A fast random walk algorithm for computing diffusion-weighted NMR signals in multi-scale porous media: A feasibility study for a Menger sponge

A fast random walk (FRW) algorithm is adapted to compute diffusion-weighted NMR signals in a Menger sponge which is formed by multiple channels of broadly distributed sizes and often considered as a model for soils and porous materials. The self-similar structure of a Menger sponge allows for rapid simulations that were not feasible by other numerical techniques. The role of multiple length scales on diffusion-weighted NMR signals is investigated.

[1]  A Mohoric,et al.  Computer simulation of the spin-echo spatial distribution in the case of restricted self-diffusion. , 2001, Journal of magnetic resonance.

[2]  Denis S. Grebenkov,et al.  NMR survey of reflected brownian motion , 2007 .

[3]  H P Huinink,et al.  Random-walk simulations of NMR dephasing effects due to uniform magnetic-field gradients in a pore. , 2002, Physical review. E, Statistical, nonlinear, and soft matter physics.

[4]  R. Lobo Microporous and Mesoporous Materials , 2014 .

[5]  G. Sposito,et al.  MODELS OF THE WATER RETENTION CURVE FOR SOILS WITH A FRACTAL PORE SIZE DISTRIBUTION , 1996 .

[6]  B. Sapoval,et al.  Restricted diffusion in a model acinar labyrinth by NMR: theoretical and numerical results. , 2007, Journal of magnetic resonance.

[7]  Per Linse,et al.  The NMR Self-Diffusion Method Applied to Restricted Diffusion. Simulation of Echo Attenuation from Molecules in Spheres and between Planes , 1993 .

[8]  Multiscaling analysis of large-scale off-lattice DLA , 1991 .

[9]  Christoph H. Arns,et al.  Numerical analysis of nuclear magnetic resonance relaxation–diffusion responses of sedimentary rock , 2011 .

[10]  Y. Chiew,et al.  Computer simulation of diffusion‐controlled reactions in dispersions of spherical sinks , 1989 .

[11]  M. E. Muller Some Continuous Monte Carlo Methods for the Dirichlet Problem , 1956 .

[12]  Ericka Stricklin-Parker,et al.  Ann , 2005 .

[13]  Denis S Grebenkov,et al.  A fast random walk algorithm for computing the pulsed-gradient spin-echo signal in multiscale porous media. , 2011, Journal of magnetic resonance.

[14]  D. Grebenkov What makes a boundary less accessible. , 2005, Physical review letters.

[15]  Paul T. Callaghan,et al.  Translational Dynamics and Magnetic Resonance: Principles of Pulsed Gradient Spin Echo NMR , 2011 .

[16]  Lee,et al.  Random-walk simulation of diffusion-controlled processes among static traps. , 1989, Physical review. B, Condensed matter.

[17]  C. Atzeni,et al.  A fractal model of the porous microstructure of earth-based materials , 2008 .

[18]  Per Linse,et al.  The Validity of the Short-Gradient-Pulse Approximation in NMR Studies of Restricted Diffusion. Simulations of Molecules Diffusing between Planes, in Cylinders and Spheres , 1995 .

[19]  Multifractal properties of the harmonic measure on Koch boundaries in two and three dimensions. , 2005, Physical review. E, Statistical, nonlinear, and soft matter physics.