Spectral diffusion time scales in InGaN/GaN quantum dots

A detailed temporal analysis of the spectral diffusion phenomenon in single photon emitting InGaN/GaN quantum dots (QDs) is performed via measurements of both time-varying emission spectra and single photon emission intensity autocorrelation times. Excitation dependent phenomena are investigated via the optical excitation of carriers into the GaN barrier material and also directly into InGaN. Excitation into InGaN reveals that the fastest environmental fluctuations occur on timescales as long as a few hundreds of nanoseconds: an order of magnitude longer than previously measured in GaN QDs. Such long time scales may in future allow for the generation of indistinguishable photons in spite of the fact that the experimentally measured linewidths are broad.A detailed temporal analysis of the spectral diffusion phenomenon in single photon emitting InGaN/GaN quantum dots (QDs) is performed via measurements of both time-varying emission spectra and single photon emission intensity autocorrelation times. Excitation dependent phenomena are investigated via the optical excitation of carriers into the GaN barrier material and also directly into InGaN. Excitation into InGaN reveals that the fastest environmental fluctuations occur on timescales as long as a few hundreds of nanoseconds: an order of magnitude longer than previously measured in GaN QDs. Such long time scales may in future allow for the generation of indistinguishable photons in spite of the fact that the experimentally measured linewidths are broad.

[1]  Y. Arakawa,et al.  III-nitride quantum dots as single photon emitters , 2019, Semiconductor Science and Technology.

[2]  J. Jarman,et al.  Improvement of single photon emission from InGaN QDs embedded in porous micropillars , 2018, Applied Physics Letters.

[3]  Sejeong Kim,et al.  Site-Selective, Two-Photon Plasmonic Nanofocusing on a Single Quantum Dot for Near-Room-Temperature Operation , 2018 .

[4]  M. Holmes,et al.  Nanosecond-scale spectral diffusion in the single photon emission of a GaN quantum dot , 2017 .

[5]  Y. Arakawa,et al.  Temperature dependence of the single photon emission from interface-fluctuation GaN quantum dots , 2017, Scientific Reports.

[6]  Christian Schneider,et al.  High-efficiency multiphoton boson sampling , 2017, Nature Photonics.

[7]  Yasuhiko Arakawa,et al.  Ultraclean Single Photon Emission from a GaN Quantum Dot. , 2017, Nano letters.

[8]  J. Jarman,et al.  Wafer-scale Fabrication of Non-Polar Mesoporous GaN Distributed Bragg Reflectors via Electrochemical Porosification , 2017, Scientific Reports.

[9]  M. Fuhrer,et al.  Room‐Temperature Single‐Photon Emission from Oxidized Tungsten Disulfide Multilayers , 2017 .

[10]  Y. Arakawa,et al.  Single-photon emission at 1.5 μm from an InAs/InP quantum dot with highly suppressed multi-photon emission probabilities , 2016 .

[11]  Y. Arakawa,et al.  Single Photons from a Hot Solid-State Emitter at 350 K , 2016 .

[12]  I. Sagnes,et al.  Near-optimal single-photon sources in the solid state , 2015, Nature Photonics.

[13]  G. Weihs,et al.  Optimal excitation conditions for indistinguishable photons from quantum dots , 2015, 1507.07404.

[14]  S. Tomić,et al.  Visible Spectrum Quantum Light Sources Based on InxGa1–xN/GaN Quantum Dots , 2015 .

[15]  Jian-Wei Pan,et al.  Quantum teleportation of multiple degrees of freedom of a single photon , 2015, Nature.

[16]  Y. Arakawa,et al.  Excitonic complexes in single zinc-blende GaN/AlN quantum dots grown by droplet epitaxy , 2014 .

[17]  P. Bhattacharya,et al.  Electrically pumped single-photon emission at room temperature from a single InGaN/GaN quantum dot , 2014 .

[18]  Igor Aharonovich,et al.  Distinctive signature of indium gallium nitride quantum dot lasing in microdisk cavities , 2014, Proceedings of the National Academy of Sciences.

[19]  C. Kindel,et al.  Spectral diffusion in nitride quantum dots: Emission energy dependent linewidths broadening via giant built‐in dipole moments , 2014 .

[20]  Y. Arakawa,et al.  Room-temperature triggered single photon emission from a III-nitride site-controlled nanowire quantum dot. , 2014, Nano letters.

[21]  Y. Arakawa,et al.  Single-photon emission from cubic GaN quantum dots , 2013 .

[22]  F. Oehler,et al.  Non‐polar (11$ \bar 2 $0) InGaN quantum dots with short exciton lifetimes grown by metal‐organic vapour phase epitaxy , 2013, 1305.5801.

[23]  C. Bougerol,et al.  Subnanosecond spectral diffusion measurement using photon correlation , 2010, 1207.0676.

[24]  Hiroto Sekiguchi,et al.  Emission color control from blue to red with nanocolumn diameter of InGaN/GaN nanocolumn arrays grown on same substrate , 2010 .

[25]  B. Daudin Polar and nonpolar GaN quantum dots , 2008 .

[26]  P. Cochat,et al.  Et al , 2008, Archives de pediatrie : organe officiel de la Societe francaise de pediatrie.

[27]  H. J. Kimble,et al.  The quantum internet , 2008, Nature.

[28]  Yasuhiko Arakawa,et al.  A gallium nitride single-photon source operating at 200 K , 2006, Nature materials.

[29]  Dieter Schuh,et al.  Optically programmable electron spin memory using semiconductor quantum dots , 2004, Nature.

[30]  C. Humphreys,et al.  Temporal variation in photoluminescence from single InGaN quantum dots , 2004 .

[31]  Robert A. Taylor,et al.  InGaN quantum dots grown by metalorganic vapor phase epitaxy employing a post-growth nitrogen anneal , 2003 .

[32]  Kyo Inoue,et al.  Secure communication: Quantum cryptography with a photon turnstile , 2002, Nature.

[33]  Yoshihisa Yamamoto,et al.  Indistinguishable photons from a single-photon device , 2002, Nature.

[34]  P. Petroff,et al.  A quantum dot single-photon turnstile device. , 2000, Science.

[35]  Nicolas Grandjean,et al.  From visible to white light emission by GaN quantum dots on Si(111) substrate , 1999 .

[36]  M. Bawendi,et al.  Quantum-confined stark effect in single CdSe nanocrystallite quantum dots , 1997, Science.

[37]  T. S. P. S.,et al.  GROWTH , 1924, Nature.

[38]  M. Holmes,et al.  Growth and optical characterisation of multilayers of InGaN quantum dots , 2012 .