Path-selective lasing in nanostructures based on molecular control of localized surface plasmons.

We propose a new type of nanodevice, capable of both path-selectivity and anisotropic lasing, that is based on loss-compensation and amplification by a localized plasmon polariton. The nanodevice is a Y-shaped plasmonic nanostructure embedded in an anisotropic host medium with gain. The anisotropy leads to path selectivity, an effect which is more pronounced once gain is included. Such a device is potentially realizable via bottom-up techniques. The path-selectivity may be coupled with activation of a rotation of the anisotropic host medium for inducing a light-guiding switching functionality.

[1]  G. M. Akselrod,et al.  Ultrafast Room-Temperature Single Photon Emission from Quantum Dots Coupled to Plasmonic Nanocavities. , 2016, Nano letters.

[2]  S. Aștilean,et al.  Surface-enhanced spectroscopy on plasmonic oligomers assembled by AFM nanoxerography. , 2015, Nanoscale.

[3]  Koji Fujita,et al.  Wavelength-tunable Spasing in the Visible , 2022 .

[4]  George C Schatz,et al.  Lasing action in strongly coupled plasmonic nanocavity arrays. , 2013, Nature nanotechnology.

[5]  M. Gather A rocky road to plasmonic lasers , 2012, Nature Photonics.

[6]  Philip Tinnefeld,et al.  Fluorescence Enhancement at Docking Sites of DNA-Directed Self-Assembled Nanoantennas , 2012, Science.

[7]  Y. Prior,et al.  Strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. , 2012, Physical review letters.

[8]  Nicolas Bonod,et al.  Accelerated single photon emission from dye molecule-driven nanoantennas assembled on DNA , 2012, Nature Communications.

[9]  D. Neuhauser Nanopolaritonics with a continuum of molecules: simulations of molecular-induced selectivity in plasmonics transport through a continuous Y-shape. , 2011, The Journal of chemical physics.

[10]  D. Neuhauser,et al.  Near-field: a finite-difference time-dependent method for simulation of electrodynamics on small scales. , 2011, The Journal of chemical physics.

[11]  Naomi J. Halas,et al.  Photodetection with Active Optical Antennas , 2011, Science.

[12]  Ortwin Hess,et al.  Gain and plasmon dynamics in active negative-index metamaterials , 2010, Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences.

[13]  H. Gibbs,et al.  Arrays of Ag split-ring resonators coupled to InGaAs single-quantum-well gain. , 2010, Optics express.

[14]  U. Chettiar,et al.  Loss-free and active optical negative-index metamaterials , 2010, Nature.

[15]  Ortwin Hess,et al.  Overcoming losses with gain in a negative refractive index metamaterial. , 2010, Physical review letters.

[16]  V. Shalaev,et al.  Demonstration of a spaser-based nanolaser , 2009, Nature.

[17]  A. Lemaître,et al.  Giant Rabi splitting between localized mixed plasmon-exciton states in a two-dimensional array of nanosize metallic disks in an organic semiconductor , 2009 .

[18]  M. Wegener,et al.  Self-consistent calculation of metamaterials with gain , 2009, 0907.0888.

[19]  D P Tsai,et al.  Towards the lasing spaser: controlling metamaterial optical response with semiconductor quantum dots. , 2009, Optics express.

[20]  R. Baer,et al.  Curve crossing and negative refraction in simulations of near-field coupled metallic nanoparticle arrays. , 2007, The Journal of chemical physics.

[21]  Shin‐Tson Wu,et al.  Super High Birefringence Isothiocyanato Biphenyl-Bistolane Liquid Crystals , 2004 .

[22]  D. Bergman,et al.  Surface plasmon amplification by stimulated emission of radiation: quantum generation of coherent surface plasmons in nanosystems. , 2003, Physical review letters.

[23]  Jiang,et al.  Time dependent theory for random lasers , 2000, Physical review letters.

[24]  A. Lagendijk,et al.  Resonant Scattering and Spontaneous Emission in Dielectrics: Microscopic Derivation of Local-Field Effects , 1998 .

[25]  A. Nagra,et al.  FDTD analysis of wave propagation in nonlinear absorbing and gain media , 1998 .

[26]  K. Tsakmakidis,et al.  Gain and plasmon dynamics in negative-index metamaterials , 2011 .