FORMATION AND INTERACTION OF HOLLOW NEON ATOMS AT AN ALUMINUM SURFACE

Theoretical and experimental methods were used to study the interaction of Ne 9+ ions with an Al surface. Theoretical models were applied to visualize the shape and dimension of hollow neon atoms formed above and below the surface. Atomic Hartree-Fock calculations were performed to determine the large hollow atoms produced with electrons in high Rydberg levels above the surface. Inside the first surface layers hollow atoms were evaluated by means of a Density Functional theory including non-linear screening effects. The time-dependent decay sequence of a hollow atom was determined from a cascade model that describes the filling of the L shell. The cascade model yields information about the life time and the interaction region of the hollow atom within the first layers of the surface. Experimental results obtained by means of Auger spectroscopy are used to verify the results of the model predictions.

[1]  A. Borisov,et al.  Resonant electron transfer between highly charged ions and metal surfaces: first-order vs. nonperturbative transition rates , 1996 .

[2]  Page,et al.  Multistep cascade model for the deexcitation of highly charged ions impinging on a solid surface. , 1995, Physical review. A, Atomic, molecular, and optical physics.

[3]  Page,et al.  Multiple-cascade model for the filling of hollow Ne atoms moving below an Al surface. , 1995, Physical review. A, Atomic, molecular, and optical physics.

[4]  Stolterfoht,et al.  Dynamic K- and L-shell filling of Ne9+ projectiles interacting with an Al(111) surface. , 1995, Physical review. A, Atomic, molecular, and optical physics.

[5]  Hughes,et al.  Velocity dependence of KLL Auger emission from hollow atoms formed during collisions of hydrogenic N6+ ions on surfaces. , 1995, Physical review. A, Atomic, molecular, and optical physics.

[6]  Stolterfoht,et al.  Molecular-orbital model for slow hollow atoms colliding with atoms in a solid. , 1995, Physical review. A, Atomic, molecular, and optical physics.

[7]  Page,et al.  Angular distribution of K Auger electrons ejected by highly charged ions interacting with an Al(111) surface. , 1994, Physical review. A, Atomic, molecular, and optical physics.

[8]  J. Limburg,et al.  THE INTERACTION OF HYDROGENIC IONS WITH METAL AND SEMICONDUCTOR SURFACES , 1994 .

[9]  Morgenstern,et al.  Atomic structure calculations of KLL Auger spectra from highly charged ion-solid-surface collisions. , 1994, Physical review. A, Atomic, molecular, and optical physics.

[10]  H. Rabitz,et al.  Atomic collisions with inhomogeneous solid surfaces: multiple scattering from surface defects and mixed overlayers , 1994 .

[11]  Schippers,et al.  Excitation of target Auger-electron emission by the impact of highly charged ions: N6+, O7+, and Ne9+ on Pt(110). , 1992, Physical Review A. Atomic, Molecular, and Optical Physics.

[12]  Schippers,et al.  Auger-electron emission from slow, highly charged ions interacting with solid Cu targets. , 1992, Physical review. A, Atomic, molecular, and optical physics.

[13]  Lerner,et al.  Above-surface neutralization of highly charged ions: The classical over-the-barrier model. , 1991, Physical review. A, Atomic, molecular, and optical physics.

[14]  Meyer,et al.  Evidence for above-surface and subsurface neutralization during interactions of highly charged ions with a metal target. , 1991, Physical review letters.

[15]  N. Stolterfoht Dielectronic processes and electron correlation in energetic ion-atom collisions , 1991 .

[16]  G. Lakits,et al.  On the measurement of statistics for particle-induced electron emission from a clean metal surface , 1991 .

[17]  R. Morgenstern,et al.  AUGER ELECTRONS RESULTING FROM SLOW H-LIKE IONS NEUTRALIZED NEAR A TUNGSTEN SURFACE , 1990 .

[18]  Desclaux,et al.  Production of hollow atoms by the excitation of highly charged ions in interaction with a metallic surface. , 1990, Physical review letters.

[19]  Pedro M. Echenique,et al.  Dynamic Screening of Ions in Condensed Matter , 1990 .

[20]  H. Andrä Electronic interaction of multicharged ions with metal surfaces at low velocities , 1989 .

[21]  N. Stolterfoht Near Resonant Vacancy Exchange between Inner Shells of Colliding Heavy Particles , 1987 .

[22]  Nolte,et al.  Selective production of Li-, Be-, and B-like K vacancy states in fast Ne projectiles studied by zero-degree Auger spectroscopy. , 1985, Physical review. A, General physics.

[23]  R. D. Cowan,et al.  The Theory of Atomic Structure and Spectra , 1981 .

[24]  M.M.R. Williams,et al.  The stopping and ranges of ions in matter , 1978 .

[25]  L. Sander,et al.  Self-consistent screening of a proton in jellium , 1977 .

[26]  Emilio Segrè,et al.  Nuclei And Particles , 1977 .

[27]  A. Pasyuk,et al.  Identification of multiply charged ions by electron emission , 1973 .