Investigation of Yb2Pt6Al15 single crystals: heavy fermion system with a large local moment degeneracy

We grew single crystals of Yb2Pt6Al15 and investigated the magnetic properties of this compound by means of susceptibility χ(T), specific heat C(T), resistivity ρ (T) and thermoelectric power S(T) measurements. While all properties follow in general the behavior typical for Kondo-lattice systems, χ(T) and C(T)/T present broad maxima in the T range 17–35 K, which matches nicely the prediction of the Coqblin–Schrieffer model for J= 7/2. A large degeneracy of the local moment is also supported by a reduced Kadowaki–Woods ratio. Thus, the analysis of all investigated properties evidences Yb2Pt6Al15 to be a paramagnetic Kondo-lattice system with the whole J= 7/2 multiplet involved in the formation of the Kondo state, a Kondo temperature of the order of 60 K, and a heavy Fermi-liquid ground state with a Sommerfeld coefficient γ 0 = 0.33 J (mol-Yb)−1 K−2 corresponding to a mass enhancement of the order of 30.

[1]  P. Canfield,et al.  Myriad of correlated electron effects found in the RT2Zn20 family , 2008 .

[2]  Philipp Gegenwart,et al.  Quantum criticality in heavy-fermion metals , 2007, 0712.2045.

[3]  R. Black,et al.  Six closely related YbT2Zn20 (T = Fe, Co, Ru, Rh, Os, Ir) heavy fermion compounds with large local moment degeneracy , 2006, Proceedings of the National Academy of Sciences.

[4]  H. Kontani,et al.  Universality in heavy fermion systems with general degeneracy. , 2005, Physical review letters.

[5]  W. Jeitschko,et al.  Ternary Aluminides with the Ideal Composition A2Pt6Al15 (A = Y, Gd—Tm, Zr) , 2004 .

[6]  H. Kontani Generalized Kadowaki–Woods Relation in Heavy Fermion Systems with Orbital Degeneracy , 2003, cond-mat/0308484.

[7]  C. Geibel,et al.  Observation of Two Distinct Superconducting Phases in CeCu2Si2 , 2003, Science.

[8]  G. Stewart Non-Fermi-liquid behavior in d - and f -electron metals , 2001 .

[9]  G. Lonzarich,et al.  Magnetically mediated superconductivity in quasi-two and three dimensions , 2001 .

[10]  Z. Fisk,et al.  Unconventional superconductivity in CeIrIn5 and CeCoIn5: specific heat and thermal conductivity studies. , 2000, Physical review letters.

[11]  K. Kadowaki,et al.  Universal relationship of the resistivity and specific heat in heavy-Fermion compounds , 1986 .

[12]  A. Hewson,et al.  Bethe ansatz and 1/N expansion results for N-fold degenerate magnetic impurity models , 1984 .

[13]  V. T. Rajan Magnetic Susceptibility and Specific Heat of the Coqblin-Schrieffer Model , 1983 .