Slow light in an artificial hybrid nanocrystal complex

A slow light effect in a hybrid nanocrystal complex composed of a semiconductor quantum dot (SQD) and a metal nanoparticle (MNP) is investigated theoretically. It is shown that a hole induced by coherent population oscillation appears at the absorption spectrum of the probe when an exciton and plasmon interact. Then a slow light effect may become possible. The numerical results further indicate that the slow light effect is greatly modified by the distance between the SQD and the MNP due to the coupling of the exciton and plasmon. For experimental conditions, the group velocity indexes with Gauss distribution and Lorenz distribution of the distance between the SQD and the MNP are evaluated. It is found that for small dispersion, almost the same values of the group velocity index can be obtained in these different distributions.

[1]  Pritchard,et al.  Amplification of light and atoms in a bose-einstein condensate , 2000, Physical review letters.

[2]  J. Mørk,et al.  Voltage-controlled slow light in an integrated semiconductor structure with net gain. , 2006, Optics express.

[3]  R. Boyd,et al.  Enhanced self-action effects by electromagnetically induced transparency in the two-level atom , 2001 .

[4]  S. Harris,et al.  Light speed reduction to 17 metres per second in an ultracold atomic gas , 1999, Nature.

[5]  Harris,et al.  Dispersive properties of electromagnetically induced transparency. , 1992, Physical review. A, Atomic, molecular, and optical physics.

[6]  Garnett W. Bryant,et al.  Metal‐nanoparticle plasmonics , 2008 .

[7]  Yadong Yin,et al.  Colloidal nanocrystal synthesis and the organic–inorganic interface , 2005, Nature.

[8]  Wei Zhang,et al.  Semiconductor-metal nanoparticle molecules: hybrid excitons and the nonlinear fano effect. , 2006, Physical review letters.

[9]  Shun Lien Chuang,et al.  Room-temperature slow light with semiconductor quantum-dot devices. , 2006, Optics letters.

[10]  Stephen R. Forrest,et al.  Optical nonlinearities in crystalline organic multiple quantum wells. , 1990 .

[11]  Philip Hemmer,et al.  Tunable ultraslow light in vertical-cavity surface-emitting laser amplifier. , 2005, Optics express.

[12]  Robert W Boyd,et al.  Observation of ultraslow light propagation in a ruby crystal at room temperature. , 2003, Physical review letters.

[13]  A. Govorov,et al.  Optical properties of coupled metal-semiconductor and metal-molecule nanocrystal complexes: Role of multipole effects , 2008, 0801.3213.

[14]  Greene,et al.  Phonon-mediated optical nonlinearity in polydiacetylene. , 1988, Physical review letters.

[15]  Edward S. Fry,et al.  ULTRASLOW GROUP VELOCITY AND ENHANCED NONLINEAR OPTICAL EFFECTS IN A COHERENTLY DRIVEN HOT ATOMIC GAS , 1999, quant-ph/9904031.

[16]  Agarwal Electromagnetic-field-induced transparency in high-density exciton systems. , 1995, Physical review. A, Atomic, molecular, and optical physics.

[17]  Garnett W. Bryant,et al.  Exciton-plasmon interaction and hybrid excitons in semiconductor-metal nanoparticle assemblies , 2006 .

[18]  T. Mossberg,et al.  DRIVING THE DRIVEN ATOM : SPECTRAL SIGNATURES , 1997 .

[19]  J. Lakowicz,et al.  Metal-enhanced fluorescence from CdTe nanocrystals: a single-molecule fluorescence study. , 2006, Journal of the American Chemical Society.

[20]  Robert W. Boyd,et al.  Superluminal and Slow Light Propagation in a Room-Temperature Solid , 2003, Science.

[21]  C. Lieber,et al.  Nanowire Nanosensors for Highly Sensitive and Selective Detection of Biological and Chemical Species , 2001, Science.

[22]  S. Duan,et al.  Plasmon-enhanced midinfrared generation from difference frequency in semiconductor quantum dots , 2008 .

[23]  Nicholas A. Kotov,et al.  Bioconjugates of CdTe Nanowires and Au Nanoparticles: Plasmon−Exciton Interactions, Luminescence Enhancement, and Collective Effects , 2004 .

[24]  T. Klar,et al.  Gold nanoparticles quench fluorescence by phase induced radiative rate suppression. , 2005, Nano letters.

[25]  D H Werner,et al.  Nanosphere dispersed liquid crystals for tunable negative-zero-positive index of refraction in the optical and terahertz regimes. , 2006, Optics letters.

[26]  M. Bawendi,et al.  Surface-enhanced emission from single semiconductor nanocrystals. , 2002, Physical review letters.