Optical trapping near resonance absorption.

Expressions for radiation-induced forces are presented for the case of a Rayleigh particle near the focus of a Gaussian laser beam at near-resonant conditions. Classical electromagnetic theory was used to obtain the dependence of the scattering and gradient forces on the incident laser frequency, the beam convergence angle, and the spatial position of the particle with respect to the focus. Approximative numerical analysis performed for particles with a single resonant absorption peak demonstrates the occurrence of up to 50-fold enhanced trapping forces at near-resonant frequencies. The use of this technique of gradient force enhancement may provide optical tweezers with enhanced trapping strengths and a degree of specificity.

[1]  Toshimitsu Asakura,et al.  Radiation forces on a dielectric sphere in the Rayleigh scattering regime , 1996 .

[2]  Chu,et al.  Experimental observation of optically trapped atoms. , 1986, Physical review letters.

[3]  A. Ashkin Acceleration and trapping of particles by radiation pressure , 1970 .

[4]  M. Nieto-Vesperinas,et al.  Time-averaged total force on a dipolar sphere in an electromagnetic field. , 2000, Optics letters.

[5]  Christoph F Schmidt,et al.  Laser-induced heating in optical traps. , 2003, Biophysical journal.

[6]  A. Ashkin,et al.  Optical trapping and manipulation of neutral particles using lasers. , 1997, Proceedings of the National Academy of Sciences of the United States of America.

[7]  K. Svoboda,et al.  Biological applications of optical forces. , 1994, Annual review of biophysics and biomolecular structure.

[8]  John E. Bjorkholm,et al.  Observation of Focusing of Neutral Atoms by the Dipole Forces of Resonance-Radiation Pressure , 1978 .

[9]  J. P. Barton,et al.  Fifth-order corrected electromagnetic field components for a fundamental Gaussian beam , 1989 .

[10]  J. Gordon,et al.  Motion of atoms in a radiation trap , 1980 .

[11]  A. Ashkin Forces of a single-beam gradient laser trap on a dielectric sphere in the ray optics regime. , 1992, Methods in cell biology.

[12]  D. C. Cronemeyer Optical Absorption Characteristics of Pink Ruby , 1966 .

[13]  E. M. Lifshitz,et al.  Course in Theoretical Physics , 2013 .

[14]  S. Chu,et al.  Observation of a single-beam gradient force optical trap for dielectric particles. , 1986, Optics letters.

[15]  Arthur Ashkin,et al.  Trapping of Atoms by Resonance Radiation Pressure , 1978 .

[16]  C. F. Schmidt,et al.  Thermal noise limitations on micromechanical experiments , 1998, European Biophysics Journal.

[17]  C. Dale Keefe,et al.  Curvefitting Imaginary Components of Optical Properties: Restrictions on the Lineshape Due to Causality. , 2001, Journal of molecular spectroscopy.

[18]  James P. Gordon,et al.  Radiation Forces and Momenta in Dielectric Media , 1973 .

[19]  P W Smith,et al.  Continuous-wave self-focusing and self-trapping of light in artificial Kerr media. , 1982, Optics letters.

[20]  J. Gordon,et al.  Stability of radiation-pressure particle traps: an optical Earnshaw theorem. , 1983, Optics letters.

[21]  Arthur Ashkin,et al.  Atomic-Beam Deflection by Resonance-Radiation Pressure , 1970 .

[22]  Hiroshi Masuhara,et al.  Three-Dimensional pH Microprobing with an Optically-Manipulated Fluorescent Particle , 1996 .

[23]  Bruce T. Draine,et al.  The discrete-dipole approximation and its application to interstellar graphite grains , 1988 .

[24]  Steven M. Block,et al.  Optical trapping of metallic Rayleigh particles. , 1994, Optics letters.

[25]  G. M. Hale,et al.  Optical Constants of Water in the 200-nm to 200-microm Wavelength Region. , 1973, Applied optics.

[26]  R. Rockafellar The multiplier method of Hestenes and Powell applied to convex programming , 1973 .