Major PM10 source location by a spatial multivariate receptor model

We present a multivariate receptor model for identifying the spatial location of major PM10 pollution sources through the concentrations at multiple monitoring stations. We build on a mixed multiplicative log-normal factor model adjusting the source contributions for meteorological covariates and for temporal correlation and considering source profiles as compositional Gaussian random fields, to account for the variability induced by the spatial distribution of the monitoring sites. Taking a Bayesian approach to estimation, the proposed hierarchical model is implemented and used to analyze average daily PM10 concentration measurements from 13 monitoring sites in Taranto, Italy, for the period April–December 2005. Three major sources of pollution are identified and characterized in terms of their spatial and temporal behavior and in relation to meteorological data.

[1]  S. Shen,et al.  The statistical analysis of compositional data , 1983 .

[2]  Brent A. Coull,et al.  Multiplicative factor analysis with a latent mixed model structure for air pollution exposure assessment , 2011 .

[3]  Bradley P. Carlin,et al.  Bayesian measures of model complexity and fit , 2002 .

[4]  Alessio Pollice,et al.  Spatiotemporal analysis of the PM10 concentration over the Taranto area , 2010, Environmental monitoring and assessment.

[5]  Peter Guttorp,et al.  Locating major PM10 source areas in Seoul using multivariate receptor modeling , 2004, Environmental and Ecological Statistics.

[6]  Pentti Paatero,et al.  Advanced factor analysis of spatial distributions of PM2.5 in the eastern United States. , 2003, Environmental science & technology.

[7]  W. Stahel,et al.  Linear Unmixing of Multivariate Observations , 2005 .

[8]  B. Kedem,et al.  Bayesian Prediction of Transformed Gaussian Random Fields , 1997 .

[9]  D. Billheimer Spatial Models for Discrete Compositional Data , 2007 .

[10]  Alessio Pollice,et al.  Recent statistical issues in multivariate receptor models , 2011 .

[11]  David D Billheimer,et al.  Compositional receptor modeling , 2001 .

[12]  Ronald C. Henry,et al.  Bilinear estimation of pollution source profiles and amounts by using multivariate receptor models , 2002 .

[13]  John Aitchison,et al.  The Statistical Analysis of Compositional Data , 1986 .

[14]  Peter Guttorp,et al.  Multivariate receptor models and model uncertainty , 2002 .

[15]  D. Gamerman,et al.  Spatial dynamic factor analysis , 2008 .

[16]  Thomas Lumley,et al.  Predicting intra‐urban variation in air pollution concentrations with complex spatio‐temporal dependencies , 2009, Environmetrics.

[17]  William F. Christensen,et al.  Dirichlet based Bayesian multivariate receptor modeling , 2008 .

[18]  Jeff W. Lingwall,et al.  Iterated confirmatory factor analysis for pollution source apportionment , 2006 .