The major stratospheric final warming in 2016: dispersal of vortex air and termination of Arctic chemical ozone loss

Abstract. The 2015/16 Northern Hemisphere winter stratosphere appeared to have the greatest potential yet seen for record Arctic ozone loss. Temperatures in the Arctic lower stratosphere were at record lows from December 2015 through early February 2016, with an unprecedented period of temperatures below ice polar stratospheric cloud thresholds. Trace gas measurements from the Aura Microwave Limb Sounder (MLS) show that exceptional denitrification and dehydration, as well as extensive chlorine activation, occurred throughout the polar vortex. Ozone decreases in 2015/16 began earlier and proceeded more rapidly than those in 2010/11, a winter that saw unprecedented Arctic ozone loss. However, on 5–6 March 2016 a major final sudden stratospheric warming ("major final warming", MFW) began. By mid-March, the mid-stratospheric vortex split after being displaced far off the pole. The resulting offspring vortices decayed rapidly preceding the full breakdown of the vortex by early April. In the lower stratosphere, the period of temperatures low enough for chlorine activation ended nearly a month earlier than that in 2011 because of the MFW. Ozone loss rates were thus kept in check because there was less sunlight during the cold period. Although the winter mean volume of air in which chemical ozone loss could occur was as large as that in 2010/11, observed ozone values did not drop to the persistently low values reached in 2011. We use MLS trace gas measurements, as well as mixing and polar vortex diagnostics based on meteorological fields, to show how the timing and intensity of the MFW and its impact on transport and mixing halted chemical ozone loss. Our detailed characterization of the polar vortex breakdown includes investigations of individual offspring vortices and the origins and fate of air within them. Comparisons of mixing diagnostics with lower-stratospheric N2O and middle-stratospheric CO from MLS (long-lived tracers) show rapid vortex erosion and extensive mixing during and immediately after the split in mid-March; however, air in the resulting offspring vortices remained isolated until they disappeared. Although the offspring vortices in the lower stratosphere survived longer than those in the middle stratosphere, the rapid temperature increase and dispersal of chemically processed air caused active chlorine to quickly disappear. Furthermore, ozone-depleted air from the lower-stratospheric vortex core was rapidly mixed with ozone rich air from the vortex edge and midlatitudes during the split. The impact of the 2016 MFW on polar processing was the latest in a series of unexpected events that highlight the diversity of potential consequences of sudden warming events for Arctic ozone loss.

[1]  V. J. García-Garrido,et al.  A dynamical systems perspective for a real-time response to a marine oil spill. , 2016, Marine pollution bulletin.

[2]  N. Huret,et al.  Poleward transport variability in the Northern Hemisphere during final stratospheric warmings simulated by CESM(WACCM) , 2016 .

[3]  Ricardo Todling,et al.  Maintaining atmospheric mass and water balance in reanalyses , 2016, Quarterly journal of the Royal Meteorological Society. Royal Meteorological Society.

[4]  V. J. García-Garrido,et al.  Response to: "Limitations of the Method of Lagrangian Descriptors" [arXiv:1510.04838] , 2016, 1602.04243.

[5]  Michael J. Schwartz,et al.  A minor sudden stratospheric warming with a major impact: Transport and polar processing in the 2014/2015 Arctic winter , 2015 .

[6]  M. Santee,et al.  A Match-based approach to the estimation of polar stratospheric ozone loss using Aura Microwave Limb Sounder observations , 2015 .

[7]  Alfonso Ruiz-Herrera,et al.  Some examples related to the method of Lagrangian descriptors. , 2015, Chaos.

[8]  Amy H. Butler,et al.  Defining Sudden Stratospheric Warmings , 2015 .

[9]  Alyn Lambert,et al.  Comparisons of polar processing diagnostics from 34 years of the ERA-Interim and MERRA reanalyses , 2014 .

[10]  Jinggao Hu,et al.  Occurrence of Winter Stratospheric Sudden Warming Events and the Seasonal Timing of Spring Stratospheric Final Warming , 2014 .

[11]  M. Smith,et al.  A quantitative measure of polar vortex strength using the function M , 2014 .

[12]  K. Ide,et al.  Isentropic Transport within the Antarctic Polar-Night Vortex: Rossby Wave Breaking Evidence and Lagrangian Structures , 2013 .

[13]  N. Huret,et al.  A climatology of frozen‐in anticyclones in the spring arctic stratosphere over the period 1960–2011 , 2013 .

[14]  E. Castelli,et al.  Extreme ozone depletion in the 2010–2011 Arctic winter stratosphere as observed by MIPAS/ENVISAT using a 2-D tomographic approach , 2012 .

[15]  P. Bernath,et al.  Uncertainties in modelling heterogeneous chemistry and Arctic ozone depletion in the winter 2009/2010 , 2012 .

[16]  Wendy P Robinson,et al.  Response to , 2012, Epigenetics.

[17]  L. Coy,et al.  Tracer transport during the Arctic stratospheric final warming based on a 33‐year (1979‐2011) tracer equivalent latitude simulation , 2012 .

[18]  I. Horenko,et al.  Supervised Learning Approaches to Classify Sudden Stratospheric Warming Events , 2012 .

[19]  K. Ide,et al.  Routes of Transport across the Antarctic Polar Vortex in the Southern Spring , 2012 .

[20]  T. Clarmann,et al.  Arctic winter 2010/2011 at the brink of an ozone hole , 2011 .

[21]  M. Pitts,et al.  The 2009–2010 Arctic stratospheric winter – general evolution, mountain waves and predictability of an operational weather forecast model , 2011 .

[22]  Mark R. Schoeberl,et al.  Unprecedented Arctic ozone loss in 2011 , 2011, Nature.

[23]  Stephen Wiggins,et al.  Lagrangian descriptors: A method for revealing phase space structures of general time dependent dynamical systems , 2011, Commun. Nonlinear Sci. Numer. Simul..

[24]  L. Gray,et al.  Characterizing the Variability and Extremes of the Stratospheric Polar Vortices Using 2D Moment Analysis , 2011 .

[25]  L. Polvani,et al.  Stratospheric Ozone Depletion: The Main Driver of Twentieth-Century Atmospheric Circulation Changes in the Southern Hemisphere , 2011 .

[26]  Carolina Mendoza,et al.  Hidden geometry of ocean flows. , 2010, Physical review letters.

[27]  T. Shepherd,et al.  Impact of climate change on stratospheric sudden warmings as simulated by the Canadian Middle Atmosphere Model. , 2009 .

[28]  Andrew Charlton-Perez,et al.  A New Look at Stratospheric Sudden Warmings. Part III: Polar Vortex Evolution and Vertical Structure , 2009 .

[29]  L. Polvani,et al.  The frequency and dynamics of stratospheric sudden warmings in the 21st century , 2008 .

[30]  Martyn P. Chipperfield,et al.  A study of stratospheric chlorine partitioning based on new satellite measurements and modeling , 2008 .

[31]  A M Mancho,et al.  Distinguished trajectories in time dependent vector fields. , 2008, Chaos.

[32]  P. Bernath,et al.  Solar occultation satellite data and derived meteorological products: Sampling issues and comparisons with Aura Microwave Limb Sounder , 2007 .

[33]  H. Akiyoshi,et al.  Midlatitude and high-latitude N2O distributions in the Northern Hemisphere in early and late Arctic polar vortex breakup years , 2007 .

[34]  R. X. Black,et al.  The Dynamics of Northern Hemisphere Stratospheric Final Warming Events , 2007 .

[35]  M. Chipperfield,et al.  Quantifying Arctic ozone loss during the 2004-2005 winter using satellite observations and a chemical transport model , 2007 .

[36]  L. Polvani,et al.  A New Look at Stratospheric Sudden Warmings. Part I: Climatology and Modeling Benchmarks , 2007 .

[37]  S. Tilmes,et al.  Chemical ozone loss in the Arctic and Antarctic stratosphere between 1992 and 2005 , 2006 .

[38]  Peter H. Siegel,et al.  The Earth observing system microwave limb sounder (EOS MLS) on the aura Satellite , 2006, IEEE Transactions on Geoscience and Remote Sensing.

[39]  M. Santee,et al.  EOS Microwave Limb Sounder observations of “frozen‐in” anticyclonic air in Arctic summer , 2006 .

[40]  L. Froidevaux,et al.  EOS MLS observations of ozone loss in the 2004–2005 Arctic winter , 2006 .

[41]  William G. Read,et al.  EOS Microwave Limb Sounder observations of the Antarctic polar vortex breakup in 2004 , 2005 .

[42]  C. Randall,et al.  On the distribution of ozone in stratospheric anticyclones , 2004 .

[43]  B. Lawrence,et al.  Dilution of the Antarctic ozone hole into southern midlatitudes, 1998–2000 , 2004 .

[44]  P. Stott,et al.  Causes of exceptional atmospheric circulation changes in the Southern Hemisphere , 2004 .

[45]  Martyn P. Chipperfield,et al.  Arctic ozone loss and climate change , 2004 .

[46]  M. Chipperfield,et al.  Model simulations of the northern extravortex ozone column: Influence of past changes in chemical composition , 2004 .

[47]  D. McKenna,et al.  Dynamics and chemistry of vortex remnants in late Arctic spring 1997 and 2000: Simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS) , 2003 .

[48]  K. Matthes,et al.  The early major warming in December 2001 – exceptional? , 2002 .

[49]  R. Bradley Pierce,et al.  A climatology of stratospheric polar vortices and anticyclones , 2002 .

[50]  D. Waugh,et al.  Interannual Variability in the Decay of Lower Stratospheric Arctic Vortices. , 2002 .

[51]  K. Labitzke The Solar Signal of the 11-Year Sunspot Cycle in the Stratosphere : Differences between the Northern and Southern Summers , 2002 .

[52]  D. Keuer,et al.  Variability of the mesospheric wind field at middle and Arctic latitudes in winter and its relation to stratospheric circulation disturbances , 2002 .

[53]  D. Allen,et al.  Tracer Equivalent Latitude: A Diagnostic Tool for Isentropic Transport Studies , 2002 .

[54]  D. Allen,et al.  Dynamical reconstruction of the record low column ozone over Europe on 30 November 1999 , 2002 .

[55]  M. Chipperfield,et al.  Modeling the effect of denitrification on Arctic ozone depletion during winter 1999/2000 , 2002 .

[56]  D. Allen,et al.  A seasonal climatology of effective diffusivity in the stratosphere , 2001 .

[57]  E. Shuckburgh,et al.  Effective diffusivity as a diagnostic of atmospheric transport: 1. Stratosphere , 2000 .

[58]  M. Santee,et al.  Polar vortex dynamics during spring and fall diagnosed using trace gas observations from the Atmospheric Trace Molecule Spectroscopy instrument , 1999 .

[59]  W. Randel,et al.  Climatology of Arctic and Antarctic Polar Vortices Using Elliptical Diagnostics , 1999 .

[60]  P. Crutzen,et al.  Arctic ozone loss due to denitrification , 1999, Science.

[61]  L. Froidevaux,et al.  UARS Microwave Limb Sounder HNO3 observations: Implications for Antarctic polar stratospheric clouds , 1998 .

[62]  G. Dutton,et al.  Dehydration and denitrification in the Arctic Polar Vortex during the 1995–1996 winter , 1998 .

[63]  J. Pyle,et al.  Effects of fluid-dynamical stirring and mixing on the deactivation of stratospheric chlorine , 1998 .

[64]  M. Chipperfield,et al.  Chlorine deactivation in the lower stratospheric polar regions during late winter: Results from UARS , 1996 .

[65]  N. Nakamura Two-Dimensional Mixing, Edge Formation, and Permeability Diagnosed in an Area Coordinate , 1996 .

[66]  Lawrence L. Takacs,et al.  Data Assimilation Using Incremental Analysis Updates , 1996 .

[67]  R. Stolarski,et al.  Interhemispheric differences in springtime production of HCl and ClONO2 in the polar vortices , 1995 .

[68]  L. Froidevaux,et al.  Formation of low‐ozone pockets in the middle stratospheric anticyclone during winter , 1995 .

[69]  A. O'Neill,et al.  On the motion of air through the stratospheric polar vortex , 1994 .

[70]  A. O'Neill,et al.  High-Resolution Stratospheric Tracer Fields Estimated from Satellite Observations Using Lagrangian Trajectory Calculations , 1994 .

[71]  A. O'Neill,et al.  Quasi‐horizontal transport and mixing in the Antarctic stratosphere , 1994 .

[72]  D. Rind,et al.  Global impact of the Antarctic ozone hole: Dynamical dilution with a three-dimensional chemical transport model , 1990 .

[73]  S. Wofsy,et al.  Condensation of HNO3 on falling ice particles: Mechanism for denitrification of the polar stratosphere , 1990 .

[74]  D. Andrews Some comparisons between the middle atmosphere dynamics of the Southern and Northern Hemispheres , 1989 .

[75]  Ellis E. Remsberg,et al.  The Area of the Stratospheric Polar Vortex as a Diagnostic for Tracer Transport on an Isentropic Surface , 1986 .

[76]  T. Dunkerton,et al.  Evolution of potential vorticity in the winter stratosphere of January‐February 1979 , 1986 .

[77]  John C. Gille,et al.  Transport of ozone in the middle stratosphere: evidence for planetary wave breaking , 1985 .

[78]  Tim Palmer,et al.  The «surf zone» in the stratosphere , 1984 .

[79]  J. Gregory Middle atmosphere dynamics , 1981, Nature.

[80]  R. Heikes,et al.  Modeling Rossby Wave Breaking in the Southern Spring Stratosphere , 2016 .

[81]  P. Bernath,et al.  Uncertainties in modelling heterogeneous chemistry and Arctic ozone depletion in the winter 2009 / 2010 , 2012 .

[82]  C. Frantzidis,et al.  Response to Reviewers Reviewer #1 , 2010 .

[83]  M. Botur,et al.  Lagrangian coherent structures , 2009 .

[84]  Douglas Lowe,et al.  Polar stratospheric cloud microphysics and chemistry , 2008 .

[85]  K. Labitzke On the Interannual Variability of the Middle Stratosphere during the Northern Winters , 1982 .