Influence of Substrate Stage Temperature and Rotation Rate on the Magneto-Optical Quality of RF-Sputtered Bi2.1Dy0.9Fe3.9Ga1.1O12 Garnet Thin Films

Highly bismuth-substituted iron garnet thin films are prepared on quartz substrates by using a radio frequency (RF) magnetron sputtering technique. We study the factors (process parameters associated with the RF magnetron sputter deposition technique) affecting the magneto-optical (MO) properties of ferrite garnet films of composition Bi2.1Dy0.9Fe3.9Ga1.1O12. All films show high MO response across the visible range of wavelengths after being annealed. In particular, the effects of substrate stage temperature and rotation rate on the various properties of films are studied. Experimental results reveal that the characteristics of garnet films of this type can be tuned and optimized for use in various magnetic field-driven nanophotonics and integrated optics devices, and that, at a substrate stage rotation rate near 16 revolutions per minute, the MO quality of the developed MO films is the best, in comparison with films deposited at other rotation rates. To the best of our knowledge, this is the first report on the effects of deposition parameters on the properties of garnet films of this stoichiometry.

[1]  G. Scott,et al.  Magnetooptic properties and applications of bismuth substituted iron garnets , 1976 .

[2]  T. Ishibashi,et al.  Magneto-optical properties of Bi-substituted yttrium iron garnet films by metal-organic decomposition method , 2010 .

[3]  K. Alameh,et al.  RF magnetron sputtered (BiDy)3(FeGa)5O12:Bi2O3 composite garnet-oxide materials possessing record magneto-optic quality in the visible spectral region. , 2009, Optics express.

[4]  Roman Sobolewski,et al.  Magneto-optical modulator for superconducting digital output interface , 2001 .

[5]  P. Paroli,et al.  Magneto-optical devices based on garnet films , 1984 .

[6]  Tanja Neumann,et al.  Elements Of X Ray Diffraction , 2016 .

[7]  A. Zvezdin,et al.  Modern magnetooptics and magnetooptical materials , 1997 .

[8]  T. Hibiya,et al.  Refractive index of Bi‐substituted gadolinium iron garnet films grown by liquid‐phase epitaxy , 1985 .

[9]  Andrew H. Eschenfelder,et al.  Magnetic Bubble Technology , 1980 .

[10]  I. Mayergoyz,et al.  Growth effects (rotation rate) on the characteristics of bismuth substituted lutetium iron garnets , 2004 .

[11]  K. Alameh,et al.  High-performance RF-sputtered Bi-substituted iron garnet thin films with almost in-plane magnetization , 2017 .

[13]  Completely Bi-Substituted Iron Garnet (BIG) Films Prepared by Electron Cyclotron Resonance (ECR) Sputtering , 1992 .

[14]  B. Cullity,et al.  Elements of X-ray diffraction , 1957 .

[15]  Huaiwu Zhang,et al.  Effects of off-stoichiometry and density on the magnetic and magneto-optical properties of yttrium iron garnet films by magnetron sputtering method , 2010 .

[16]  K. Alameh,et al.  Growth, Characterisation, And Properties of Bi1.8Lu1.2Fe3.6Al1.4O12 Garnet Films Prepared Using Two Different Substrate Temperatures , 2014 .

[17]  K. Alameh,et al.  Plasmon-mediated magneto-optical transparency , 2013, Nature Communications.

[18]  A. Grishin,et al.  Bi/sub 3/Fe/sub 5/O/sub 12/ thin film visualizer , 2001 .

[19]  Joonhee Kang,et al.  Fabrication and characterization of Bi-substituted yttrium iron garnet films by pulsed laser deposition , 2003 .

[20]  T. Suzuki Magnetic and magneto‐optic properties of rapid thermally crystallized garnet films (invited) , 1991 .

[21]  Lars Hultman,et al.  Microstructural evolution during film growth , 2003 .

[22]  D. S. Misra,et al.  The influence of substrate temperature and annealing on the properties of pulsed laser-deposited YIG films on fused quartz substrate , 2008 .

[23]  J. Thornton The microstructure of sputter-deposited coatings , 1986 .

[24]  Y. T. Lee,et al.  Annealing behaviour and crystal structure of RF-sputtered Bi-substituted dysprosium iron-garnet films having excess co-sputtered Bi-oxide content , 2011 .