Double Fano-type resonances in heptamer-hole array transmission spectra with high refractive index sensing

Nanohole arrays or individual nanohole oligomers in metallic films have attracted intense attention due to their unique optical properties such as extraordinary optical transmission or Fano resonance. However, the nanohole oligomer array still remains largely unexplored. In this work, we numerically investigate the heptamer-hole arrays in an optically thin silver film, which can support double Fano-type resonances in the transmission spectra. The two Fano-type transmissions arise from the interference between the non-resonant direct transmission through holes and the resonant indirect scatterings based on the excitations of surface plasmons polaritons (SPPs, set up by the array periodicity) and a sub-radiant localized surface plasmon resonance (LSPR, arising from the anti-bonding hybridization between the central and the surrounding holes). Because of their different physical mechanisms, the two Fano resonances can be tuned independently. In addition, the LSPR-related Fano resonance shows an ultra-high sensitivity to surrounding dielectric medium with a figure of merit of 25 due to its sub-radiant feature, far larger than the SPP-related Fano resonance, offering tremendous potentials for plasmonic biosensors.

[1]  Ajay Nahata,et al.  Transmission resonances through aperiodic arrays of subwavelength apertures , 2007, Nature.

[2]  W. A. Murray,et al.  Surface plasmon polaritons and their role in the enhanced transmission of light through periodic arrays of subwavelength holes in a metal film. , 2004, Physical review letters.

[3]  Mikael Käll,et al.  Plasmonic sensing characteristics of single nanometric holes. , 2005, Nano letters.

[4]  Stefan Enoch,et al.  Role of shape and localized resonances in extraordinary transmission through periodic arrays of subwavelength holes: Experiment and theory , 2005 .

[5]  K. Crozier,et al.  Experimental study of the interaction between localized and propagating surface plasmons. , 2009, Optics letters.

[6]  Federico Capasso,et al.  DNA-enabled self-assembly of plasmonic nanoclusters. , 2011, Nano letters.

[7]  J. P. Woerdman,et al.  Fano-type interpretation of red shifts and red tails in hole array transmission spectra , 2003, physics/0401054.

[8]  Enhanced transmission through arrays of subwavelength holes in gold films coated by a finite dielectric layer , 2007, physics/0703092.

[9]  R. W. Christy,et al.  Optical Constants of the Noble Metals , 1972 .

[10]  Mohsen Rahmani,et al.  Subgroup decomposition of plasmonic resonances in hybrid oligomers: modeling the resonance lineshape. , 2012, Nano letters.

[11]  H. Raether Surface Plasmons on Smooth and Rough Surfaces and on Gratings , 1988 .

[12]  George C. Schatz,et al.  Nanosphere Lithography: Effect of Substrate on the Localized Surface Plasmon Resonance Spectrum of Silver Nanoparticles , 2001 .

[13]  N. Zheludev,et al.  Nanohole array as a lens. , 2008, Nano letters.

[14]  H. Lezec,et al.  Effects of hole depth on enhanced light transmission through subwavelength hole arrays , 2002 .

[15]  Federico Capasso,et al.  Self-Assembled Plasmonic Nanoparticle Clusters , 2010, Science.

[16]  W. Barnes,et al.  Surface plasmon subwavelength optics , 2003, Nature.

[17]  Xiaofeng Li,et al.  Plasmonic Fano resonances in nanohole quadrumers for ultra-sensitive refractive index sensing. , 2014, Nanoscale.

[18]  Federico Capasso,et al.  Fano-like interference in self-assembled plasmonic quadrumer clusters. , 2010, Nano letters.

[19]  C. Mirkin,et al.  Localized surface plasmon resonance spectroscopy of single silver triangular nanoprisms. , 2006, Nano letters.

[20]  H. Lezec,et al.  Extraordinary optical transmission through sub-wavelength hole arrays , 1998, Nature.

[21]  A Paul Alivisatos,et al.  Transition from isolated to collective modes in plasmonic oligomers. , 2010, Nano letters.

[22]  Thomas W. Ebbesen,et al.  Surface plasmons enhance optical transmission through subwavelength holes , 1998 .

[23]  J. Dionne,et al.  Controlling the interplay of electric and magnetic modes via Fano-like plasmon resonances. , 2011, Nano letters.

[24]  Junqiao Wang,et al.  A giant localized field enhancement and high sensitivity in an asymmetric ring by exhibiting Fano resonance , 2013 .

[25]  M. Käll,et al.  Sensing characteristics of NIR localized surface plasmon resonances in gold nanorings for application as ultrasensitive biosensors. , 2007, Nano letters.

[26]  M. Kahrizi,et al.  Optical behaviour of thick gold and silver films with periodic circular nanohole arrays , 2012 .

[27]  Stephen Gray,et al.  Surface plasmon generation and light transmission by isolated nanoholes and arrays of nanoholes in thin metal films. , 2005, Optics express.

[28]  Peter Nordlander,et al.  Fano resonances in plasmonic nanoparticle aggregates. , 2009, The journal of physical chemistry. A.

[29]  Teri W Odom,et al.  Multiscale patterning of plasmonic metamaterials. , 2007, Nature nanotechnology.

[30]  M. Hentschel,et al.  Babinet to the half: coupling of solid and inverse plasmonic structures. , 2013, Nano letters.

[31]  Ajay Nahata,et al.  Role of metal film thickness on the enhanced transmission properties of a periodic array of subwavelength apertures. , 2005, Optics express.

[32]  Pei Ding,et al.  Dual-band perfect absorption and field enhancement by interaction between localized and propagating surface plasmons in optical metamaterials , 2011 .

[33]  N. V. van Hulst,et al.  Strong influence of hole shape on extraordinary transmission through periodic arrays of subwavelength holes. , 2004, Physical review letters.

[34]  Thomas W. Ebbesen,et al.  The role of localized surface plasmon modes in the enhanced transmission of periodic subwavelength apertures , 2005 .

[35]  Peter Nordlander,et al.  Symmetry breaking in plasmonic nanocavities: subradiant LSPR sensing and a tunable Fano resonance. , 2008, Nano letters.

[36]  J. Lakowicz,et al.  Imaging three-dimensional light propagation through periodic nanohole arrays using scanning aperture microscopy. , 2007, Applied physics letters.

[37]  U. Eigenthaler,et al.  Planar metamaterial analogue of electromagnetically induced transparency for plasmonic sensing. , 2010, Nano letters.

[38]  Borja Sepúlveda,et al.  Nanohole plasmons in optically thin gold films , 2007 .