Flexible quantum dot light-emitting diodes for next-generation displays
暂无分享,去创建一个
Dae-Hyeong Kim | Taeghwan Hyeon | Jiwoong Yang | Moon Kee Choi | T. Hyeon | Dae‐Hyeong Kim | M. Choi | Jiwoong Yang
[1] V. Bulović,et al. Emergence of colloidal quantum-dot light-emitting technologies , 2012, Nature Photonics.
[2] Yonghoon Choi,et al. Large-Scale Synthesis of Highly Luminescent InP@ZnS Quantum Dots Using Elemental Phosphorus Precursor , 2017 .
[3] Lazaro A. Padilha,et al. Controlling the influence of Auger recombination on the performance of quantum-dot light-emitting diodes , 2013, Nature Communications.
[4] V. Bulović,et al. NiO as an inorganic hole-transporting layer in quantum-dot light-emitting devices. , 2006, Nano letters.
[5] Eric A. Dauler,et al. High‐Performance Shortwave‐Infrared Light‐Emitting Devices Using Core–Shell (PbS–CdS) Colloidal Quantum Dots , 2015, Advanced materials.
[6] Taeghwan Hyeon,et al. Nonclassical nucleation and growth of inorganic nanoparticles , 2016 .
[7] V. Bulović,et al. Colloidal quantum dot light-emitting devices , 2010, Nano reviews.
[8] Won Chul Lee,et al. Self-organized growth and self-assembly of nanostructures on 2D materials , 2017 .
[9] Qibing Pei,et al. Highly Flexible Silver Nanowire Electrodes for Shape‐Memory Polymer Light‐Emitting Diodes , 2011, Advanced materials.
[10] Dae-Hyeong Kim,et al. The quest for miniaturized soft bioelectronic devices , 2017, Nature Biomedical Engineering.
[11] Taeghwan Hyeon,et al. Cephalopod‐Inspired Miniaturized Suction Cups for Smart Medical Skin , 2016, Advanced healthcare materials.
[12] K. Char,et al. Multicolored light-emitting diodes based on all-quantum-dot multilayer films using layer-by-layer assembly method. , 2010, Nano letters.
[13] Zhaoqun Zhou,et al. 32.4: Quantum Dot Light Emitting Diodes for Full-color Active-matrix Displays , 2010 .
[14] M. Bawendi,et al. Colloidal quantum--dot light-emitting diodes with metal-oxide charge transport layers , 2008 .
[15] Liangbing Hu,et al. Emerging Transparent Electrodes Based on Thin Films of Carbon Nanotubes, Graphene, and Metallic Nanostructures , 2011, Advanced materials.
[16] Benoit Dubertret,et al. Quasi‐2D Colloidal Semiconductor Nanoplatelets for Narrow Electroluminescence , 2014 .
[17] Dandan Zhang,et al. Vacuum-free transparent quantum dot light-emitting diodes with silver nanowire cathode , 2015, Scientific Reports.
[18] J. Y. Han,et al. High-performance crosslinked colloidal quantum-dot light-emitting diodes , 2009 .
[19] Dong Chan Kim,et al. High‐Resolution Spin‐on‐Patterning of Perovskite Thin Films for a Multiplexed Image Sensor Array , 2017, Advanced materials.
[20] Kookheon Char,et al. Single-Step Synthesis of Quantum Dots with Chemical Composition Gradients , 2008 .
[21] V. Bulović,et al. High-efficiency quantum-dot light-emitting devices with enhanced charge injection , 2013, Nature Photonics.
[22] Xiangang Luo,et al. Efficiency Enhancement of Organic Solar Cells Using Transparent Plasmonic Ag Nanowire Electrodes , 2010, Advanced materials.
[23] Yan Fu,et al. Polyethylenimine Ethoxylated-Mediated All-Solution-Processed High-Performance Flexible Inverted Quantum Dot-Light-Emitting Device. , 2017, ACS nano.
[24] Takao Someya,et al. Ultrathin, highly flexible and stretchable PLEDs , 2013, Nature Photonics.
[25] B. Dubertret,et al. Colloidal nanoplatelets with two-dimensional electronic structure. , 2011, Nature materials.
[26] Jin Jang,et al. Semi-transparent quantum-dot light emitting diodes with an inverted structure , 2014 .
[27] V. Bulović,et al. Contact printing of quantum dot light-emitting devices. , 2008, Nano letters.
[28] E. Sargent,et al. Size-tunable infrared (1000–1600 nm) electroluminescence from PbS quantum-dot nanocrystals in a semiconducting polymer , 2003 .
[29] Taeghwan Hyeon,et al. Designed Assembly and Integration of Colloidal Nanocrystals for Device Applications , 2016, Advanced materials.
[30] 金洛煥,et al. Printed assemblies of ultrathin, microscale inorganic light emitting diodes for deformable and semitransparent displays , 2010 .
[31] A. Alivisatos,et al. Light-emitting diodes made from cadmium selenide nanocrystals and a semiconducting polymer , 1994, Nature.
[32] Jung Ho Yu,et al. Route to the Smallest Doped Semiconductor: Mn(2+)-Doped (CdSe)13 Clusters. , 2015, Journal of the American Chemical Society.
[33] Dae-Hyeong Kim,et al. Heterogeneous stacking of nanodot monolayers by dry pick-and-place transfer and its applications in quantum dot light-emitting diodes , 2013, Nature Communications.
[34] Jin-Song Hu,et al. Zn-Cu-In-Se Quantum Dot Solar Cells with a Certified Power Conversion Efficiency of 11.6%. , 2016, Journal of the American Chemical Society.
[35] Dae-Hyeong Kim,et al. Wearable Sensing Systems with Mechanically Soft Assemblies of Nanoscale Materials , 2017 .
[36] Jung Ho Yu,et al. Dimension-controlled synthesis of CdS nanocrystals: from 0D quantum dots to 2D nanoplates. , 2012, Small.
[37] A. Alivisatos. Semiconductor Clusters, Nanocrystals, and Quantum Dots , 1996, Science.
[38] John A Rogers,et al. Double-heterojunction nanorod light-responsive LEDs for display applications , 2017, Science.
[39] A. Alivisatos,et al. Improved efficiencies in light emitting diodes made with CdSe(CdS) core/shell type nanocrystals and a semiconducting polymer , 1997 .
[40] Moonsub Shim,et al. Double-heterojunction nanorods , 2014, Nature Communications.
[41] Moungi G Bawendi,et al. Air-stable operation of transparent, colloidal quantum dot based LEDs with a unipolar device architecture. , 2010, Nano letters.
[42] V. Bulović,et al. Large‐Area Ordered Quantum‐Dot Monolayers via Phase Separation During Spin‐Casting , 2005 .
[43] Yei Hwan Jung,et al. Stretchable silicon nanoribbon electronics for skin prosthesis , 2014, Nature Communications.
[44] Cherie R. Kagan,et al. Building devices from colloidal quantum dots , 2016, Science.
[45] Zhibin Yu,et al. User-interactive electronic skin for instantaneous pressure visualization. , 2013, Nature materials.
[46] A. Rogach,et al. Infrared-emitting colloidal nanocrystals: synthesis, assembly, spectroscopy, and applications. , 2007, Small.
[47] Louis Brus,et al. Chemical Synthesis and Luminescence Applications of Colloidal Semiconductor Quantum Dots. , 2017, Journal of the American Chemical Society.
[48] Benoit Dubertret,et al. Cadmium-free CuInS2/ZnS quantum dots for sentinel lymph node imaging with reduced toxicity. , 2010, ACS nano.
[49] D. Y. Yoon,et al. Bright and efficient full-color colloidal quantum dot light-emitting diodes using an inverted device structure. , 2012, Nano letters.
[50] Kookheon Char,et al. R/G/B/Natural White Light Thin Colloidal Quantum Dot‐Based Light‐Emitting Devices , 2014, Advanced materials.
[51] B. G. DeLacy,et al. Transparent displays enabled by resonant nanoparticle scattering , 2014, Nature Communications.
[52] Ji Hoon Kim,et al. Wearable red–green–blue quantum dot light-emitting diode array using high-resolution intaglio transfer printing , 2015, Nature Communications.
[53] Yonggang Huang,et al. Waterproof AlInGaP optoelectronics on stretchable substrates with applications in biomedicine and robotics. , 2010, Nature materials.
[54] P. Jain,et al. (CdSe)ZnS Core−Shell Quantum Dots: Synthesis and Characterization of a Size Series of Highly Luminescent Nanocrystallites , 2009 .
[55] P. Holloway,et al. Stable and efficient quantum-dot light-emitting diodes based on solution-processed multilayer structures , 2011 .
[56] Hye Rim Cho,et al. Wearable/disposable sweat-based glucose monitoring device with multistage transdermal drug delivery module , 2017, Science Advances.
[57] J. L. Zhao,et al. Improved Performance from Multilayer Quantum Dot Light‐Emitting Diodes via Thermal Annealing of the Quantum Dot Layer , 2007 .
[58] Jian Xu,et al. Employing heavy metal-free colloidal quantum dots in solution-processed white light-emitting diodes. , 2011, Nano letters.
[59] Jung Ho Yu,et al. Highly Efficient Copper-Indium-Selenide Quantum Dot Solar Cells: Suppression of Carrier Recombination by Controlled ZnS Overlayers. , 2015, ACS nano.
[60] H. Goesmann,et al. Nanoparticulate functional materials. , 2010, Angewandte Chemie.
[61] Jung Ho Yu,et al. Copper-indium-selenide quantum dot-sensitized solar cells. , 2013, Physical chemistry chemical physics : PCCP.
[62] Dae-Hyeong Kim,et al. Multifunctional wearable devices for diagnosis and therapy of movement disorders. , 2014, Nature nanotechnology.
[63] U. Banin,et al. Efficient Near-Infrared Polymer Nanocrystal Light-Emitting Diodes , 2002, Science.
[64] Norris,et al. Size dependence of exciton fine structure in CdSe quantum dots. , 1996, Physical review. B, Condensed matter.
[65] Vladimir Lesnyak,et al. Layer‐by‐Layer All‐Inorganic Quantum‐Dot‐Based LEDs: A Simple Procedure with Robust Performance , 2010 .
[66] V. Bulović,et al. Inkjet‐Printed Quantum Dot–Polymer Composites for Full‐Color AC‐Driven Displays , 2009 .
[67] Ken-Tye Yong,et al. New Generation Cadmium-Free Quantum Dots for Biophotonics and Nanomedicine. , 2016, Chemical reviews.
[68] V. Bulović,et al. Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer. , 2007, Nano letters.
[69] Hye Rim Cho,et al. An endoscope with integrated transparent bioelectronics and theranostic nanoparticles for colon cancer treatment , 2015, Nature Communications.
[70] Jongha Lee. Synthesis, Photophysics and Applications of Organic Excited-state Intramolecular Proton Transfer (ESIPT) Materials , 2012 .
[71] Ja Hoon Koo,et al. Colloidal Synthesis of Uniform‐Sized Molybdenum Disulfide Nanosheets for Wafer‐Scale Flexible Nonvolatile Memory , 2016, Advanced materials.
[72] Andre K. Geim,et al. Electric Field Effect in Atomically Thin Carbon Films , 2004, Science.
[73] Eun Kyung Lee,et al. Full-colour quantum dot displays fabricated by transfer printing , 2011 .
[74] Hyung Joon Shim,et al. Wearable Electrocardiogram Monitor Using Carbon Nanotube Electronics and Color-Tunable Organic Light-Emitting Diodes. , 2017, ACS nano.
[75] Xiao Wei Sun,et al. Highly flexible, electrically driven, top-emitting, quantum dot light-emitting stickers. , 2014, ACS nano.
[76] Heng Zhang,et al. Cadmium-Free InP/ZnSeS/ZnS Heterostructure-Based Quantum Dot Light-Emitting Diodes with a ZnMgO Electron Transport Layer and a Brightness of Over 10 000 cd m-2. , 2017, Small.
[77] V. Bulović,et al. Selection of metal oxide charge transport layers for colloidal quantum dot LEDs. , 2009, ACS nano.
[78] Taeghwan Hyeon,et al. A wearable multiplexed silicon nonvolatile memory array using nanocrystal charge confinement , 2016, Science Advances.
[79] Francesco Galeotti,et al. High-Efficiency All-Solution-Processed Light-Emitting Diodes Based on Anisotropic Colloidal Heterostructures with Polar Polymer Injecting Layers. , 2015, Nano letters.
[80] Byungki Kim,et al. White‐Light‐Emitting Diodes with Quantum Dot Color Converters for Display Backlights , 2010, Advanced materials.
[81] Yongwoo Kwon,et al. Over 40 cd/A efficient green quantum dot electroluminescent device comprising uniquely large-sized quantum dots. , 2014, ACS nano.
[82] Taeghwan Hyeon,et al. Nanomaterial‐Based Soft Electronics for Healthcare Applications , 2016 .
[83] Jung Ho Yu,et al. Advances in the Colloidal Synthesis of Two-Dimensional Semiconductor Nanoribbons , 2013 .
[84] Risto Myllylä,et al. Display Technology Letters Inkjet Printed RGB Quantum Dot-Hybrid LED , 2010 .
[85] Jinju Zheng,et al. Shell-dependent electroluminescence from colloidal CdSe quantum dots in multilayer light-emitting diodes , 2009 .
[86] Jingkang Wang,et al. Near‐Band‐Edge Electroluminescence from Heavy‐Metal‐Free Colloidal Quantum Dots , 2011, Advanced materials.
[87] T. Hyeon,et al. Fabric‐Based Integrated Energy Devices for Wearable Activity Monitors , 2014, Advanced materials.
[88] M. Kaltenbrunner,et al. Ultraflexible organic photonic skin , 2016, Science Advances.
[89] Nathan T. Shewmon,et al. High-efficiency, low turn-on voltage blue-violet quantum-dot-based light-emitting diodes. , 2015, Nano letters.
[90] Eiji Ohtani,et al. Electroluminescence from single monolayers of nanocrystals in molecular organic devices , 2022 .
[91] NoSoung Myoung,et al. Highly Efficient, Color-Reproducible Full-Color Electroluminescent Devices Based on Red/Green/Blue Quantum Dot-Mixed Multilayer. , 2015, ACS nano.
[92] M. Petruska,et al. Multicolor light-emitting diodes based on semiconductor nanocrystals encapsulated in GaN charge injection layers. , 2005, Nano letters.
[93] Taeghwan Hyeon,et al. Fully Stretchable Optoelectronic Sensors Based on Colloidal Quantum Dots for Sensing Photoplethysmographic Signals. , 2017, ACS nano.
[94] Liang Li,et al. One-pot synthesis of highly luminescent InP/ZnS nanocrystals without precursor injection. , 2008, Journal of the American Chemical Society.
[95] Kookheon Char,et al. InP@ZnSeS, Core@Composition Gradient Shell Quantum Dots with Enhanced Stability , 2011 .
[96] P. Guyot-Sionnest,et al. Synthesis and Characterization of Strongly Luminescing ZnS-Capped CdSe Nanocrystals , 1996 .
[97] Ja Hoon Koo,et al. Nanomaterials for bioelectronics and integrated medical systems , 2018, Korean Journal of Chemical Engineering.
[98] D. Jeon,et al. White Light‐Emitting Diodes with Excellent Color Rendering Based on Organically Capped CdSe Quantum Dots and Sr3SiO5:Ce3+,Li+ Phosphors , 2008, Advanced materials.
[99] Lee Soon Park,et al. Highly luminescent InP/GaP/ZnS nanocrystals and their application to white light-emitting diodes. , 2012, Journal of the American Chemical Society.
[100] Oleksandr Voznyy,et al. Highly efficient quantum dot near-infrared light-emitting diodes , 2016, Nature Photonics.
[101] Igor L. Medintz,et al. Meta-analysis of cellular toxicity for cadmium-containing quantum dots. , 2016, Nature nanotechnology.
[102] Lin-Wang Wang,et al. Two- versus three-dimensional quantum confinement in indium phosphide wires and dots , 2003, Nature materials.
[103] Donghee Son,et al. Deformable devices with integrated functional nanomaterials for wearable electronics , 2016, Nano Convergence.
[104] Gil Ju Lee,et al. Wearable Force Touch Sensor Array Using a Flexible and Transparent Electrode , 2017 .
[105] Cherie R. Kagan,et al. Long-range resonance transfer of electronic excitations in close-packed CdSe quantum-dot solids. , 1996, Physical review. B, Condensed matter.
[106] Tonino Greco,et al. Semitransparent quantum dot light-emitting diodes by cadmium-free colloidal quantum dots. , 2014, Journal of nanoscience and nanotechnology.
[107] Taeghwan Hyeon,et al. Digital Doping in Magic-Sized CdSe Clusters. , 2016, ACS nano.
[108] G. Gigli,et al. Hybrid Light‐Emitting Diodes from Microcontact‐Printing Double‐Transfer of Colloidal Semiconductor CdSe/ZnS Quantum Dots onto Organic Layers , 2008 .
[109] R. Janssen,et al. Red, green, and blue quantum dot LEDs with solution processable ZnO nanocrystal electron injection layers , 2008 .
[110] G. Bacher,et al. Solution-Processed CuInS2-Based White QD-LEDs with Mixed Active Layer Architecture. , 2017, ACS applied materials & interfaces.
[111] J. Vela,et al. "Giant" multishell CdSe nanocrystal quantum dots with suppressed blinking. , 2008, Journal of the American Chemical Society.
[112] Hye Rim Cho,et al. Stretchable and Transparent Biointerface Using Cell‐Sheet–Graphene Hybrid for Electrophysiology and Therapy of Skeletal Muscle , 2016 .
[113] Jung Ho Yu,et al. High-resolution three-photon biomedical imaging using doped ZnS nanocrystals. , 2013, Nature materials.
[114] Ji Hoon Kim,et al. Reverse‐Micelle‐Induced Porous Pressure‐Sensitive Rubber for Wearable Human–Machine Interfaces , 2014, Advanced materials.
[115] Shuming Chen,et al. Highly transparent quantum-dot light-emitting diodes with sputtered indium-tin-oxide electrodes , 2016 .
[116] P. Holloway,et al. High-efficiency light-emitting devices based on quantum dots with tailored nanostructures , 2013, Nature Photonics.
[117] Yi Cui,et al. Solution-processed metal nanowire mesh transparent electrodes. , 2008, Nano letters.
[118] Moonsub Shim,et al. High efficiency and optical anisotropy in double-heterojunction nanorod light-emitting diodes. , 2015, ACS nano.
[119] B. Dubertret,et al. Towards non-blinking colloidal quantum dots. , 2008, Nature materials.
[120] M. Bawendi,et al. Synthesis and characterization of nearly monodisperse CdE (E = sulfur, selenium, tellurium) semiconductor nanocrystallites , 1993 .
[121] Patrick J. Whitham,et al. Luminescent Colloidal Semiconductor Nanocrystals Containing Copper: Synthesis, Photophysics, and Applications. , 2016, Chemical reviews.
[122] Taeghwan Hyeon,et al. Ultrathin Quantum Dot Display Integrated with Wearable Electronics , 2017, Advanced materials.
[123] Young Min Song,et al. Human eye-inspired soft optoelectronic device using high-density MoS2-graphene curved image sensor array , 2017, Nature Communications.
[124] J. Rogers,et al. Inorganic semiconducting materials for flexible and stretchable electronics , 2017, npj Flexible Electronics.
[125] Taeghwan Hyeon,et al. Ultra‐Wideband Multi‐Dye‐Sensitized Upconverting Nanoparticles for Information Security Application , 2017, Advanced materials.
[126] A. Jen,et al. Efficient CdSe/CdS quantum dot light-emitting diodes using a thermally polymerized hole transport layer. , 2006, Nano letters.
[127] T. Someya,et al. Stretchable active-matrix organic light-emitting diode display using printable elastic conductors. , 2009, Nature materials.
[128] Christophe Lincheneau,et al. Chemistry of InP Nanocrystal Syntheses , 2016 .
[129] Minbaek Lee,et al. Stretchable carbon nanotube charge-trap floating-gate memory and logic devices for wearable electronics. , 2015, ACS nano.
[130] David Battaglia,et al. Colloidal InP nanocrystals as efficient emitters covering blue to near-infrared. , 2007, Journal of the American Chemical Society.
[131] James S. Speck,et al. Prospects for LED lighting , 2009 .
[132] Claire M. Lochner,et al. All-organic optoelectronic sensor for pulse oximetry , 2014, Nature Communications.
[133] Samarth S. Raut,et al. Electromechanical cardioplasty using a wrapped elasto-conductive epicardial mesh , 2016, Science Translational Medicine.
[134] Heesun Yang,et al. High-Efficiency Cu–In–S Quantum-Dot-Light-Emitting Device Exceeding 7% , 2016 .
[135] John A Rogers,et al. High-resolution patterns of quantum dots formed by electrohydrodynamic jet printing for light-emitting diodes. , 2015, Nano letters.
[136] Yizheng Jin,et al. Quantum‐Dot Light‐Emitting Diodes for Large‐Area Displays: Towards the Dawn of Commercialization , 2017, Advanced materials.
[137] Andre K. Geim,et al. The rise of graphene. , 2007, Nature materials.
[138] Zhibin Yu,et al. Elastomeric polymer light-emitting devices and displays , 2013, Nature Photonics.
[139] Xiaogang Peng,et al. Epitaxial Growth of Highly Luminescent CdSe/CdS Core/Shell Nanocrystals with Photostability and Electronic Accessibility , 1997 .
[140] K. Char,et al. Highly efficient cadmium-free quantum dot light-emitting diodes enabled by the direct formation of excitons within InP@ZnSeS quantum dots. , 2013, ACS nano.
[141] M. Bawendi,et al. Electroluminescence from heterostructures of poly(phenylene vinylene) and inorganic CdSe nanocrystals , 1998 .
[142] Victor I. Klimov,et al. Lifetime blinking in nonblinking nanocrystal quantum dots , 2012, Nature Communications.
[143] Yonggang Huang,et al. Printed Assemblies of Inorganic Light-Emitting Diodes for Deformable and Semitransparent Displays , 2009, Science.
[144] Jung-Tak Seo,et al. Fully transparent quantum dot light-emitting diode integrated with graphene anode and cathode. , 2014, ACS nano.
[145] Cherie R. Kagan,et al. Electronic energy transfer in CdSe quantum dot solids. , 1996, Physical review letters.
[146] M. Bawendi,et al. Renal clearance of quantum dots , 2007, Nature Biotechnology.
[147] Byeong Kwon Ju,et al. Transparent InP Quantum Dot Light‐Emitting Diodes with ZrO2 Electron Transport Layer and Indium Zinc Oxide Top Electrode , 2016 .
[148] Yi Cui,et al. Scalable coating and properties of transparent, flexible, silver nanowire electrodes. , 2010, ACS nano.
[149] R. Ghaffari,et al. Recent Advances in Flexible and Stretchable Bio‐Electronic Devices Integrated with Nanomaterials , 2016, Advanced materials.
[150] M. Kovalenko,et al. Prospects of colloidal nanocrystals for electronic and optoelectronic applications. , 2010, Chemical reviews.
[151] Yun Cheol Han,et al. Highly Transparent and Flexible Organic Light‐Emitting Diodes with Structure Optimized for Anode/Cathode Multilayer Electrodes , 2015 .
[152] Young Bum Lee,et al. Stretchable Heater Using Ligand-Exchanged Silver Nanowire Nanocomposite for Wearable Articular Thermotherapy. , 2015, ACS nano.
[153] Hye Rim Cho,et al. A graphene-based electrochemical device with thermoresponsive microneedles for diabetes monitoring and therapy. , 2016, Nature nanotechnology.
[154] Dong Jun Lee,et al. Transparent and Stretchable Interactive Human Machine Interface Based on Patterned Graphene Heterostructures , 2015 .
[155] Myeongjin Park,et al. Influence of Shell Thickness on the Performance of Light‐Emitting Devices Based on CdSe/Zn1‐XCdXS Core/Shell Heterostructured Quantum Dots , 2014, Advanced materials.
[156] Kyoung Won Cho,et al. Thermally Controlled, Patterned Graphene Transfer Printing for Transparent and Wearable Electronic/Optoelectronic System , 2015 .
[157] Jong-Hyun Ahn,et al. Extremely efficient flexible organic light-emitting diodes with modified graphene anode , 2012, Nature Photonics.
[158] Taeghwan Hyeon,et al. Chemical Synthesis, Doping, and Transformation of Magic-Sized Semiconductor Alloy Nanoclusters. , 2017, Journal of the American Chemical Society.
[159] Taeghwan Hyeon,et al. Extremely Vivid, Highly Transparent, and Ultrathin Quantum Dot Light‐Emitting Diodes , 2018, Advanced materials.
[160] Yizheng Jin,et al. Solution-processed, high-performance light-emitting diodes based on quantum dots , 2014, Nature.