INDOEX aerosol: A comparison and summary of chemical, microphysical, and optical properties observed from land, ship, and aircraft

converged on values of about 3.8 ± 0.3 m 2 g � 1 , providing a firm constraint upon the description and modeling of haze optical properties. MSE values trended lower with more dilute haze but became more variable in clean air or regions of low concentrations. This cross-platform comparison resolved a number of measurement differences but also revealed that regional characterization from different platforms results in differences linked to variability in time and space. This emphasizes the need to combine such efforts with coordinated satellite and modeling studies able to characterize large-scale regional structure and variability. These comparisons also indicate that ‘‘closure’’ between chemical, microphysical, and optical properties across platforms to better than about 20% will require significant improvements in techniques, calibration procedures, and comparison efforts. INDEX TERMS: 0305 Atmospheric Composition and Structure: Aerosols and particles (0345, 4801); 0345 Atmospheric Composition and Structure: Pollution—urban and regional (0305); 0394 Atmospheric Composition and Structure: Instruments and techniques; KEYWORDS: INDOEX, data comparison, optical properties, chemistry, microphysics, size distributions

[1]  T. Kirchstetter,et al.  Carbonaceous aerosols over the Indian Ocean during INDOEX: Chemical characterization, optical properties and probable sources , 2004 .

[2]  T. Kirchstetter,et al.  Carbonaceous aerosols over the Indian Ocean during the Indian Ocean Experiment (INDOEX): Chemical characterization, optical properties, and probable sources , 2002 .

[3]  P. Quinn,et al.  Regional marine boundary layer aerosol size distributions in the Indian, Atlantic, and Pacific Oceans: A comparison of INDOEX measurements with ACE‐1, ACE‐2, and Aerosols99 , 2002 .

[4]  P. Quinn,et al.  Carbonaceous aerosol over the Indian Ocean: OC/EC fractions and selected specifications from size‐segregated onboard samples , 2002 .

[5]  M. Andreae,et al.  Chemical characterization of submicron aerosol particles collected over the Indian Ocean , 2002 .

[6]  A. Ansmann,et al.  An intercomparison of aerosol light extinction and 180° backscatter as derived using in situ instruments and Raman lidar during the INDOEX field campaign , 2002 .

[7]  A. Jefferson,et al.  Spatial variability of submicrometer aerosol radiative properties over the Indian Ocean during INDOEX , 2002 .

[8]  J. Prospero,et al.  Marine biogenic and anthropogenic contributions to non‐sea‐salt sulfate in the marine boundary layer over the North Atlantic Ocean , 2002 .

[9]  David J. Delene,et al.  Variability of Aerosol Optical Properties at Four North American Surface Monitoring Sites , 2002 .

[10]  Glenn E. Shaw,et al.  Indian Ocean Experiment: An integrated analysis of the climate forcing and effects of the great Indo-Asian haze , 2001 .

[11]  M. L. Laucks,et al.  An Evaluation of the Community Aerosol Inlet for the NCAR C-130 Research Aircraft , 2001 .

[12]  V. Ramanathan,et al.  Latitude gradient in aerosol properties across the Inter Tropical Convergence Zone: results from the joint Indo-US study onboard Sagar Kanya , 2001 .

[13]  P. Quinn,et al.  Surface submicron aerosol chemical composition : What fraction is not sulfate? , 2000 .

[14]  D. Covert,et al.  Size-segregated chemical, gravimetric and number distribution-derived mass closure of the aerosol in Sagres, Portugal during ACE-2 , 2000 .

[15]  B. Huebert,et al.  Uncertainties in data on organic aerosols , 2000 .

[16]  D. Covert,et al.  Hygroscopic properties of aerosol particles in the north-eastern Atlantic during ACE-2 , 2000 .

[17]  Barbara J. Turpin,et al.  Measuring and simulating particulate organics in the atmosphere: problems and prospects , 2000 .

[18]  J. D. Wheeler,et al.  Aerosol backscatter fraction and single scattering albedo: Measured values and uncertainties at a coastal station in the Pacific Northwest , 1999 .

[19]  Michael J. Kleeman,et al.  Size and composition distribution of atmospheric particles in southern California , 1999 .

[20]  Michael J. Kleeman,et al.  Size and Composition Distribution of Fine Particulate Matter Emitted from Wood Burning, Meat Charbroiling, and Cigarettes , 1999 .

[21]  Tami C. Bond,et al.  Calibration and Intercomparison of Filter-Based Measurements of Visible Light Absorption by Aerosols , 1999 .

[22]  A. Clarke,et al.  Nucleation in the equatorial free troposphere: Favorable environments during PEM‐Tropics , 1999 .

[23]  Peter V. Hobbs,et al.  Humidification factors for atmospheric aerosols off the mid‐Atlantic coast of the United States , 1999 .

[24]  D. Blake,et al.  Emission factors of hydrocarbons, halocarbons, trace gases and particles from biomass burning in Brazil , 1998 .

[25]  D. Blake,et al.  Physical, chemical, and optical properties of regional hazes dominated by smoke in Brazil , 1998 .

[26]  P. Quinn,et al.  Local closure during the First Aerosol Characterization Experiment (ACE 1): Aerosol mass concentration and scattering and backscattering coefficients , 1998 .

[27]  P. Quinn,et al.  Aerosol optical properties in the marine boundary layer during the First Aerosol Characterization Experiment (ACE 1) and the underlying chemical and physical aerosol properties , 1998 .

[28]  D. Covert,et al.  Comparison of directly measured CCN with CCN modeled from the number-size distribution in the marine boundary layer during ACE 1 at Cape Grim, Tasmania , 1998 .

[29]  J. Ogren,et al.  Determining Aerosol Radiative Properties Using the TSI 3563 Integrating Nephelometer , 1998 .

[30]  J. Hudson,et al.  Intercomparison Study of the Size-Dependent Counting Efficiency of 26 Condensation Particle Counters , 1997 .

[31]  F. Stratmann,et al.  A new data inversion algorithm for DMPS-measurements , 1996 .

[32]  M. Kulmala,et al.  Formation of respirable particles during ski waxing , 1996 .

[33]  R. Cary,et al.  Elemental Carbon-Based Method for Monitoring Occupational Exposures to Particulate Diesel Exhaust , 1996 .

[34]  C. Liousse,et al.  Particulate content of savanna fire emissions , 1995 .

[35]  D. Baumgardner,et al.  Interpretation of measurements made by the forward scattering spectrometer probe (FSSP-300) during the Airborne Arctic Stratospheric Expedition , 1992 .

[36]  Kenneth L. Rubow,et al.  A Microorifice Uniform Deposit Impactor (MOUDI): Description, Calibration, and Use , 1991 .

[37]  A. Clarke A thermo-optic technique for in situ analysis of size-resolved aerosol physicochemistry , 1991 .

[38]  A. W. Stelson URBAN AEROSOL REFRACTIVE INDEX PREDICTION BY PARTIAL MOLAR REFRACTION APPROACH , 1990 .

[39]  H. Fissan,et al.  Micro-orifice uniform deposit impactor , 1986 .

[40]  D. Garvey,et al.  Response Characteristics of the Particle Measuring Systems Active Scattering Aerosol Spectrometer Probe (ASASP–X) , 1983 .

[41]  Benjamin Y. H. Liu,et al.  Sampling of carbon fiber aerosols , 1983 .

[42]  P. Walker Particulate carbon atmospheric life cycle: Edited by George T. Wolff and Richard L. Klimisch, Plenum Press, New York, 1982. 411 pp. $49.50 , 1982 .

[43]  G. Wolff,et al.  Particulate carbon, atmospheric life cycle , 1982 .

[44]  I. Tang,et al.  Aerosol growth studies—III ammonium bisulfate aerosols in a moist atmosphere , 1977 .

[45]  E. Sawicki,et al.  Ion Chromatographic Analysis of Sulfate and Nitrate in Ambient Aerosols , 1976 .