Shifted power-law relationship between NO2 concentration and the distance from a highway: A new dispersion model based on the wind profile model

Abstract In this paper, a shifted power-law model, based on the wind profile model, had been supposed to simulate concentration gradient of nitrogen dioxide (NO2) with distance from a highway. Field experiments were performed for NO2 gradients from a highway in Shanghai by using passive samplers. The shifted power-law model was fitted well with experimental results of field experiments both in this study and in the literature. The results not only verified the validity of shifted power-law relationship between NO2 concentration and the distance from a highway, but also partially demonstrated that there were some significant similarities between wind profile and air pollutants concentration profile near highway. With known concentration of chosen reference point and appropriate value of the parameter k, the model could be practically applied for predicting the NO2 distributions near a highway. The methods of determining the parameter k were also discussed for further detailed studies.

[1]  Hanefi Bayraktar,et al.  Impacts of some meteorological parameters on SO2 and TSP concentrations in Erzurum, Turkey. , 2005, Chemosphere.

[2]  Yasushi Kodama,et al.  Environmental NO2 concentration and exposure in daily life along main roads in Tokyo. , 2002, Environmental research.

[3]  M. Jenkin,et al.  Analysis of the relationship between ambient levels of O3, NO2 and NO as a function of NOx in the UK , 2001 .

[4]  F. T. M. Nieuwstadt,et al.  Atmospheric Turbulence and Air Pollution Modelling , 1982 .

[5]  S. Arya Air Pollution Meteorology and Dispersion , 1998 .

[6]  Bert Brunekreef,et al.  Assessment of exposure to traffic related air pollution of children attending schools near motorways , 2001 .

[7]  L. Skärby,et al.  Effects of air pollutant emissions from a rural motorway on Petunia and Trifolium , 1994 .

[8]  H. Elminir Dependence of urban air pollutants on meteorology. , 2005, The Science of the total environment.

[9]  J. R. Eagleman,et al.  Air Pollution Meteorology , 1991 .

[10]  David M Stieb,et al.  Ambient nitrogen dioxide and distance from a major highway. , 2003, The Science of the total environment.

[11]  Diffusion from a line source deployed in a homogeneous roughness layer: interpretation of wind-tunnel measurements by means of simple mathematical models , 2002 .

[12]  H. Tennekes,et al.  Similarity Relations, Scaling Laws and Spectral Dynamics , 1984 .

[13]  C. Kirby,et al.  Temporal and Spatial Variations in Nitrogen Dioxide Concentrations Across an Urban Landscape: Cambridge, UK , 1998 .

[14]  A Statistical Analysis of Particulate Data Sets for Jawaharlal Nehru Port and Surrounding Harbour Region in India , 2004, Environmental monitoring and assessment.

[15]  M. A. Mugglestone,et al.  Local and seasonal variations in atmospheric nitrogen dioxide levels at Rothamsted, UK, and relationships with meteorological conditions , 2000 .

[16]  David M. Holland,et al.  Variations of NO, NO2 and O3 concentrations downwind of a Los Angeles freeway , 1981 .

[17]  E. Plate Methods of investigating urban wind fields—physical models , 1999 .

[18]  H. Mayer Air pollution in cities , 1999 .

[19]  H. Pleijel,et al.  On the logarithmic relationship between NO2 concentration and the distance from a highroad. , 2004, The Science of the total environment.

[20]  Bert Brunekreef,et al.  Air pollution from traffic in city districts near major motorways. , 1998 .

[21]  A. Wiedensohler,et al.  Long term measurements of submicrometer urban aerosols: statistical analysis for correlations with meteorological conditions and trace gases , 2002 .

[22]  J. Cape,et al.  Vegetation composition of roadside verges in Scotland: the effects of nitrogen deposition, disturbance and management. , 2005, Environmental pollution.