A theoretical study of the effect of relative humidity on light scattering by tropospheric aerosols

A theoretical analysis of the factors which contribute to the hygroscopic growth of atmospheric aerosols is presented within the context of the climatic impact of these aerosols. It is found that the factor which most influences the growth factor is the position of the initial dry aerosol size distribution relative to the efficient light scattering particle size range. When this factor is taken into consideration, rural aerosols have much larger growth factors than those currently utilized in assessment of the climatic impact of atmospheric aerosols.

[1]  H. Hansson,et al.  Hygroscopic growth of aerosol particles in the Po Valley , 1992 .

[2]  J. Coakley,et al.  Climate Forcing by Anthropogenic Aerosols , 1992, Science.

[3]  Robert J. Charlson,et al.  Perturbation of the northern hemisphere radiative balance by backscattering from anthropogenic sulfate aerosols , 1991 .

[4]  G. Isaac,et al.  Tropospheric aerosol size distributions from 1982 to 1988 over eastern North America , 1991 .

[5]  S. Jennings,et al.  Physical characteristics of the ambient aerosol at Mace Head , 1991 .

[6]  R. E. Larson,et al.  Aerosol size distributions at a site on the east coast of the united states , 1984 .

[7]  T. Larson,et al.  In-situ, rapid response measurement of H2SO4/(NH4)2SO4 aerosols in urban Houston: A comparison with rural Virginia , 1983 .

[8]  T. Larson,et al.  In situ rapid-response measurement of sulfuric acid/ammonium sulfate aerosols in rural Virginia , 1982 .

[9]  T. Larson,et al.  In situ rapid-response measurement of H2SO4/(NH4)2 SO4 aerosols in rural Virginia. , 1982 .

[10]  S. Friedlander FUTURE AEROSOLS OF THE SOUTHWEST: IMPLICATIONS FOR FUNDAMENTAL AEROSOL RESEARCH * , 1980 .

[11]  J. Butler,et al.  AMBIENT SULFATE MEASUREMENTS ON ALLEGHENY MOUNTAIN AND THE QUESTION OF ATMOSPHERIC SULFATE IN THE NORTHEASTERN UNITED STATES , 1980 .

[12]  C. Lürzer Trimodal mass-size distributions of urban aerosol measured by cascade impactors , 1980 .

[13]  K. T. Whitby THE PHYSICAL CHARACTERISTICS OF SULFUR AEROSOLS , 1978 .

[14]  I. Tang,et al.  Aerosol growth studies — IV. Phase transformation of mixed salt aerosols in a moist atmosphere , 1978 .

[15]  Á. Mészáros,et al.  On the concentration and size distribution of atmospheric sulfate particles under rural conditions , 1978 .

[16]  I. Tang,et al.  Aerosol growth studies—III ammonium bisulfate aerosols in a moist atmosphere , 1977 .

[17]  I. Tang,et al.  Phase transformation and growth of aerosol particles composed of mixed salts , 1976 .

[18]  Gottfried Hänel,et al.  The Properties of Atmospheric Aerosol Particles as Functions of the Relative Humidity at Thermodynamic Equilibrium with the Surrounding Moist Air , 1976 .

[19]  R. Charlson,et al.  Sulfuric Acid-Ammonium Sulfate Aerosol: Optical Detection in the St. Louis Region , 1974, Science.

[20]  J. Dave,et al.  Scattering of electromagnetic radiation by a large, absorbing sphere , 1969 .