Ultrabroadband single-cycle terahertz pulses with peak fields of 300 kV cm−1 from a metallic spintronic emitter

We explore the capabilities of metallic spintronic thin-film stacks as a source of intense and broadband terahertz electromagnetic fields. For this purpose, we excite a W/CoFeB/Pt trilayer (thickness of 5.6 nm) on a large-area glass substrate (diameter of 7.5 cm) by a femtosecond laser pulse (energy 5.5 mJ, duration 40 fs, and wavelength 800 nm). After focusing, the emitted terahertz pulse is measured to have a duration of 230 fs, a peak field of 300 kV cm−1, and an energy of 5 nJ. In particular, the waveform exhibits a gapless spectrum extending from 1 to 10 THz at 10% of its amplitude maximum, thereby facilitating nonlinear control over matter in this difficult-to-reach frequency range on the sub-picosecond time scale.

[1]  William L. Barnes,et al.  Mechanisms of THz generation from silver nanoparticle and nanohole arrays illuminated by 100 fs pulses of infrared light , 2014 .

[2]  M. Hoffmann,et al.  Nonlinear Terahertz Spectroscopy , 2012 .

[3]  T. Huisman,et al.  THz Emission Spectroscopy for THz Spintronics , 2017 .

[4]  T. Kampfrath,et al.  Terahertz-field-induced optical birefringence in common window and substrate materials. , 2015, Optics express.

[5]  B. Liu,et al.  Generation of narrowband, high-intensity, carrier-envelope phase-stable pulses tunable between 4 and 18 THz , 2017, 2017 Conference on Lasers and Electro-Optics (CLEO).

[6]  Rupert Huber,et al.  Tracking the ultrafast motion of a single molecule by femtosecond orbital imaging , 2016, Nature.

[7]  K. Tanaka,et al.  Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3 and applications to nonlinear optics , 2011, Other Conferences.

[8]  S. Ganichev,et al.  Intense terahertz excitation of semiconductors , 2006 .

[9]  Tobias Kampfrath,et al.  Sampling of broadband terahertz pulses with thick electro-optic crystals , 2007 .

[10]  E. Abraham,et al.  Terahertz Kerr effect in Gallium Phosphide crystal , 2014, 2014 39th International Conference on Infrared, Millimeter, and Terahertz waves (IRMMW-THz).

[11]  A. Cavalleri,et al.  Nonlinear light–matter interaction at terahertz frequencies , 2016, 1608.05611.

[12]  Ronger Zheng,et al.  Powerful and Tunable THz Emitters Based on the Fe/Pt Magnetic Heterostructure , 2016, 1607.02814.

[13]  张存林 Zhang Cunlin,et al.  Terahertz Spectroscopy and Imaging , 2010 .

[14]  M Unlu,et al.  Significant performance enhancement in photoconductive terahertz optoelectronics by incorporating plasmonic contact electrodes. , 2013, Nature communications.

[15]  Alfred Leitenstorfer,et al.  Phase-locked generation and field-resolved detection of widely tunable terahertz pulses with amplitudes exceeding 100 MV/cm. , 2008, Optics letters.

[16]  F. Freimuth,et al.  Terahertz spin current pulses controlled by magnetic heterostructures. , 2012, Nature nanotechnology.

[17]  P. Planken,et al.  Emission of terahertz pulses from nanostructured metal surfaces , 2014 .

[18]  T. Elsaesser,et al.  Focus: Phase-resolved nonlinear terahertz spectroscopy--From charge dynamics in solids to molecular excitations in liquids. , 2015, The Journal of chemical physics.

[19]  Yang Liu,et al.  High‐Performance THz Emitters Based on Ferromagnetic/Nonmagnetic Heterostructures , 2016, Advanced materials.

[20]  Yan Zhang,et al.  Extreme terahertz science , 2017, Nature Photonics.

[21]  Jairo Sinova,et al.  Experimental observation of the spin-Hall effect in a two-dimensional spin-orbit coupled semiconductor system. , 2005 .

[22]  G. Jakob,et al.  Efficient metallic spintronic emitters of ultrabroadband terahertz radiation , 2016 .

[23]  D. A. Kleinman,et al.  Infrared Lattice Bands of Quartz , 1961 .

[24]  Clemens Ruchert,et al.  Strong-field single-cycle THz pulses generated in an organic crystal , 2011 .

[25]  S. Hunsche,et al.  Detectors and sources for ultrabroadband electro-optic sampling: Experiment and theory , 1999 .

[26]  K. Nelson,et al.  Resonant and nonresonant control over matter and light by intense terahertz transients , 2013, Nature Photonics.

[27]  J. Coey,et al.  Narrow-band tunable terahertz emission from ferrimagnetic Mn3-xGa thin films , 2016 .

[28]  B. Monoszlai,et al.  Highly efficient scalable monolithic semiconductor terahertz pulse source , 2016 .

[29]  Wei Han,et al.  Enhanced spin–orbit torques by oxygen incorporation in tungsten films , 2016, Nature Communications.

[30]  Tobias Kampfrath,et al.  Terahertz field enhancement via coherent superposition of the pulse sequences after a single optical-rectification crystal , 2014 .

[31]  Yung-Jun Yoo,et al.  Generation of strong terahertz fields exceeding 8 MV/cm at 1 kHz and real-time beam profiling , 2014 .

[32]  S. Maekawa,et al.  Observation of the spin Seebeck effect , 2008, Nature.

[33]  M. Justus,et al.  High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter , 2016, Scientific Reports.

[34]  A. Taylor,et al.  High-Power Broadband Terahertz Generation via Two-Color Photoionization in Gases , 2012, IEEE Journal of Quantum Electronics.

[35]  Kai-Erik Peiponen,et al.  Terahertz spectroscopy and imaging , 2013 .

[36]  Ely E. Bell,et al.  Measurement of the optical constants of crystal quartz in the far infrared with the asymmetric Fourier-transform method , 1967 .

[37]  Cyril C. Renaud,et al.  The 2017 terahertz science and technology roadmap , 2017, Journal of Physics D: Applied Physics.

[38]  R. Rosenfeld Nature , 2009, Otolaryngology--head and neck surgery : official journal of American Academy of Otolaryngology-Head and Neck Surgery.

[39]  C Vicario,et al.  High efficiency THz generation in DSTMS, DAST and OH1 pumped by Cr:forsterite laser. , 2015, Optics express.

[40]  A. Schneider Beam-size effects in electro-optic sampling of terahertz pulses. , 2009, Optics letters.

[41]  D. Grischkowsky,et al.  Terahertz time-domain spectroscopy characterization of the far-infrared absorption and index of refraction of high-resistivity, float-zone silicon , 2004 .

[42]  K. Nelson,et al.  Terahertz Kerr effect , 2009, 0907.5081.

[43]  K. Nelson,et al.  A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses , 2015 .