Influence of alloy buffer and capping layers on InAs/GaAs quantum dot formation

We have investigated the influence of alloy buffer and capping layers on the shape, size, and density of self-assembled InAs/GaAs quantum dots. Cross-sectional scanning tunneling microscopy (XSTM) images reveal ellipse-shaped dots with highest (lowest) diameter, height, and density, for dots with (without) surrounding alloy layers. Furthermore, the wetting layer is thicker in the presence of the alloy layers. We propose a strain-based mechanism for dot formation and collapse in the absence and presence of alloy buffer and capping layers. This mechanism is likely to be applicable to a wide range of lattice-mismatched thin-film systems.

[1]  Siddhartha Ghosh,et al.  QUANTUM DOT OPTO-ELECTRONIC DEVICES , 2004 .

[2]  Andreas Stintz,et al.  Characterization of InAs quantum dots in strained InxGa1-xAs quantum wells , 2000 .

[3]  M. S. Skolnick,et al.  Optimizing the growth of 1.3 μm InAs/InGaAs dots-in-a-well structure , 2003 .

[4]  N. Yokoyama,et al.  Interdiffusion between InAs Quantum Dots and GaAs Matrices. , 1997 .

[5]  K. Kern,et al.  Interplay between thermodynamics and kinetics in the capping of InAs/GaAs(001) quantum dots. , 2006, Physical review letters.

[6]  M. Kawashima,et al.  Low-Temperature Growth of GaAs and AlAs-GaAs Quantum-Well Layers by Modified Molecular Beam Epitaxy , 1986 .

[7]  M. Hopkinson,et al.  Atomic scale study of the impact of the strain and composition of the capping layer on the formation of InAs quantum dots , 2007 .

[8]  G. E. Cirlin,et al.  STM and RHEED study of InAsGaAs quantum dots obtained by submonolayer epitaxial techniques , 1996 .

[9]  P. Bhattacharya,et al.  Interdiffusion and surface segregation in stacked self-assembled InAs/GaAs quantum dots , 1999 .

[10]  P. Bhattacharya,et al.  Lateral indium–indium pair correlations within the wetting layers of buried InAs/GaAs quantum dots , 2002 .

[11]  Il Ki Han,et al.  Influence of arsenic during indium deposition on the formation of the wetting layers of InAs quantum dots grown by migration enhanced epitaxy , 2004 .

[12]  Yuhai Tu,et al.  Origin of apparent critical thickness for island formation in heteroepitaxy. , 2004, Physical review letters.

[13]  R. Goldman,et al.  Nanometer-scale measurements of electronic states in InAs/GaAs quantum dots , 2009 .

[14]  M. Hopkinson,et al.  Nature of the Stranski-Krastanow transition during epitaxy of InGaAs on GaAs. , 2001, Physical review letters.

[15]  A. Holmes,et al.  Spatial correlation-anticorrelation in strain-driven self-assembled InGaAs quantum dots , 2004 .

[16]  B. A. Joyce,et al.  Composition of InAs quantum dots on GaAs(001): Direct evidence for (In,Ga)As alloying , 1998 .

[17]  Jen-Wei Pan,et al.  Formation of self-organized In0.5Ga0.5As quantum dots on GaAs by molecular beam epitaxy , 1997 .

[18]  P. Frigeri,et al.  InAs/GaAs self-assembled quantum dots grown by ALMBE and MBE , 1997 .

[19]  Rachel S. Goldman Nanoprobing of semiconductor heterointerfaces: quantum dots, alloys and diffusion , 2004 .

[20]  O. Schmidt,et al.  Shape evolution of InAs quantum dots during overgrowth , 2003 .