Sub-ps Laser Deposited Copper Films for Application in RF Guns

Copper thin films are intended to serve as a cover layer of photocathodes that are deposited by ablating copper targets in a high vacuum by temporally clean 600 fs laser pulses at 248 nm. The extremely forward-peaked plume produced by the ultrashort UV pulses of high-energy contrast ensures fast film growth. The deposition rate, defined as peak thickness per number of pulses, rises from 0.03 to 0.11 nm/pulse with an increasing ablated area while keeping the pulse energy constant. The material distribution over the surface-to-be-coated can also effectively be controlled by tuning the dimensions of the ablated area: surface patterning from airbrush-like to broad strokes is available. The well-adhering films of uniform surface morphology consist of densely packed lentil-like particles of several hundred nm in diameter and several ten nm in height. Task-optimized ultrashort UV laser deposition is thereby an effective approach for the production of thin film patterns of predetermined geometry, serving e.g., as critical parts of photocathodes.

[1]  M. Ferrario,et al.  Nano-machining, surface analysis and emittance measurements of a copper photocathode at SPARC_LAB , 2018, Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment.

[2]  E. Broitman,et al.  Pulsed laser deposition of yttrium photocathode suitable for use in radio-frequency guns , 2017 .

[3]  E. Broitman,et al.  Tight comparison of Mg and Y thin film photocathodes obtained by the pulsed laser deposition technique , 2016 .

[4]  S. Szatmári,et al.  Plasma mirrors for short pulse KrF lasers. , 2016, The Review of scientific instruments.

[5]  M. Anni,et al.  Deposition of Y thin films by nanosecond UV pulsed laser ablation for photocathode application , 2016 .

[6]  Chung-Wei Cheng,et al.  Femtosecond laser ablation of copper at high laser fluence: Modeling and experimental comparison , 2016 .

[7]  E. Broitman,et al.  Nanomechanical and electrical properties of Nb thin films deposited on Pb substrates by pulsed laser deposition as a new concept photocathode for superconductor cavities , 2015 .

[8]  C. Fotakis,et al.  Growth of poly-crystalline Cu films on Y substrates by picosecond pulsed laser deposition for photocathode applications , 2015 .

[9]  S. S. Harilal,et al.  Morphological changes in ultrafast laser ablation plumes with varying spot size. , 2015, Optics express.

[10]  T. Schietinger,et al.  Intrinsic emittance reduction of copper cathodes by laser wavelength tuning in an rf photoinjector , 2015 .

[11]  S. Amoruso,et al.  Multidiagnostic analysis of ion dynamics in ultrafast laser ablation of metals over a large fluence range , 2015 .

[12]  A. Cola,et al.  Non-conventional photocathodes based on Cu thin films deposited on Y substrate by sputtering , 2014 .

[13]  A. Cola,et al.  New configuration of metallic photocathodes prepared by pulsed laser deposition , 2013 .

[14]  Barbara Marchetti,et al.  The SPARC linear accelerator based terahertz source , 2013 .

[15]  A. Lorusso Overview and development of metallic photocathodes prepared by laser ablation , 2013 .

[16]  J. Schou,et al.  Femtosecond ultraviolet laser ablation of silver and comparison with nanosecond ablation , 2013 .

[17]  P. Emma,et al.  High-brightness Electron Beam Evolution Following Laser-based Cleaning of a Photocathode , 2012 .

[18]  A. Abdolvand,et al.  Laser-assisted highly organized structuring of copper , 2011 .

[19]  Peter Balling,et al.  Ultra-short pulse laser ablation of copper, silver and tungsten: experimental data and two-temperature model simulations , 2011 .

[20]  Xijie Wang,et al.  Surface photoemission in a high-brightness electron beam radio frequency gun , 2010 .

[21]  S. Amoruso,et al.  Angular distributions of plume components in ultrafast laser ablation of metal targets , 2010 .

[22]  L Cultrera,et al.  Multiphoton photoemission from a copper cathode illuminated by ultrashort laser pulses in an RF photoinjector. , 2010, Physical review letters.

[23]  M. Sentis,et al.  Subpicosecond laser ablation of copper and fused silica: Initiation threshold and plasma expansion , 2009 .

[24]  Na Li,et al.  The spatial detection on distribution of metal nano-particles during femtosecond laser ablation , 2009, Applied Optics and Photonics China.

[25]  A. Perrone,et al.  Electron emission characterization of Mg photocathode grown by pulsed laser deposition within an S-band rf gun , 2009 .

[26]  S. Grigorescu,et al.  Photoelectron emission from yttrium thin films prepared by pulsed laser deposition. , 2009, Journal of nanoscience and nanotechnology.

[27]  J. Maldonado,et al.  Robust CsBr/Cu Photocathodes for the Linac Coherent Light Source , 2008 .

[28]  L. Torrisi,et al.  Laser ablation threshold of cultural heritage metals , 2007, 2007 European Conference on Lasers and Electro-Optics and the International Quantum Electronics Conference.

[29]  Bo-Sung Shin,et al.  Theoretical and experimental investigations into laser ablation of polyimide and copper films with 355-nm Nd:YVO4 laser , 2007 .

[30]  C. Ristoscu,et al.  Mg based photocathodes for high brightness RF photoinjectors , 2007 .

[31]  P. A. Atanasov,et al.  Femtosecond laser ablation of nickel in vacuum , 2007 .

[32]  A. Loir,et al.  Towards the deposition of tetrahedral diamond-like carbon films on hip joints by femtosecond pulsed laser ablation , 2004 .

[33]  C. Fotakis,et al.  Expansion velocities of 0.5 ps KrF excimer laser induced plasma by Doppler-shift analysis of pump and probe measurements , 2004 .

[34]  T. Glynn,et al.  The effect of damage accumulation behaviour on ablation thresholds and damage morphology in ultrafast laser micro-machining of common metals in air , 2004 .

[35]  Eitan Grossman,et al.  Synthesis of nanoparticles with femtosecond laser pulses , 2004 .

[36]  G. Duscher,et al.  Plasma plume characteristics and properties of pulsed laser deposited diamond-like carbon films , 2003 .

[37]  A. Loir,et al.  Femtosecond pulsed laser deposition of diamond-like carbon thin films for tribological applications , 2003 .

[38]  Guillaume Petite,et al.  Ablation threshold dependence on pulse duration for copper , 2002 .

[39]  X. Chang,et al.  S-BAND HIGH DUTY PHOTO-INJECTION SYSTEM. , 2002 .

[40]  B. Luther-Davies,et al.  Ablation of solids by femtosecond lasers: ablation mechanism and ablation thresholds for metals and dielectrics , 2001, physics/0102046.

[41]  K. Chen,et al.  Modelling and Analysis of UV Laser Micromachining of Copper , 2001 .

[42]  Christopher J. Sutcliffe,et al.  Micromachining of copper using Nd:YAG laser radiation at 1064, 532, and 355 nm wavelengths , 2001 .

[43]  Michael D. Feit,et al.  Modeling of long-term behavior of ablation plumes produced with ultrashort laser pulses , 2000, Photonics West - Lasers and Applications in Science and Engineering.

[44]  K. Gal,et al.  Properties of high harmonics generated by ultrashort UV laser pulses on solid surfaces , 2000 .

[45]  T. Srinivasan-Rao,et al.  Sputtered magnesium as a photocathode material for rf injectors , 1998 .

[46]  J. Ihlemann,et al.  Ablation of submicron structures on metals and semiconductors by femtosecond UV-laser pulses , 1997 .

[47]  A. Tünnermann,et al.  Precise Laser Ablation with Ultra-Short Pulses , 1997, Conference on Lasers and Electro-Optics Europe.

[48]  Teubner,et al.  Absorption and hot electron production by high intensity femtosecond uv-laser pulses in solid targets. , 1996, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[49]  C. Lewis,et al.  Polar distribution of ablated atomic material during the pulsed laser deposition of Cu in vacuum: Dependence on focused laser spot size and power density , 1996 .

[50]  M. Stuke,et al.  Sub-picosecond UV laser ablation of metals , 1995 .

[51]  J. Fischer,et al.  Measurements on photoelectrons from a magnesium cathode in a microwave electron gun , 1995 .

[52]  J. Lunney,et al.  Pulsed laser ablation of copper , 1995 .

[53]  Klaus R. Mann,et al.  Comparative study of deposition of thin films by laser-induced PVD with femtosecond and nanosecond laser pulses , 1993, Photonics West - Lasers and Applications in Science and Engineering.

[54]  J. Fischer,et al.  Photoemission studies on metals using picosecond ultraviolet laser pulses , 1991 .

[55]  Narayan,et al.  Pulsed-laser evaporation technique for deposition of thin films: Physics and theoretical model. , 1990, Physical review. B, Condensed matter.