The SPIDER fission fragment spectrometer for fission product yield measurements

Abstract The SPectrometer for Ion DEtermination in fission Research (SPIDER) has been developed for measuring mass yield distributions of fission products from spontaneous and neutron-induced fission. The 2 E –2 v method of measuring the kinetic energy ( E ) and velocity ( v ) of both outgoing fission products has been utilized, with the goal of measuring the mass of the fission products with an average resolution of 1 atomic mass unit (amu). The SPIDER instrument, consisting of detector components for time-of-flight, trajectory, and energy measurements, has been assembled and tested using 229 Th and 252 Cf radioactive decay sources. For commissioning, the fully assembled system measured fission products from spontaneous fission of 252 Cf. Individual measurement resolutions were met for time-of-flight (250 ps FWHM), spacial resolution (2 mm FHWM), and energy (92 keV FWHM for 8.376 MeV). Mass yield results measured from 252 Cf spontaneous fission products are reported from an E – v measurement.

[1]  A. Oed,et al.  Precision measurements of mean kinetic energy release in thermal-neutron-induced fission of 233U, 235U and 239Pu , 1986 .

[2]  J. R. Dunning,et al.  The Fission of Uranium , 1939 .

[3]  R. Brissot,et al.  A mass spectrometer for fission fragments based on time-of-flight and energy measurements , 1984 .

[4]  A. Kohnle,et al.  Absolute measurement of velocities, masses and energies of fission fragments from californium-252 (SF) , 1981 .

[5]  M. Chadwick Future Challenges for Nuclear Data Research in Fission , 2011 .

[6]  G. Barreau,et al.  High resolution study of u235(nth, f) and Th229(nth, f) with cosi fan tutte mass spectrometer , 1986 .

[7]  G. Knoll Radiation detection and measurement , 1979 .

[8]  O. Hahn,et al.  Nachweis der Entstehung aktiver Bariumisotope aus Uran und Thorium durch Neutronenbestrahlung; Nachweis weiterer aktiver Bruchstücke bei der Uranspaltung , 1939, Naturwissenschaften.

[9]  F. Hambsch,et al.  A twin ionization chamber for fission fragment detection , 1987 .

[10]  P. Perrin,et al.  Mass spectrometry of fission fragments by simultaneous energy and time-of-flight measurements , 1986 .

[11]  T. R. England,et al.  Evaluation and compilation of fission product yields 1993 , 1995 .

[12]  D. Mcnabb,et al.  Review of the Status of Cumulative Fission Yields from 239Pu(n,f) of Interest to Nuclear Forensics , 2010 .

[13]  J. Lestone Energy Dependence of Plutonium Fission-Product Yields , 2011 .

[14]  Valentin T. Jordanov,et al.  Digital synthesis of pulse shapes in real time for high resolution radiation spectroscopy , 1994 .

[15]  W. E. Kiker,et al.  PRECISION MEASUREMENTS OF CORRELATED ENERGIES AND VELOCITIES OF $sup 252$Cf FISSION FRAGMENTS , 1965 .

[16]  F. Strassmann,et al.  Über den Nachweis und das Verhalten der bei der Bestrahlung des Urans mittels Neutronen entstehenden Erdalkalimetalle , 2005, Naturwissenschaften.

[17]  G. Barreau,et al.  A high-resolution multi-parametric study of 239Pu(nth, f) with the Cosi-Fan-Tutte spectrometer , 1991 .

[18]  LISE MEITNER,et al.  Disintegration of Uranium by Neutrons: a New Type of Nuclear Reaction , 1939, Nature.

[19]  S. Whetstone COINCIDENT TIME-OF-FLIGHT MEASUREMENTS OF THE VELOCITIES OF Cf$sup 252$ FISSION FRAGMENTS , 1963 .

[20]  A. Oed,et al.  A new method to identify nuclear charges of fission fragments , 1983 .

[21]  Kurt F. Schoenberg,et al.  The Los Alamos Neutron Science Center , 2006 .

[22]  P. Schillebeeckx,et al.  Investigation of mass, charge and energy of 241Pu(nth, f) fragments with the Cosi-Fan-Tutte spectrometer , 1994 .

[23]  G. Barreau,et al.  High resolution measurements of mass, energy and nuclear charge correlations for 229Th(nth, f) with the cosi fan tutte spectrometer , 1989 .

[24]  R. E. Blakeley,et al.  Development of position-sensitive time-of-flight spectrometer for fission fragment research , 2014, 1403.1573.

[25]  J. Ziegler,et al.  SRIM – The stopping and range of ions in matter (2010) , 2010 .