Radiation effects in concrete for nuclear power plants – Part I: Quantification of radiation exposure and radiation effects

A large fraction of light water reactor (LWR) construction utilizes concrete, including safety-related structures such as the biological shielding and containment building. Concrete is an inherently complex material, with the properties of concrete structures changing over their lifetime due to the intrinsic nature of concrete and influences from local environment. As concrete structures within LWRs age, the total neutron fluence exposure of the components, in particular the biological shield, can increase to levels where deleterious effects are introduced as a result of neutron irradiation. This work summarizes the current state of the art on irradiated concrete, including a review of the current literature and estimates the total neutron fluence expected in biological shields in typical LWR configurations. It was found a first-order mechanism for loss of mechanical properties of irradiated concrete is due to radiation-induced swelling of aggregates, which leads to volumetric expansion of the concrete. This phenomena is estimated to occur near the end of life of biological shield components in LWRs based on calculations of estimated peak neutron fluence in the shield after 80 years of operation.

[1]  Gary S. Was,et al.  Fundamentals of Radiation Materials Science: Metals and Alloys , 2007 .

[2]  Vesa Penttala,et al.  Effects of High Temperature on the Pore Structure and Strength of Plain and Polypropylene Fiber Reinforced Cement Pastes , 2003 .

[3]  Kunio Onizawa,et al.  Experimental Study of the Effect of Radiation Exposure to Concrete. , 2009 .

[4]  M. Wittels,et al.  RADIATION DAMAGE IN SiO$sub 2$ STRUCTURES , 1954 .

[5]  B. S. Hickman RADIATION EFFECTS IN BERYLLIUM AND BERYLLIUM OXIDE. , 1968 .

[6]  Steven J. Zinkle,et al.  Radiation effects in ceramics , 1994 .

[7]  A. D. Goër Phonon Scattering in Disordered Systems , 1986 .

[8]  Theodore Rockwell,et al.  Reactor Shielding Design Manual , 1956 .

[9]  Steven J. Zinkle,et al.  Radiation effects in crystalline ceramics for the immobilization of high-level nuclear waste and plutonium , 1998 .

[10]  S. Ibragimov,et al.  Radiation damage in ordinary concrete , 1967 .

[11]  E. Salje,et al.  Diffuse X-ray scattering in WO3 , 1998 .

[12]  William Primak,et al.  Fast-Neutron-Induced Changes in Quartz and Vitreous Silica , 1958 .

[13]  W. A. Rhoades,et al.  The TORT three-dimensional discrete ordinates neutron/photon transport code (TORT version 3) , 1997 .

[14]  Steven J. Zinkle,et al.  Defect production in ceramics , 1997 .

[15]  P. Piszora,et al.  Effect of Gamma Irradiation on Cement Composites Observed with XRD and SEM Methods in the Range of Radiation Dose 0-1409 MGy , 2008 .

[16]  M. Avrami Granulation, Phase Change, and Microstructure Kinetics of Phase Change. III , 1941 .

[17]  Y. Le Pape,et al.  Radiation effects in concrete for nuclear power plants, Part II: Perspective from micromechanical modeling , 2015 .

[18]  J. E. White Production and testing of the VITAMIN-B6 fine-group and the BUGLE-93 broad-group neutron/photon cross-section libraries derived from ENDF/B-VI nuclear data , 1995 .

[19]  R. Swamy,et al.  The Alkali-silica reaction in concrete , 1998 .

[20]  Jianzhuang Xiao,et al.  Study on concrete at high temperature in China--an overview , 2004 .

[21]  D. V. Phillips,et al.  Relationship between brittleness and moisture loss of concrete exposed to high temperatures , 2002 .

[22]  J. Kropp,et al.  The Effects of Nuclear Radiation on the Mechanical Properties of Concrete , 1978 .

[23]  G. Mayer,et al.  Effet des neutrons rapides sur le quartz cristallin et la silice vitreuse , 1960 .

[24]  Paulo J.M. Monteiro,et al.  The alkali–silica reaction: The effect of monovalent and bivalent cations on the surface charge of opal , 1999 .

[25]  B. Golding,et al.  Diffuse X-Ray Scattering and Phonon Echoes from Neutron-Irradiated Crystalline Quartz , 1981 .

[26]  D. L. Fillmore Literature Review of the Effects of Radiation and Temperature on the Aging of Concrete , 2004 .

[27]  Ulrich Schneider,et al.  Effect of temperature on steel and concrete for PCRV's , 1982 .

[28]  Ippei Maruyama,et al.  Strength and Young's modulus change in concrete due to long-term drying and heating up to 90 °C , 2014 .

[29]  O. Hauser,et al.  Veränderungen der Kristallstruktur einiger Oxyde, Karbonate und Titanate durch Neutronenbestrahlung , 1964 .

[30]  S. E. Pihlajavaara,et al.  A review of some of the main results of a research on the ageing phenomena of concrete: Effect of moisture conditions on strength, shrinkage and creep of mature concrete , 1974 .

[31]  Gary S. Was,et al.  Fundamentals of radiation materials science , 2007 .

[32]  K. Nakajima,et al.  Defect Structure and Density Decrease in Neutron‐Irradiated Quartz , 1963 .

[33]  George N. Freskakis Behavior of reinforced concrete at elevated temperatures , 1980 .

[34]  Dan J Naus,et al.  The Effect of Elevated Temperature on Concrete Materials and Structures - a Literature Review. , 2006 .

[35]  F.B.K. Kam,et al.  H.B. Robinson-2 pressure vessel benchmark , 1998 .

[36]  F De Larrard,et al.  The influence of aggregate on the compressive strength of normal and high-strength concrete , 1997 .

[37]  I. Janotka,et al.  Effect of temperature on structural quality of the cement paste and high-strength concrete with silica fume , 2005 .

[38]  Lumin Wang,et al.  Irradiation-induced amorphization: Effects of temperature, ion mass, cascade size, and dose rate , 2000 .

[39]  V. G. Zubov,et al.  EXPANSION OF QUARTZ CAUSED BY IRRADIATION WITH FAST NEUTRONS. , 1966 .

[40]  P. K. Mehta,et al.  Concrete: Microstructure, Properties, and Materials , 2005 .

[41]  J. Duraud,et al.  Amorphization of α-Quartz under Irradiation , 1996 .

[42]  L. Hobbs,et al.  CHAPTER 7 - Radiation Effects in Non-Metals* , 1986 .

[43]  R. C. Birtcher,et al.  Ion beam amorphization of muscovite mica , 1996 .

[44]  Kevin T. Clarno,et al.  Denovo: A New Three-Dimensional Parallel Discrete Ordinates Code in SCALE , 2010 .

[45]  A. Neville Properties of Concrete , 1968 .

[46]  Osamu Sato,et al.  Irradiation Effects on Concrete Structures , 2013 .

[47]  S. Sawada,et al.  EVALUATION OF IRRADIATION EFFECTS ON CONCRETE STRUCTURE -GAMMA-RAY IRRADIATION TESTS ON CEMENT PASTE- , 2013 .

[48]  R. Ewing,et al.  The amorphization of complex silicates by ion-beam irradiation , 1992 .

[49]  C. F. Wong Neutron radiation damege in some birefringent crystals , 1974 .

[50]  S. Sawada,et al.  Evaluation of irradiation effects on concrete structure-background and preparation of neutron irradiation test , 2013 .

[51]  W. Bolse Formation and development of disordered networks in Si-based ceramics under ion bombardment , 1998 .

[52]  J. Bonnet,et al.  The amorphization process of neutron-irradiated crystalline quartz studied by Brillouin scattering , 1994 .

[53]  L. M. Milian,et al.  The effect of gamma radiation on the strength of Portland cement mortars , 2001 .