Formation mechanisms of sub-wavelength ripples during femtosecond laser pulse train processing of dielectrics

A new model is proposed to investigate femtosecond laser pulse train processing of dielectrics by including the laser wave properties in the photon particle properties based plasma model. In the case studies, the pulse duration is 50?fs and the pulse delays are 0, 25, 50 and 75?fs. Both the laser wave?particle duality and transient localized changes of material properties are considered in the proposed model, and the formation mechanism of sub-wavelength ripples is revealed. This study shows that the interference between surface plasmons and laser field plays a key role in the formation of sub-wavelength ripples for which the excitation of surface plasmons is necessary. The predicted period of sub-wavelength ripples is in agreement with the experiments.

[1]  Philippe M. Fauchet,et al.  Stimulated Wood's anomalies on laser-illuminated surfaces , 1986 .

[2]  D. C. Emmony,et al.  Laser mirror damage in germanium at 10.6 μm , 1973 .

[3]  E. V. Chulkov,et al.  Theory of surface plasmons and surface-plasmon polaritons , 2007 .

[4]  Heinz Sturm,et al.  Chemical, morphological and accumulation phenomena in ultrashort-pulse laser ablation of TiN in air , 2000 .

[5]  Ming Zhou,et al.  Superhydrophobic surfaces prepared by microstructuring of silicon using a femtosecond laser. , 2006, Langmuir : the ACS journal of surfaces and colloids.

[6]  A. Rosenfeld,et al.  On the role of surface plasmon polaritons in the formation of laser-induced periodic surface structures upon irradiation of silicon by femtosecond-laser pulses , 2009 .

[7]  Jeff F. Young,et al.  Laser-induced periodic surface structure. II. Experiments on Ge, Si, Al, and brass , 1983 .

[8]  Alexander Horn,et al.  Formation of subwavelength-laser-induced periodic surface structures by tightly focused femtosecond laser radiation , 2004, International Symposium on Laser Precision Microfabrication.

[9]  Heinz Sturm,et al.  Structure formation on the surface of indium phosphide irradiated by femtosecond laser pulses , 2005 .

[10]  Jens Gottmann,et al.  Sub-wavelength ripple formation on dielectric and metallic materials induced by tightly focused femto-second laser radiation , 2006, SPIE LASE.

[11]  W. Kautek,et al.  Physico-chemical aspects of femtosecond-pulse-laser-induced surface nanostructures , 2005 .

[12]  Gerard Mourou,et al.  SHORT-PULSE LASER DAMAGE IN TRANSPARENT MATERIALS AS A FUNCTION OF PULSE DURATION , 1999 .

[13]  Jörg Krüger,et al.  Femtosecond laser interaction with silicon under water confinement , 2004 .

[14]  Florenta Costache,et al.  Ripples revisited: non-classical morphology at the bottom of femtosecond laser ablation craters in transparent dielectrics , 2002 .

[15]  Gerard Mourou,et al.  Laser‐induced breakdown by impact ionization in SiO2 with pulse widths from 7 ns to 150 fs , 1994 .

[16]  B. Luther-Davies,et al.  Ablation of solids by femtosecond lasers: ablation mechanism and ablation thresholds for metals and dielectrics , 2002 .

[17]  Chunlei Guo,et al.  Colorizing metals with femtosecond laser pulses , 2008 .

[18]  J. Meyer-ter-Vehn,et al.  Hydrodynamic simulation of subpicosecond laser interaction with solid-density matter , 2000, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[19]  Lan Jiang,et al.  Prediction of crater shape in femtosecond laser ablation of dielectrics , 2004 .

[20]  Perry,et al.  Nanosecond-to-femtosecond laser-induced breakdown in dielectrics. , 1996, Physical review. B, Condensed matter.

[21]  Lan Jiang,et al.  Repeatable nanostructures in dielectrics by femtosecond laser pulse trains , 2005 .

[22]  Radiative tail of realistic rotating gravitational collapse , 1999, Physical review letters.

[23]  Guillaume Petite,et al.  Dynamics of femtosecond laser interactions with dielectrics , 2004 .

[24]  G. Mourou,et al.  Femtosecond Optical Breakdown in Dielectrics , 1998 .

[25]  Ruediger Grunwald,et al.  Femtosecond laser-induced periodic surface structures revisited: A comparative study on ZnO , 2009 .

[26]  Perry,et al.  Laser-induced damage in dielectrics with nanosecond to subpicosecond pulses. , 1995, Physical review letters.

[27]  Chunlei Guo,et al.  Ultrafast dynamics of femtosecond laser-induced periodic surface pattern formation on metals , 2005 .

[28]  John E. Sipe,et al.  Laser-Induced Periodic Surface Structure on Solids: A Universal Phenomenon , 1982 .

[29]  O. Misochko Nonclassical states of lattice excitations: squeezed and entangled phonons , 2013 .

[30]  Chunlei Guo,et al.  Formation of extraordinarily uniform periodic structures on metals induced by femtosecond laser pulses , 2006 .

[31]  Mengyan Shen,et al.  Femtosecond Laser-Induced Formation Of Submicrometer Spikes On Silicon In Water , 2004 .

[32]  E. Audouard,et al.  Controlled nanostructrures formation by ultra fast laser pulses for color marking. , 2010, Optics express.

[33]  Jeff F. Young,et al.  Laser-induced periodic surface structure. I. Theory , 1983 .

[34]  Karen Willcox,et al.  Kinetics and kinematics for translational motions in microgravity during parabolic flight. , 2009, Aviation, space, and environmental medicine.

[35]  M. Birnbaum Semiconductor Surface Damage Produced by Ruby Lasers , 1965 .