Experimental study of surface-plasmon scattering by individual surface defects

A direct-write ablation technique has been implemented in a photon scanning tunneling microscope setup. This combination allows us to study surface-plasmon (SP) scattering by in situ created individual surface defects, while the sizes and shapes of the defects are varied continuously. It is found that within a certain range of its size, a ``hill'' on an otherwise flat surface can be the source of a very narrow plasmon beam. This effect is explained using the Huygens-Fresnel principle. Shadowing and refraction of the SP field by smaller defects has also been observed. In order to explain these results we introduce an effective SP refractive index for two classes of surface defects: shallow topographical defects and areas covered with absorbed molecular layers. This concept allows us to achieve a qualitative understanding of plasmon scattering in many practical cases. Some simple optical elements for the control of SP propagation are suggested and demonstrated. Our observations suggest numerous practical applications in multichannel chemical sensing, biosensing, and integrated optics.

[1]  R. W. Alexander,et al.  Multimedia dispersion relation for surface electromagnetic waves , 1975 .

[2]  Wolfgang Knoll,et al.  Surface–plasmon microscopy , 1988, Nature.

[3]  P. Leiderer,et al.  Near-field optical measurement of the surface plasmon field , 1993 .

[4]  Ferrell,et al.  New form of scanning optical microscopy. , 1989, Physical review. B, Condensed matter.

[5]  Mazzoni,et al.  Imaging of Surface Plasmon Scattering by Lithographically Created Individual Surface Defects. , 1996, Physical review letters.

[6]  Christopher C. Davis,et al.  Near‐field direct‐write ultraviolet lithography and shear force microscopic studies of the lithographic process , 1995 .

[7]  N. F. Hulst,et al.  Near field plasmon and force microscopy , 1995 .

[8]  J. Gordon,et al.  The effect of thin organic films on the surface plasma resonance on gold , 1977 .

[9]  Adam,et al.  Determination of the spatial extension of the surface-plasmon evanescent field of a silver film with a photon scanning tunneling microscope. , 1993, Physical review. B, Condensed matter.

[10]  Specht,et al.  Scanning plasmon near-field microscope. , 1992, Physical review letters.

[11]  H. Walther,et al.  Decay length of surface plasmons determined with a tunnelling microscope , 1991 .

[12]  Greffet,et al.  Scattering of a surface plasmon polariton by a surface defect. , 1994, Physical review. B, Condensed matter.

[13]  B. Liedberg,et al.  Surface plasmon resonance for gas detection and biosensing , 1983 .

[14]  E. Kretschmann,et al.  Notizen: Radiative Decay of Non Radiative Surface Plasmons Excited by Light , 1968 .

[15]  R. Rendell,et al.  Surface plasmons confined by microstructures on tunnel junctions , 1981 .

[16]  J. Ketterson,et al.  Scanning plasmon optical microscope operation in atomic force microscope mode. , 1996, Optics letters.

[17]  Bozhevolnyi,et al.  Near-field microscopy of surface-plasmon polaritons: Localization and internal interface imaging. , 1995, Physical review. B, Condensed matter.

[18]  Dawson,et al.  Imaging of surface plasmon propagation and edge interaction using a photon scanning tunneling microscope. , 1994, Physical review letters.

[19]  P. Leiderer,et al.  Detection of surface plasmons by scanning tunneling microscopy , 1991 .