Electric field control of the LaAlO3/SrTiO3 interface ground state

Interfaces between complex oxides are emerging as one of the most interesting systems in condensed matter physics. In this special setting, in which translational symmetry is artificially broken, a variety of new and unusual electronic phases can be promoted. Theoretical studies predict complex phase diagrams and suggest the key role of the charge carrier density in determining the systems’ ground states. A particularly fascinating system is the conducting interface between the band insulators LaAlO3 and SrTiO3 (ref. 3). Recently two possible ground states have been experimentally identified: a magnetic state and a two-dimensional superconducting condensate. Here we use the electric field effect to explore the phase diagram of the system. The electrostatic tuning of the carrier density allows an on/off switching of superconductivity and drives a quantum phase transition between a two-dimensional superconducting state and an insulating state. Analyses of the magnetotransport properties in the insulating state are consistent with weak localization and do not provide evidence for magnetism. The electric field control of superconductivity demonstrated here opens the way to the development of new mesoscopic superconducting circuits.

[1]  Alexey V. Ustinov,et al.  The Physics of Superconductors , 1997 .

[2]  J. M. Singer,et al.  Universal Critical Quantum Properties of Cuprate Superconductors , 1997 .

[3]  D. Muller,et al.  Why some interfaces cannot be sharp , 2005, cond-mat/0510491.

[4]  R. Clarke,et al.  Structural basis for the conducting interface between LaAlO3 and SrTiO3. , 2007, Physical review letters.

[5]  Jochen Mannhart,et al.  Electrostatic modification of novel materials , 2006 .

[6]  Satoshi Okamoto,et al.  Electronic reconstruction at an interface between a Mott insulator and a band insulator , 2004, Nature.

[7]  H. Hwang Atomic Control of the Electronic Structure at Complex Oxide Heterointerfaces , 2006 .

[8]  H. Rogalla,et al.  In-situ monitoring during pulsed laser deposition of complex oxides using reflection high energy electron diffraction under high oxygen pressure , 1997 .

[9]  T. Claeson,et al.  Effect of oxygen vacancies in the SrTiO3 substrate on the electrical properties of the LaAlO3/SrTiO3 interface , 2007 .

[10]  S. M. Girvin,et al.  Continuous quantum phase transitions , 1997 .

[11]  A. Goldman,et al.  Electrostatic tuning of the superconductor-insulator transition in two dimensions. , 2005, Physical review letters.

[12]  G. Bergmann Weak Localization in Thin Films , 1986 .

[13]  M. Vojta,et al.  Fermi-liquid instabilities at magnetic quantum phase transitions , 2006, cond-mat/0606317.

[14]  K. Bouzehouane,et al.  Mapping the spatial distribution of charge carriers in LaAlO3/SrTiO3 heterostructures. , 2007, Nature materials.

[15]  J. M. Singer,et al.  Phase transition approach to high temperature superconductivity : universal properties of cuprate superconductors , 2000 .

[16]  J. Triscone,et al.  Field-effect experiments in NdBa2Cu3O7−δ ultrathin films using a SrTiO3 single-crystal gate insulator , 2003 .

[17]  Weakly localized bosons , 1998, cond-mat/9803345.

[18]  J. Mannhart,et al.  Tunable Quasi-Two-Dimensional Electron Gases in Oxide Heterostructures , 2006, Science.

[19]  John B Ketterson,et al.  The Physics of Superconductors , 2003 .

[20]  Akira Ohtomo,et al.  A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface , 2004, Nature.

[21]  Origin of charge density at LaAlO3 on SrTiO3 heterointerfaces: possibility of intrinsic doping. , 2006, Physical review letters.

[22]  U Zeitler,et al.  Magnetic effects at the interface between non-magnetic oxides. , 2007, Nature materials.

[23]  N. Reyren,et al.  Superconducting Interfaces Between Insulating Oxides , 2007, Science.

[24]  G. Bergmann,et al.  Weak localization in thin films: a time-of-flight experiment with conduction electrons , 1984 .

[25]  S. Sachdev Quantum Phase Transitions , 1999 .

[26]  Fisher,et al.  Quantum critical phenomena in charged superconductors. , 1988, Physical review letters.

[27]  J. Triscone,et al.  Electric-field-effect modulation of the transition temperature, mobile carrier density, and in-plane penetration depth of NdBa2Cu3O7-delta thin films. , 2006, Physical review letters.

[28]  Williams,et al.  Dielectric properties of sputtered SrTiO3 films. , 1994, Physical review. B, Condensed matter.

[29]  C. Ahn,et al.  Electric field effect in correlated oxide systems , 2003, Nature.

[30]  A. Fert,et al.  High mobility in LaAlO3/SrTiO3 heterostructures: origin, dimensionality, and perspectives. , 2007, Physical review letters.