Antiphase boundaries in bulk Ni-Mn-Ga Heusler alloy observed by magnetic force microscopy

The antiphase boundaries (APBs) in Ni-Mn-Ga Heusler alloys with L21 ordering have been so far possible to observe only in the foils using electron holography. Here, we present the possibility to observe the APBs in bulk materials by conventional magnetic force microscopy using particularly oriented and magnetized single crystal samples in the martensite state. The bipolar APB contrast occurs where in-plane magnetization is oriented perpendicularly to APBs. This is in agreement with a qualitative model of an APB as a planar non-magnetic layer in the ferromagnetic matrix.The antiphase boundaries (APBs) in Ni-Mn-Ga Heusler alloys with L21 ordering have been so far possible to observe only in the foils using electron holography. Here, we present the possibility to observe the APBs in bulk materials by conventional magnetic force microscopy using particularly oriented and magnetized single crystal samples in the martensite state. The bipolar APB contrast occurs where in-plane magnetization is oriented perpendicularly to APBs. This is in agreement with a qualitative model of an APB as a planar non-magnetic layer in the ferromagnetic matrix.

[1]  J. Drahokoupil,et al.  Structure and microstructure of Ni-Mn-Ga single crystal exhibiting magnetic shape memory effect analysed by high resolution X-ray diffraction , 2016 .

[2]  H. Seiner,et al.  Magnetic Domains and Twin Microstructure of Single Crystal Ni–Mn–Ga Exhibiting Magnetic Shape Memory Effect , 2015, IEEE Transactions on Magnetics.

[3]  Y. Murakami,et al.  Magnetization amplified by structural disorder within nanometre-scale interface region , 2014, Nature Communications.

[4]  J. Drahokoupil,et al.  The effect of antiphase boundaries on the elastic properties of Ni–Mn–Ga austenite and premartensite , 2013, Journal of physics. Condensed matter : an Institute of Physics journal.

[5]  Y. W. Lai,et al.  Magnetic Domains and Twin Boundary Movement of NiMnGa Magnetic Shape Memory Crystals , 2012 .

[6]  L. Schultz,et al.  Magnetic domain structure of epitaxial Ni-Mn-Ga films , 2012, 1203.3840.

[7]  Y. Murakami,et al.  Suppression of ferromagnetism within antiphase boundaries in Ni50Mn25Al12.5Ga12.5 alloy , 2011 .

[8]  M. Graef,et al.  In Situ Lorentz TEM Magnetization Study of a Ni-Mn-Ga Ferromagnetic Shape Memory Alloy , 2011 .

[9]  L. Schultz,et al.  Volume magnetic domain mirroring in magnetic shape memory crystals , 2010 .

[10]  E. Cesari,et al.  Ferromagnetic shape memory alloys: Alternatives to Ni–Mn–Ga , 2008 .

[11]  M. Graef,et al.  Magnetic domain memory in multiferroic Ni2MnGa , 2007 .

[12]  M. Graef,et al.  Anti-phase boundaries and magnetic domain structures in Ni2MnGa-type Heusler alloys , 2007 .

[13]  Y. Murakami,et al.  Recent Advances in Domain Analysis , 2005 .

[14]  K. Ullakko,et al.  Relation between structure, magnetization process and magnetic shape memory effect of various martensites occurring in Ni-Mn-Ga alloys , 2003 .

[15]  C. Ross,et al.  Structure and thermomagnetic properties of polycrystalline Ni–Mn–Ga thin films , 2003 .

[16]  R. Nieminen,et al.  Coexistence of ferromagnetic and antiferromagnetic order in Mn-doped Ni2MnGa , 2002, cond-mat/0212442.

[17]  M. Wuttig,et al.  Chemical ordering in Ni-Mn-Ga Heusler alloys , 1999 .

[18]  V. V. Kokorin,et al.  Magnetically controlled shape memory effect in Ni2MnGa intermetallics , 1997 .

[19]  W. Soffa,et al.  The structure and properties of L10 ordered ferromagnets: Co-Pt, FePt, FePd and MnAl , 1994 .

[20]  H. Hug,et al.  Models for the stray field from magnetic tips used in magnetic force microscopy , 1992 .

[21]  J. E. Stern,et al.  Magnetic force microscopy: General principles and application to longitudinal recording media , 1990 .

[22]  H. Hilzinger The influence of planar defects on the coercive field of hard magnetic materials , 1977 .

[23]  J. Jakubovics,et al.  Effect of antiphase boundaries on the magnetic properties of Cu-Mn-Al Heusler alloys , 1974 .

[24]  M. Acet,et al.  Magnetic-Field-Induced Effects in Martensitic Heusler-Based Magnetic Shape Memory Alloys , 2011 .

[25]  O. Heczko,et al.  Magnetic Shape Memory Phenomena , 2009 .

[26]  S. Takahashi,et al.  Cold-working effect on magnetic properties in the Heusler alloys , 1984 .