Large deviations of the dynamical activity in the East model: analysing structure in biased trajectories

We consider large deviations of the dynamical activity in the East model. We bias this system to larger than average activity and investigate the structure that emerges. To best characterize this structure, we exploit the fact that there are effective interactions that would reproduce the same behaviour in an equilibrium system. We combine numerical results with linear response theory and variational estimates of these effective interactions, giving the first insights into such interactions in a many-body system, across a wide range of biases. The system exhibits a hierarchy of responses to the bias, remaining quasi-equilibrated on short length scales, but deviating far from equilibrium on large length scales. We discuss the connection between this hierarchy and the hierarchical ageing behaviour of the system.

[1]  Alan D. Sokal,et al.  Regularity properties and pathologies of position-space renormalization-group transformations , 1991 .

[2]  C. Landim,et al.  Towards a Nonequilibrium Thermodynamics: A Self-Contained Macroscopic Description of Driven Diffusive Systems , 2008, 0807.4457.

[3]  Jorge Kurchan,et al.  Fluctuation theorem for stochastic dynamics , 1998 .

[4]  C. Maes,et al.  The Restriction of the Ising Model to a Layer , 1998, math/9810094.

[5]  F. Martinelli,et al.  Relaxation times of kinetically constrained spin models with glassy dynamics , 2006, cond-mat/0603745.

[6]  G. Crooks Path-ensemble averages in systems driven far from equilibrium , 1999, cond-mat/9908420.

[7]  E. Cohen,et al.  Dynamical ensembles in stationary states , 1995, chao-dyn/9501015.

[8]  The Fluctuation Theorem as a Gibbs Property , 1998, math-ph/9812015.

[9]  V. Popkov,et al.  ASEP on a ring conditioned on enhanced flux , 2010 .

[10]  R. Jack,et al.  Space-time phase transitions in the East model with a softened kinetic constraint. , 2012, The Journal of chemical physics.

[11]  F. van Wijland,et al.  Equilibriumlike fluctuations in some boundary-driven open diffusive systems. , 2009, Physical review. E, Statistical, nonlinear, and soft matter physics.

[12]  A. Baule,et al.  Nonequilibrium statistical mechanics of shear flow: invariant quantities and current relations , 2009, 0911.1145.

[13]  David Chandler,et al.  Space-time thermodynamics of the glass transition. , 2005, Proceedings of the National Academy of Sciences of the United States of America.

[14]  A. Sokal,et al.  Regularity properties and pathologies of position-space renormalization-group transformations: Scope and limitations of Gibbsian theory , 1991, hep-lat/9210032.

[15]  C. Jarzynski Nonequilibrium Equality for Free Energy Differences , 1996, cond-mat/9610209.

[16]  Chaotic properties of systems with Markov dynamics. , 2005, Physical review letters.

[17]  Peter Sollich,et al.  Glassy dynamics in the asymmetrically constrained kinetic Ising chain. , 2003, Physical review. E, Statistical, nonlinear, and soft matter physics.

[18]  C. Maes,et al.  Time-symmetric fluctuations in nonequilibrium systems. , 2006, Physical Review Letters.

[19]  V. Lecomte,et al.  Thermodynamic Formalism for Systems with Markov Dynamics , 2007 .

[20]  U. Schollwoeck The density-matrix renormalization group in the age of matrix product states , 2010, 1008.3477.

[21]  Ericka Stricklin-Parker,et al.  Ann , 2005 .

[22]  Numerical study of a fragile three-dimensional kinetically constrained model. , 2004, The journal of physical chemistry. B.

[23]  Persi Diaconis,et al.  The Asymmetric One-Dimensional Constrained Ising Model: Rigorous Results , 2002 .

[24]  J. P. Garrahan,et al.  Preparation and relaxation of very stable glassy states of a simulated liquid. , 2011, Physical review letters.

[25]  J. Hooyberghs,et al.  Density-matrix renormalization-group study of current and activity fluctuations near nonequilibrium phase transitions. , 2008, Physical review. E, Statistical, nonlinear, and soft matter physics.

[26]  Peter Sollich,et al.  Large deviations and ensembles of trajectories in stochastic models , 2009, 0911.0211.

[27]  J. Jäckle,et al.  A hierarchically constrained kinetic Ising model , 1991 .

[28]  J. P. Garrahan,et al.  First-order dynamical phase transition in models of glasses: an approach based on ensembles of histories , 2008, 0810.5298.

[29]  R. Evans,et al.  Comment on `Detailed balance has a counterpart in non-equilibrium steady states' , 2004, 0901.4879.

[30]  J. P. Garrahan,et al.  Dynamic Order-Disorder in Atomistic Models of Structural Glass Formers , 2009, Science.

[31]  T. Speck,et al.  First-order phase transition in a model glass former: coupling of local structure and dynamics. , 2012, Physical review letters.

[32]  David Chandler,et al.  Transition path sampling: throwing ropes over rough mountain passes, in the dark. , 2002, Annual review of physical chemistry.

[33]  J. P. Garrahan,et al.  Dynamics on the way to forming glass: bubbles in space-time. , 2009, Annual review of physical chemistry.

[34]  Space-time thermodynamics and subsystem observables in a kinetically constrained model of glassy materials. , 2006, The Journal of chemical physics.

[35]  Hugo Touchette,et al.  Nonequilibrium microcanonical and canonical ensembles and their equivalence. , 2013, Physical review letters.

[36]  D. Ruelle,et al.  Ergodic theory of chaos and strange attractors , 1985 .

[37]  J. P. Garrahan,et al.  Metastable states and space-time phase transitions in a spin-glass model. , 2009, Physical review. E, Statistical, nonlinear, and soft matter physics.

[38]  A. Baule,et al.  Properties of a nonequilibrium heat bath. , 2007, Physical review. E, Statistical, nonlinear, and soft matter physics.

[39]  J. P. Garrahan,et al.  Finite-temperature critical point of a glass transition , 2010, Proceedings of the National Academy of Sciences.

[40]  H. Touchette The large deviation approach to statistical mechanics , 2008, 0804.0327.

[41]  Glassy Time-Scale Divergence and Anomalous Coarsening in a Kinetically Constrained Spin Chain , 1999, cond-mat/9904136.

[42]  B. Derrida,et al.  Current fluctuations in nonequilibrium diffusive systems: an additivity principle. , 2004, Physical review letters.

[43]  D. Simon Construction of a coordinate Bethe ansatz for the asymmetric simple exclusion process with open boundaries , 2009, 0903.4968.

[44]  Peter Harrowell,et al.  How reproducible are dynamic heterogeneities in a supercooled liquid? , 2004, Physical review letters.

[45]  J P Garrahan,et al.  Dynamical first-order phase transition in kinetically constrained models of glasses. , 2007, Physical review letters.

[46]  Invariant quantities in shear flow. , 2008, Physical review letters.

[47]  V. Popkov,et al.  Transition Probabilities and Dynamic Structure Function in the ASEP Conditioned on Strong Flux , 2010, 1011.3913.

[48]  R M L Evans Rules for transition rates in nonequilibrium steady states. , 2004, Physical review letters.

[49]  J. Lebowitz,et al.  A Gallavotti–Cohen-Type Symmetry in the Large Deviation Functional for Stochastic Dynamics , 1998, cond-mat/9811220.

[50]  David Chandler,et al.  Geometrical explanation and scaling of dynamical heterogeneities in glass forming systems. , 2002, Physical review letters.

[51]  Peter Sollich,et al.  Glassy dynamics of kinetically constrained models , 2002, cond-mat/0210382.