Crystal-facet-oriented altermagnets for detecting ferromagnetic and antiferromagnetic states by giant tunneling magnetoresistance

Emerging altermagnetic materials with vanishing net magnetizations and unique band structures have been envisioned as an ideal electrode to design antiferromagnetic tunnel junctions. Their momentum-resolved spin splitting in band structures defines a spin-polarized Fermi surface, which allows altermagnetic materials to polarize current as a ferromagnet, when the current flows along specific directions relevant to their altermagnetism. Here, we design an Altermagnet/Insulator barrier/Ferromagnet junction, renamed as altermagnetic tunnel junction (ATMTJ), using RuO$_2$/TiO$_2$/CrO$_2$ as a prototype. Through first-principles calculations, we investigate the tunneling properties of the ATMTJ along the [001] and [110] directions, which shows that the tunneling magnetoresistance (TMR) is almost zero when the current flows along the [001] direction, while it can reach as high as 6100\% with current flows along the [110] direction. The spin-resolved conduction channels of the altermagnetic RuO$_2$ electrode are found responsible for this momentum-dependent (or transport-direction-dependent) TMR effect. Furthermore, this ATMTJ can also be used to readout the N\'{e}el vector of the altermagnetic electrode RuO$_2$. Our work promotes the understanding toward the altermagnetic materials and provides an alternative way to design magnetic tunnel junctions with ultrahigh TMR ratios and robustness of the altermagnetic electrode against external disturbance, which broadens the application avenue for antiferromagnetic spintronic devices.

[1]  Z. Zeng,et al.  Room-temperature magnetoresistance in an all-antiferromagnetic tunnel junction , 2023, Nature.

[2]  R. Arita,et al.  Octupole-driven magnetoresistance in an antiferromagnetic tunnel junction , 2023, Nature.

[3]  J. Sinova,et al.  Emerging Research Landscape of Altermagnetism , 2022, Physical Review X.

[4]  E. Tsymbal,et al.  Tunneling Magnetoresistance in Noncollinear Antiferromagnetic Tunnel Junctions , 2021, 2023 IEEE International Magnetic Conference - Short Papers (INTERMAG Short Papers).

[5]  J. Sinova,et al.  Giant and Tunneling Magnetoresistance in Unconventional Collinear Antiferromagnets with Nonrelativistic Spin-Momentum Coupling , 2021, Physical Review X.

[6]  E. Tsymbal,et al.  Spin-neutral currents for spintronics , 2021, Nature Communications.

[7]  A. Zunger,et al.  Prediction of low-Z collinear and noncollinear antiferromagnetic compounds having momentum-dependent spin splitting even without spin-orbit coupling , 2020, 2008.08532.

[8]  A. Zunger,et al.  Giant momentum-dependent spin splitting in centrosymmetric low- Z antiferromagnets , 2020 .

[9]  S. Hayami,et al.  Momentum-Dependent Spin Splitting by Collinear Antiferromagnetic Ordering , 2019, Journal of the Physical Society of Japan.

[10]  J. Sinova,et al.  Crystal time-reversal symmetry breaking and spontaneous Hall effect in collinear antiferromagnets , 2019, Science Advances.

[11]  Yu-Jun Zhao,et al.  Ferromagnetic Weyl fermions in CrO2 , 2017, Physical Review B.

[12]  K. Ohno,et al.  Momentum-dependent band spin splitting in semiconducting MnO2: a density functional calculation. , 2016, Physical chemistry chemical physics : PCCP.

[13]  J. Wunderlich,et al.  Antiferromagnetic spintronics. , 2015, Nature nanotechnology.

[14]  J. Aarts,et al.  Anomalous transport in half-metallic ferromagnetic CrO2 , 2013, 1303.3746.

[15]  Fujio Izumi,et al.  VESTA 3 for three-dimensional visualization of crystal, volumetric and morphology data , 2011 .

[16]  J. Lenz,et al.  Magnetic sensors and their applications , 2006, IEEE Sensors Journal.

[17]  E. Tsymbal,et al.  Spin-dependent tunnelling in magnetic tunnel junctions , 2003 .

[18]  G. Schütz,et al.  Strong anisotropy of projected 3d moments in epitaxial CrO2 films. , 2002, Physical review letters.

[19]  Stuart A. Wolf,et al.  Spintronics: A Spin-Based Electronics Vision for the Future , 2001, Science.

[20]  Jian Wang,et al.  Ab initio modeling of quantum transport properties of molecular electronic devices , 2001 .

[21]  W. Butler,et al.  Band structure, evanescent states, and transport in spin tunnel junctions , 2001 .

[22]  A Kokalj,et al.  XCrySDen--a new program for displaying crystalline structures and electron densities. , 1999, Journal of molecular graphics & modelling.

[23]  G. Kresse,et al.  From ultrasoft pseudopotentials to the projector augmented-wave method , 1999 .

[24]  C. Humphreys,et al.  Electron-energy-loss spectra and the structural stability of nickel oxide: An LSDA+U study , 1998 .

[25]  J. Haines,et al.  Neutron Diffraction Study of the Ambient-Pressure, Rutile-Type and the High-Pressure, CaCl2-Type Phases of Ruthenium Dioxide , 1997 .

[26]  Burke,et al.  Generalized Gradient Approximation Made Simple. , 1996, Physical review letters.

[27]  Kresse,et al.  Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set. , 1996, Physical review. B, Condensed matter.

[28]  J. Moodera,et al.  Large magnetoresistance at room temperature in ferromagnetic thin film tunnel junctions. , 1995, Physical review letters.

[29]  T. Miyazaki,et al.  Giant magnetic tunneling e ect in Fe/Al2O3/Fe junction , 1995 .

[30]  Blöchl,et al.  Projector augmented-wave method. , 1994, Physical review. B, Condensed matter.

[31]  V. Anisimov,et al.  Band theory and Mott insulators: Hubbard U instead of Stoner I. , 1991, Physical review. B, Condensed matter.

[32]  M. Julliere Tunneling between ferromagnetic films , 1975 .

[33]  G. Shirane,et al.  MAGNETIC STRUCTURES IN THE MnSb-CrSb SYSTEM , 1963 .

[34]  J. Klinowski,et al.  A multinuclear NMR study of clinochlore , 1995 .