et al.  Controlling the emission profile of a nanowire with a conical taper. , 2008, Optics letters.

[15]  Philippe Lalanne,et al.  Perfectly matched layers as nonlinear coordinate transforms: a generalized formalization. , 2005, Journal of the Optical Society of America. A, Optics, image science, and vision.

[16]  Jean-Michel Gérard,et al.  Solid-State Cavity-Quantum Electrodynamics with Self-Assembled Quantum Dots , 2003 .

[17]  C. Ning,et al.  Distribution of optical emission between guided modes and free space in a semiconductor nanowire , 2006 .

[18]  Chu,et al.  Photonic-wire laser. , 1995, Physical review letters.

[19]  V. Zwiller,et al.  Growth and characterization of InP nanowires with InAsP insertions. , 2007, Nano letters.

[20]  Tobias Heindel,et al.  Single photon emission from positioned GaAs/AlGaAs photonic nanowires , 2010 .

[21]  T. Asano,et al.  Spontaneous-emission control by photonic crystals and nanocavities , 2007 .

[22]  P Lalanne,et al.  Solid-state single photon sources: the nanowire antenna. , 2009, Optics express.

[23]  Jean-Michel Gérard,et al.  Polarization of the interband optical dipole in InAs/GaAs self-organized quantum dots , 2001 .