Nonlinear Inferential Cascade Control of Exothermic Fixed-bed Reactors

A nonlinear inferential cascade control strategy for a tubular fixed-bed reactor with highly exothermic reaction is presented. Tight control of exit conversion and stabilization of hot-spot temperature was achieved over a wide range of operating conditions. A multiple cascade structure was developed by lumping the distributed-parameter system and partitioning it into three subsystems. Practical issues of implementing the control system are addressed, as well as physical insight and assumptions used for model reduction of each subsystem. The direct synthesis approach for nonlinear control systems is used to design the controllers of the important subsystems separately. A lag was added in the primary subsystem, and fast stabilization of the secondary subsystem was implemented. Unknown temperature states and inlet concentration were estimated by a nonlinear observer from only a few temperature measurements. The control problem of the moving hot-spot temperature was also addressed. Simulation on an industrial phthalic anhydride fixed-bed reactor showed that the observer can give excellent dynamic tracking of the reactor. The resulting cascade control system can achieve good set-point tracking and disturbance rejection performance, which is robust in the presence of measurement error and model mismatch, and superior to a single-loop control system.

[1]  David W. Clarke,et al.  Generalized predictive control - Part I. The basic algorithm , 1987, Autom..

[2]  Mondher Farza,et al.  Nonlinear observers for parameter estimation in bioprocesses , 1997 .

[3]  Hassan Hammouri,et al.  Nonlinear observers for chemical reactors , 1994 .

[4]  Chun-Yu Chen,et al.  Adaptive inferential control of packed-bed reactors , 1991 .

[5]  M. Soroush Nonlinear state-observer design with application to reactors , 1997 .

[6]  G. R. Sullivan,et al.  Generic model control (GMC) , 1988 .

[7]  Alessandro Brambilla,et al.  Nonlinear filter in cascade control schemes , 1992 .

[8]  M. Chidambaram,et al.  MODEL REFERENCE CASCADE CONTROL OF NONLINEAR SYSTEMS: APPLICATION TO AN UNSTABLE CSTR , 1992 .

[9]  Manfred Morari,et al.  Robust Inferential Control for a Packed-Bed Reactor , 1990, 1990 American Control Conference.

[10]  Achim Kienle,et al.  State profile estimation of an autothermal periodic fixed-bed reactor , 1998 .

[11]  Wolfgang Marquardt,et al.  DIVA—an open architecture for dynamic simulation , 1990 .

[12]  W. Harmon Ray,et al.  A control scheme for packed bed reactors having a changing catalyst activity profile. I: On-line parameter estimation and feedback control , 1992 .

[13]  J. Gauthier,et al.  High gain estimation for nonlinear systems , 1992 .

[14]  Gilbert F. Froment,et al.  FIXED BED CATALYTIC REACTORS—CURRENT DESIGN STATUS , 1967 .

[15]  B. Bequette Nonlinear control of chemical processes: a review , 1991 .

[16]  Arthur Jutan,et al.  Multivariable computer control of a butane hydrogenolysis reactor: Part I. State space reactor modeling , 1977 .

[17]  Manfred Morari,et al.  Linearizing controller design for a packed-bed reactor using a low-order wave propagation model , 1996 .

[18]  John F. MacGregor,et al.  Application of LQ and IMC controllers to a packed‐bed reactor , 1987 .

[19]  C. Kravaris,et al.  Geometric methods for nonlinear process control. 1. Background , 1990 .

[20]  Peter L. Lee,et al.  Process model-based engineering , 1989 .