Attosecond time-scale feedback control of coherent X-ray generation

Abstract High-harmonic generation is an extreme, high-order, nonlinear process that converts intense, ultrafast, visible and infrared laser light pulses coherently into the soft X-ray region of the spectrum. We demonstrate that by optimizing the shape of an ultrafast laser pulse, we can selectively enhance this process by promoting strong constructive interference between X-ray bursts emitted from adjacent optical cycles. This work demonstrates that coherent control of highly nonlinear processes in the strong-field regime is possible by adjusting the relative timing of the crests of an electromagnetic wave on a sub-optical cycle, attosecond time scale.

[1]  Kapteyn,et al.  Enhanced high-harmonic generation using 25 fs laser pulses. , 1996, Physical review letters.

[2]  Rick Trebino,et al.  Frequency-resolved optical gating with the use of second-harmonic generation , 1994 .

[3]  Ulrich A. Russek,et al.  Pulse compression by use of deformable mirrors. , 1999, Optics letters.

[4]  Vladislav V. Yakovlev,et al.  Feedback quantum control of molecular electronic population transfer , 1997 .

[5]  Gordon,et al.  High-order harmonic generation using intense femtosecond pulses. , 1993, Physical review letters.

[6]  D Yelin,et al.  Adaptive femtosecond pulse compression. , 1997, Optics letters.

[7]  Ferenc Krausz,et al.  Generation of Coherent X-rays in the Water Window Using 5-Femtosecond Laser Pulses , 1997 .

[8]  I. Christov,et al.  TEMPORAL PHASE CONTROL OF SOFT-X-RAY HARMONIC EMISSION , 1998 .

[9]  Thomas Weinacht,et al.  Toward strong field mode-selective chemistry , 1999 .

[10]  I. Christov,et al.  Shaped-pulse optimization of coherent emission of high-harmonic soft X-rays , 2000, Nature.

[11]  Henry C. Kapteyn,et al.  High-Harmonic Generation of Attosecond Pulses in the ``Single-Cycle'' Regime , 1997 .

[12]  M. Lewenstein,et al.  TEMPORAL AND SPECTRAL TAILORING OF HIGH-ORDER HARMONICS , 1998 .

[13]  Richard Haight,et al.  Electron dynamics at surfaces , 1995 .

[14]  Schafer,et al.  Higher-order harmonic generation in xenon at 1064 nm: The role of phase matching. , 1991, Physical review letters.

[15]  Andrew M. Weiner,et al.  High-resolution femtosecond pulse shaping , 1988 .

[16]  M. Murnane,et al.  Phase-matched generation of coherent soft X-rays , 1998, Science.

[17]  M. Murnane,et al.  Adaptive pulse compression for transform-limited 15-fs high-energy pulse generation. , 2000, Optics letters.

[18]  Charles K. Rhodes,et al.  Studies of multiphoton production of vacuum-ultraviolet radiation in the rare gases , 1987 .

[19]  Gerber,et al.  Control of chemical reactions by feedback-optimized phase-shaped femtosecond laser pulses , 1998, Science.

[20]  Kompa,et al.  Whither the future of controlling quantum phenomena? , 2000, Science.

[21]  I. Christov,et al.  Generation and propagation of attosecond x-ray pulses in gaseous media , 1998 .

[22]  Henry C. Kapteyn,et al.  GENERATION OF COHERENT SOFT X RAYS AT 2.7 NM USING HIGH HARMONICS , 1997 .

[23]  Charles G. Durfee,et al.  High power ultrafast lasers , 1998 .

[24]  Ivanov,et al.  Theory of high-harmonic generation by low-frequency laser fields. , 1994, Physical review. A, Atomic, molecular, and optical physics.

[25]  P. Bucksbaum,et al.  Controlling the shape of a quantum wavefunction , 1999, Nature.

[26]  H. Rabitz,et al.  Teaching lasers to control molecules. , 1992, Physical review letters.

[27]  H. Rabitz Ramifications of Feedback for Control of Quantum Dynamics Feedback for Control of Quantum Dynamics , 1997 .

[28]  Bernard Piraux,et al.  Super-Intense Laser-Atom Physics , 1993 .

[29]  Yaron Silberberg,et al.  Coherent quantum control of two-photon transitions by a femtosecond laser pulse , 1998, Nature.