Quantum oscillations in an optically-illuminated two-dimensional electron system at the LaAlO3/SrTiO3 interface

We have investigated the illumination effect on the magnetotransport properties of a two-dimensional electron system at the LaAlO3/SrTiO3 interface. The illumination significantly reduces the zero-field sheet resistance, eliminates the Kondo effect at low-temperature, and switches the negative magnetoresistance into the positive one. A large increase in the density of high-mobility carriers after illumination leads to quantum oscillations in the magnetoresistance originating from the Landau quantization. The carrier density (∼2 × 1012 cm−2) and effective mass (∼1.7m e) estimated from the oscillations suggest that the high-mobility electrons occupy the d xz/yz subbands of Ti:t2g orbital extending deep within the conducting sheet of SrTiO3. Our results demonstrate that the illumination which induces additional carriers at the interface can pave the way to control the Kondo-like scattering and study the quantum transport in the complex oxide heterostructures.

[1]  N. Pryds,et al.  Band-Order Anomaly at the γ-Al2O3/SrTiO3 Interface Drives the Electron-Mobility Boost. , 2021, ACS nano.

[2]  M. Goiran,et al.  Aperiodic quantum oscillations in the two-dimensional electron gas at the LaAlO3/SrTiO3 interface , 2019, npj Quantum Materials.

[3]  N. Pryds,et al.  Microscopic origin of the mobility enhancement at a spinel/perovskite oxide heterointerface revealed by photoemission spectroscopy , 2017, 1710.05574.

[4]  W. G. van der Wiel,et al.  Gate-Tunable Band Structure of the LaAlO_{3}-SrTiO_{3} Interface. , 2016, Physical review letters.

[5]  G. Guo,et al.  Hidden lattice instabilities as origin of the conductive interface between insulating LaAlO3 and SrTiO3 , 2016, Nature Communications.

[6]  Yucheng Jiang,et al.  Light induced suppression of Kondo effect at amorphous LaAlO3/SrTiO3 interface , 2016 .

[7]  C. J. Li,et al.  Controlling Kondo-like Scattering at the SrTiO3-based Interfaces , 2016, Scientific Reports.

[8]  M. Goiran,et al.  High field magneto-transport in two-dimensional electron gas LaAlO3/SrTiO3 , 2016, 1604.03451.

[9]  R. Dittmann,et al.  Disentanglement of growth dynamic and thermodynamic effects in LaAlO3/SrTiO3 heterostructures , 2016, Scientific Reports.

[10]  D. Koelle,et al.  Quantum interference in an interfacial superconductor. , 2015, Nature nanotechnology.

[11]  N. Pryds,et al.  Evidence of weak superconductivity at the room-temperature grown LaAlO3/SrTiO3 interface , 2015, 1510.01199.

[12]  A. Filippetti,et al.  Polaronic metal state at the LaAlO3/SrTiO3 interface , 2015, Nature Communications.

[13]  Y. Li,et al.  Visible-light-accelerated oxygen vacancy migration in strontium titanate , 2015, Scientific Reports.

[14]  C. M. Folkman,et al.  Gate-tunable superconducting weak link behavior in top-gated LaAlO3-SrTiO3 , 2015 .

[15]  L. Gor’kov Antiferromagnetism of two-dimensional electronic gas on light-irradiated SrTiO3 and at LaAlO3/SrTiO3 interfaces , 2015, Journal of physics. Condensed matter : an Institute of Physics journal.

[16]  J. Maan,et al.  Transport and thermoelectric properties of the LaAlO3/SrTiO3 interface , 2014, 1407.7433.

[17]  M. Gabay,et al.  Large modulation of the Shubnikov–de Haas oscillations by the Rashba interaction at the LaAlO3/SrTiO3 interface , 2014, 1407.4925.

[18]  H. Hwang,et al.  Quantum longitudinal and Hall transport at the LaAlO3/SrTiO3 interface at low electron densities , 2014, 1403.4343.

[19]  Dapeng Yu,et al.  Photoelectrical properties of insulating LaAlO3-SrTiO3 interfaces. , 2014, Nanoscale.

[20]  E. Altman,et al.  Competition between Kondo screening and magnetism at the LaAlO 3 / SrTiO 3 interface , 2013, 1311.4541.

[21]  P. Delugas,et al.  Doping-dependent band structure of LaAlO3/SrTiO3 interfaces by soft x-ray polarization-controlled resonant angle-resolved photoemission , 2013, 1307.6943.

[22]  V. K. Guduru Surprising magnetotransport in oxide heterostructures , 2014 .

[23]  J. Maan,et al.  Thermally excited multiband conduction in LaAlO3/SrTiO3 heterostructures exhibiting magnetic scattering , 2013, 1311.5807.

[24]  D. Muller,et al.  Interface superconductor with gap behaviour like a high-temperature superconductor , 2013, Nature.

[25]  D. Paparo,et al.  Persistent Photoconductivity in 2D Electron Gases at Different Oxide Interfaces , 2013, 1309.3120.

[26]  H. Hwang,et al.  Titanium dxy ferromagnetism at the LaAlO3/SrTiO3 interface. , 2013, Nature materials.

[27]  Jin Zhao,et al.  Giant photovoltaic effects driven by residual polar field within unit-cell-scale LaAlO3 films on SrTiO3 , 2013, Scientific Reports.

[28]  P. Christianen,et al.  Optically excited multi-band conduction in LaAlO3/SrTiO3 heterostructures , 2012, 1211.4778.

[29]  J. Maan,et al.  Quantum oscillations and subband properties of the two-dimensional electron gas at the LaAlO3/SrTiO3 interface , 2012, 1207.7003.

[30]  S. Pennycook,et al.  Electron Transfer and Ionic Displacements at the Origin of the 2D Electron Gas at the LAO/STO Interface: Direct Measurements with Atomic‐Column Spatial Resolution , 2012, Advanced materials.

[31]  M. Gabay,et al.  Rashba induced magnetoconductance oscillations in the LaAlO 3 -SrTiO 3 heterostructure , 2012, 1203.5239.

[32]  C. Bark,et al.  Localization of two-dimensional electron gas in LaAlO 3 /SrTiO 3 heterostructures , 2011, 1110.3252.

[33]  E. Altman,et al.  A universal critical density underlying the physics of electrons at the LaAlO3/SrTiO3 interface , 2011, Nature Communications.

[34]  H. Hwang,et al.  Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO3/SrTiO3 interface , 2011, 1108.3150.

[35]  T. Venkatesan,et al.  Magnetoresistance of two-dimensional and three-dimensional electron gas in LaAlO 3 /SrTiO 3 heterostructures: Influence of magnetic ordering, interface scattering, and dimensionality , 2011, 1110.5290.

[36]  P. Delugas,et al.  Spontaneous 2-dimensional carrier confinement at the n-type SrTiO3/LaAlO3 interface. , 2011, Physical review letters.

[37]  A. Palevski,et al.  Shubnikov-de Haas oscillations in SrTiO3/LaAlO3 interface. , 2010, Physical review letters.

[38]  J. Triscone,et al.  Superconductivity at the LaAlO3/SrTiO3 interface , 2009, Journal of physics. Condensed matter : an Institute of Physics journal.

[39]  R. Martin,et al.  Origin of the two-dimensional electron gas carrier density at the LaAlO3 on SrTiO3 interface. , 2008, Physical review letters.

[40]  N. Reyren,et al.  Electric field control of the LaAlO3/SrTiO3 interface ground state , 2008, Nature.

[41]  N. Reyren,et al.  Superconducting Interfaces Between Insulating Oxides , 2007, Science.

[42]  W. G. van der Wiel,et al.  Magnetic effects at the interface between non-magnetic oxides. , 2007, Nature materials.

[43]  Akira Ohtomo,et al.  A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface , 2004, Nature.

[44]  A. Wilson,et al.  The theory of the magneto-resistance effects in metals , 1947, Proceedings of the Royal Society of London. Series A. Mathematical and Physical Sciences.

[45]  M. Lifshitz Theory of Magnetic Susceptibility in Metals at Low Temperatures , 2022 .