Giant resonance for the actinide nuclei: Photoneutron and photofission cross sections for U-235, U-236, U-238, and Th-232

The photoneutron cross sections sigma (..gamma..,n) and sigma (..gamma..,2n), and total photofission cross sections sigma (..gamma..,F) have been measured for /sup 235/U, /sup 236/U, /sup 238/U, and /sup 232/Th from threshold to 18.3 MeV using monoenergetic photons from the annihilation in flight of fast positrons and neutron-multiplicity detection in an efficient 4..pi.. neutron detector. Use of the ring-ratio technique allowed both the average photofission neutron energy for each nucleus to be obtained as a function of photon energy and, for /sup 236/U and /sup 238/U, the determination of the partial cross sections for first-chance sigma (..gamma.., f ) and second-chance sigma (..gamma..,n f ) photofission as well. Information extracted from the data includes integrated cross sections and their moments, giant-resonance parameters, deformation and radius parameters, and relative and absolute neutron and fission probabilities.

[1]  J. Huizenga,et al.  Photofission and Photoneutron Emission in Uranium , 1953 .

[2]  G. Baldwin,et al.  Photo-Fission in Heavy Elements , 1947 .

[3]  B. Back,et al.  Fission of doubly even actinide nuclei induced by direct reactions , 1974 .

[4]  R. C. Morrison,et al.  Photofission cross sections of 238U and 235U from 5.0 MeV to 8.0 MeV , 1973 .

[5]  A. S. Soldatov,et al.  Deep subbarrier anomalies in the photofission of heavy nuclei , 1977 .

[6]  J. T. Caldwell,et al.  GIANT RESONANCE IN DEFORMED NUCLEI: PHOTONEUTRON CROSS SECTIONS FOR $sup 153$Eu, $sup 160$Gd, $sup 165$Ho, AND $sup 186$W. , 1969 .

[7]  J. T. Caldwell,et al.  Photoneutron Cross Sections for Zr 90 , Zr 91 , Zr 92 , Zr 94 , and Y 89 , 1967 .

[8]  A. Gavron,et al.  GAMMA/sub n//GAMMA/sub f/ for actinide nuclei using (/sup 3/He, df) and (/sup 3/He, tf) reactions , 1976 .

[9]  M. Vetter,et al.  NUCLEAR INTRINSIC QUADRUPOLE MOMENTS AND DEFORMATION PARAMETERS , 1970 .

[10]  B. Berman,et al.  Photoneutron cross sections of ^{58}Ni and ^{60}Ni , 1974 .

[11]  B. L. Berman,et al.  Measurements of the giant dipole resonance with monoenergetic photons , 1975 .

[12]  J. T. Caldwell,et al.  PHOTONEUTRON CROSS SECTIONS OF $sup 141$Pr AND $sup 127$I FROM THRESHOLD TO 33 Mev , 1966 .

[13]  J. Terrell Distributions of Fission Neutron Numbers , 1957 .

[14]  K. Mcneill,et al.  PHOTONEUTRON EMISSION FROM Th232, U233, U238, AND Pu239 , 1957 .

[15]  A. H. Wapstra,et al.  The 1977 atomic mass evaluation: in four parts part II. Nuclear-reaction and separation energies , 1977 .

[16]  I. C. Nascimento,et al.  Present status of photofission of actinides near threshold. [Review, cross sections, threshold energy angular distribution] , 1976 .

[17]  M. Danos On the long-range correlation model of the photonuclear effect , 1958 .

[18]  J. T. Caldwell,et al.  Experimental Determination of Photofission Neutron Multiplicities for Eight Isotopes in the Mass Range 232 ≤ A ≤ 239 , 1975 .

[19]  H. Beil,et al.  Giant dipole resonance in N = 82 nuclei , 1971 .

[20]  J. D. Cramer,et al.  FISSION OF ODD-A URANIUM AND PLUTONIUM ISOTOPES EXCITED BY (d,p), (t,d), AND (t,p) REACTIONS. , 1970 .

[21]  Niels Bohr,et al.  The Mechanism of nuclear fission , 1939 .

[22]  J. T. Caldwell,et al.  Photoneutron Cross Sections for Sn 116 , Sn 117 , Sn 118 , Sn 119 , Sn 120 , Sn 124 , and Indium , 1969 .

[23]  A. M. Khan,et al.  Photofission of 232Th, 282U and 235U near threshold using a variable energy beam of γ-rays , 1972 .

[24]  R. C. Morrison,et al.  Photofission cross sections of 232Th and 236U from threshold to 8 MeV , 1973 .

[25]  R. E. Sund,et al.  $sup 141$Pr($gamma$,n) CROSS SECTION FROM THRESHOLD TO 24 MeV. , 1970 .

[26]  J. Goldemberg,et al.  The 232Th(γ, n)231Th cross section near threshold , 1974 .

[27]  L. Lindgren,et al.  Photoinduced fission of the doubly even uranium isotopes 234U, 236U and 238U , 1978 .

[28]  G. Gurevich,et al.  Giant resonance in the total photoabsorption cross section of Z ≈ 90 nuclei , 1976 .

[29]  J. T. Caldwell,et al.  Experimental Determination of Photofission Neutron Multiplicities for 235U, 236U, 238U, and 232Th Using Monoenergetic Photons , 1980 .

[30]  P. Axel,et al.  U 238 and Th 232 Photofission and Photoneutron Emission near Threshold , 1975 .

[31]  C. Bowman,et al.  Very low energy photofission of $sup 238$U , 1975 .

[32]  W. Stephens,et al.  Photo-Fission of Uranium and Thorium , 1940 .

[33]  J. Huizenga,et al.  Photofission cross sections of several nuclei with mono-energetic gamma rays , 1962 .

[34]  B. Back,et al.  Fission of odd-A and doubly odd actinide nuclei induced by direct reactions , 1974 .

[35]  A. Gavron,et al.  Complexity of the potential-energy surface for fission of /sup 238/U , 1977 .

[36]  C. Bowman,et al.  PHOTODISINTEGRATION OF U$sup 23$$sup 5$ , 1964 .

[37]  J. Goldemberg,et al.  Intermediate structure in the photoneutron and photofission cross sections in 238U and 232Th , 1972 .

[38]  John R. Huizenga,et al.  Photofission and Photoneutron Emission in Thorium and Uranium , 1956 .

[39]  A. Leprêtre,et al.  A study of the photofission and photoneutron processes in the giant dipole resonance of 232Th, 238U and 237Np , 1973 .

[40]  J. D. Cramer,et al.  FISSION STUDIES OF THORIUM, URANIUM, AND PLUTONIUM ISOTOPES WITH (t,pf) REACTIONS. , 1970 .