Two-dimensional mixture of dipolar fermions: Equation of state and magnetic phases

We study a two-component mixture of fermionic dipoles in two dimensions at zero temperature, interacting via a purely repulsive $1/r^3$ potential. This model can be realized with ultracold atoms or molecules, when their dipole moments are aligned in the confinement direction orthogonal to the plane. We characterize the unpolarized mixture by means of the Diffusion Monte Carlo technique. Computing the equation of state, we identify the regime of validity for a mean-field theory based on a low-density expansion and compare our results with the hard-disk model of repulsive fermions. At high density, we address the possibility of itinerant ferromagnetism, namely whether the ground state can be fully polarized in the fluid phase. Within the fixed-node approximation, we show that the accuracy of Jastrow-Slater trial wave functions, even with the typical two-body backflow correction, is not sufficient to resolve the relevant energy differences. By making use of the iterative-backflow improved trial wave functions, we observe no signature of a fully-polarized ground state up to the freezing density.

[1]  W. Hager,et al.  and s , 2019, Shallow Water Hydraulics.

[2]  J. Tempere,et al.  Exchange interactions and itinerant ferromagnetism in ultracold Fermi gases , 2018, Physical Review A.

[3]  W. Ketterle,et al.  Time-Resolved Observation of Competing Attractive and Repulsive Short-Range Correlations in Strongly Interacting Fermi Gases. , 2018, Physical review letters.

[4]  Innsbruck,et al.  Dipolar Quantum Mixtures of Erbium and Dysprosium Atoms. , 2018, Physical review letters.

[5]  J. Becher,et al.  Realization of a Strongly Interacting Fermi Gas of Dipolar Atoms. , 2018, Physical review letters.

[6]  Markus Holzmann,et al.  Nonlinear Network Description for Many-Body Quantum Systems in Continuous Space. , 2017, Physical review letters.

[7]  J. Tempere,et al.  Exchange interactions in the Hubbard-Stratonovich transformation for the stability analysis of itinerant ferromagnetism , 2015, 1511.04502.

[8]  J. Boronat,et al.  Dipolar Bose Supersolid Stripes. , 2017, Physical review letters.

[9]  Jun Ye,et al.  Cold molecules: Progress in quantum engineering of chemistry and quantum matter , 2017, Science.

[10]  A. Recati,et al.  Exploring the ferromagnetic behaviour of a repulsive Fermi gas through spin dynamics , 2016, Nature Physics.

[11]  Tilman Pfau,et al.  Self-bound droplets of a dilute magnetic quantum liquid , 2016, Nature.

[12]  L. Santos,et al.  Quantum-Fluctuation-driven crossover from a dilute bose-einstein condensate to a macrodroplet in a dipolar quantum fluid , 2016, 1607.06613.

[13]  Tilman Pfau,et al.  Observation of Quantum Droplets in a Strongly Dipolar Bose Gas. , 2016, Physical review letters.

[14]  J. Krieg,et al.  Physical dipoles and second-order perturbation theory for dipolar fermions in two dimensions , 2015, 1512.06029.

[15]  P. Zoller,et al.  Extended Bose-Hubbard models with ultracold magnetic atoms , 2015, Science.

[16]  Sandro Stringari,et al.  Bose-Einstein condensation and superfluidity , 2016 .

[17]  S. Will,et al.  Ultracold Dipolar Gas of Fermionic 23Na40 K Molecules in Their Absolute Ground State. , 2015, Physical review letters.

[18]  Man-Ching Wong,et al.  57 , 2015, Tao te Ching.

[19]  Markus Holzmann,et al.  Iterative backflow renormalization procedure for many-body ground-state wave functions of strongly interacting normal Fermi liquids , 2015, 1501.02199.

[20]  Xu-Guang Huang,et al.  Stoner ferromagnetism of a strongly interacting Fermi gas in the quasirepulsive regime , 2014, 1412.2412.

[21]  S. Giorgini,et al.  Single-particle versus pair superfluidity in a bilayer system of dipolar bosons , 2014, 1407.6805.

[22]  A. Frisch,et al.  Observation of Fermi surface deformation in a dipolar quantum gas , 2014, Science.

[23]  M. Troyer,et al.  Ferromagnetism of a repulsive atomic Fermi gas in an optical lattice: a quantum Monte Carlo study. , 2013, Physical review letters.

[24]  Lei Wang,et al.  Ferromagnetism of the repulsive atomic Fermi gas: three-body recombination and domain formation , 2013, 1308.1961.

[25]  Masahito Ueda,et al.  Spinor Bose gases: Symmetries, magnetism, and quantum dynamics , 2013 .

[26]  G. Bertaina Two-dimensional short-range interacting attractive and repulsive Fermi gases at zero temperature , 2013, 1303.3840.

[27]  S. Giorgini,et al.  Liquid and crystal phases of dipolar fermions in two dimensions. , 2012, Physical review letters.

[28]  Y. Castin,et al.  General relations for quantum gases in two and three dimensions: Two-component fermions , 2012, 1204.3204.

[29]  A. Polls,et al.  Ferromagnetic transition of a two-component Fermi gas of hard spheres , 2012, 1203.2521.

[30]  G. Shlyapnikov,et al.  Fermi liquid of two-dimensional polar molecules , 2012 .

[31]  W. Ketterle,et al.  Correlations and pair formation in a repulsively interacting Fermi gas. , 2011, Physical review letters.

[32]  M. Nava,et al.  Equation of state of two-dimensional 3 He at zero temperature , 2011, 1103.0915.

[33]  R. Zillich,et al.  Microscopic description of anisotropic low-density dipolar Bose gases in two dimensions , 2011, 1105.5914.

[34]  R. Needs,et al.  Quantum Monte Carlo calculation of the zero-temperature phase diagram of the two-component fermionic hard-core gas in two dimensions , 2011, 1102.1318.

[35]  L. Mitas,et al.  Applications of quantum Monte Carlo methods in condensed systems , 2010, 1010.4992.

[36]  D. S. Jin,et al.  Controlling the quantum stereodynamics of ultracold bimolecular reactions , 2010, 1010.3731.

[37]  E. Demler,et al.  Competition between pairing and ferromagnetic instabilities in ultracold Fermi gases near Feshbach resonances. , 2010, Physical review letters.

[38]  M. Randeria,et al.  Ferromagnetism in the upper branch of the Feshbach resonance and the hard-sphere Fermi gas , 2010, Proceedings of the National Academy of Sciences.

[39]  M. Troyer,et al.  Itinerant ferromagnetism of a repulsive atomic Fermi gas: a quantum monte carlo study. , 2010, Physical review letters.

[40]  J. Ye,et al.  Dipolar collisions of polar molecules in the quantum regime , 2010, Nature.

[41]  C. Ticknor Two-dimensional dipolar scattering , 2009, 0908.0155.

[42]  N. Cooper,et al.  Stable topological superfluid phase of ultracold polar fermionic molecules. , 2009, Physical review letters.

[43]  David E. Pritchard,et al.  Itinerant Ferromagnetism in a Fermi Gas of Ultracold Atoms , 2009, Science.

[44]  B. Alder,et al.  Computer simulation of phase transitions in classical and quantum systems , 2009 .

[45]  I. L. Kurbakov,et al.  Equation of state of a weakly interacting two-dimensional Bose gas studied at zero temperature by means of quantum Monte Carlo methods , 2009 .

[46]  M. Lewenstein,et al.  The physics of dipolar bosonic quantum gases , 2009, 0905.0386.

[47]  R. Needs,et al.  Phase diagram of the low-density two-dimensional homogeneous electron gas. , 2009, Physical review letters.

[48]  G. Bruun,et al.  Quantum phases of a two-dimensional dipolar fermi gas. , 2008, Physical review letters.

[49]  M. Baranov,et al.  Theoretical progress in many-body physics with ultracold dipolar gases , 2008 .

[50]  Sandro Stringari,et al.  Theory of ultracold atomic Fermi gases , 2007, 0706.3360.

[51]  X. Waintal,et al.  Variational wave functions and their overlap with the ground state. , 2007, Physical review letters.

[52]  I. L. Kurbakov,et al.  Weakly interacting two-dimensional system of dipoles : Limitations of the mean-field theory , 2006, cond-mat/0612691.

[53]  I. L. Kurbakov,et al.  Quantum phase transition in a two-dimensional system of dipoles. , 2006, Physical review letters.

[54]  P. Zoller,et al.  Strongly correlated 2D quantum phases with cold polar molecules: controlling the shape of the interaction potential. , 2006, Physical review letters.

[55]  D. Ceperley,et al.  Many-body wavefunctions for normal liquid He3 , 2006, cond-mat/0605513.

[56]  R. Hulet,et al.  Pairing and Phase Separation in a Polarized Fermi Gas , 2005, Science.

[57]  Giovanni Vignale,et al.  Quantum Theory of the Electron Liquid , 2005 .

[58]  S. Giorgini,et al.  Quantum Monte Carlo simulation of a two-dimensional Bose gas , 2004, cond-mat/0411049.

[59]  B. Bernu,et al.  Optimized periodic 1/r Coulomb potential in two dimensions , 2004, cond-mat/0407244.

[60]  D. Ceperley,et al.  The polarization energy of normal liquid 3He , 2003 .

[61]  J. Boronat,et al.  Zero-temperature equation of state of two-dimensional 3He. , 2002, Physical review letters.

[62]  D. Ceperley,et al.  Spin polarization of the low-density three-dimensional electron gas. , 2002, Physical review. E, Statistical, nonlinear, and soft matter physics.

[63]  D. Ceperley,et al.  Twist-averaged boundary conditions in continuum quantum Monte Carlo algorithms. , 2001, Physical review. E, Statistical, nonlinear, and soft matter physics.

[64]  R. Needs,et al.  Quantum Monte Carlo simulations of solids , 2001 .

[65]  Santos,et al.  Bose-einstein condensation in trapped dipolar gases , 2000, Physical review letters.

[66]  Boronat,et al.  Progress in monte carlo calculations of fermi systems: normal liquid 3He , 1999, Physical review letters.

[67]  Los Alamos National Laboratory,et al.  Zero Temperature Phases of the Electron Gas , 1998, cond-mat/9810126.

[68]  J. Boronat,et al.  QUANTUM MONTE CARLO STUDY OF STATIC PROPERTIES OF ONE 3HE ATOM IN SUPERFLUID 4HE , 1998, cond-mat/9807273.

[69]  F. Dalfovo,et al.  Theory of Bose-Einstein condensation in trapped gases , 1998, cond-mat/9806038.

[70]  James B. Anderson,et al.  Fixed-node quantum Monte Carlo , 1995 .

[71]  David M. Ceperley,et al.  An optimized method for treating long-range potentials , 1995 .

[72]  Boronat,et al.  Unbiased estimators in quantum Monte Carlo methods: Application to liquid 4He. , 1995, Physical review. B, Condensed matter.

[73]  Peter Reynolds,et al.  Monte Carlo Methods In Ab Initio Quantum Chemistry , 1994 .

[74]  Goedecker,et al.  Comment on "Criterion for a good variational wave function" , 1991, Physical review. B, Condensed matter.

[75]  D. Ceperley,et al.  Ground state of the two-dimensional electron gas. , 1989, Physical review. B, Condensed matter.

[76]  E. Manousakis,et al.  Microscopic calculations for normal and polarized liquidHe3 , 1983 .

[77]  B. Alder,et al.  THE GROUND STATE OF THE ELECTRON GAS BY A STOCHASTIC METHOD , 2010 .

[78]  D. Ceperley Ground state of the fermion one-component plasma: A Monte Carlo study in two and three dimensions , 1978 .

[79]  V. Pandharipande Variational Method for Dense Systems , 1973 .

[80]  M. Schick Two-Dimensional System of Hard-Core Bosons , 1971 .

[81]  E. C. Stoner,et al.  Collective Electron Ferromagnetism , 1938 .

[82]  D H Weinstein,et al.  Modified Ritz Method. , 1934, Proceedings of the National Academy of Sciences of the United States of America.

[83]  F. Bloch,et al.  Bemerkung zur Elektronentheorie des Ferromagnetismus und der elektrischen Leitfähigkeit , 1929 .

[84]  G. Temple The Theory of Rayleigh's Principle as Applied to Continuous Systems , 1928 .