Peel-and-Stick: Mechanism Study for Efficient Fabrication of Flexible/Transparent Thin-film Electronics

Peel-and-stick process, or water-assisted transfer printing (WTP), represents an emerging process for transferring fully fabricated thin-film electronic devices with high yield and fidelity from a SiO2/Si wafer to various non-Si based substrates, including papers, plastics and polymers. This study illustrates that the fundamental working principle of the peel-and-stick process is based on the water-assisted subcritical debonding, for which water reduces the critical adhesion energy of metal-SiO2 interface by 70 ~ 80%, leading to clean and high quality transfer of thin-film electronic devices. Water-assisted subcritical debonding is applicable for a range of metal-SiO2 interfaces, enabling the peel-and-stick process as a general and tunable method for fabricating flexible/transparent thin-film electronic devices.

[1]  Joseph C. Fogarty,et al.  A reactive molecular dynamics simulation of the silica-water interface. , 2010, The Journal of chemical physics.

[2]  Justin A. Blanco,et al.  Dissolvable films of silk fibroin for ultrathin conformal bio-integrated electronics. , 2010, Nature materials.

[3]  Myeong-Lok Seol,et al.  Transfer of functional memory devices to any substrate , 2013 .

[4]  Metin Sitti,et al.  Microstructured elastomeric surfaces with reversible adhesion and examples of their use in deterministic assembly by transfer printing , 2010, Proceedings of the National Academy of Sciences.

[5]  John A Rogers,et al.  Optimized structural designs for stretchable silicon integrated circuits. , 2009, Small.

[6]  A. V. Duin,et al.  Development and Validation of ReaxFF Reactive Force Field for Hydrocarbon Chemistry Catalyzed by Nickel , 2010 .

[7]  Xiaolin Zheng,et al.  Peel-and-Stick: Fabricating Thin Film Solar Cell on Universal Substrates , 2012, Scientific Reports.

[8]  Xun Cai,et al.  Effects of residual stresses on interfacial adhesion measurement , 2009 .

[9]  Reinhold H. Dauskardt,et al.  Moisture-assisted subcritical debonding of a polymer/metal interface , 2002 .

[10]  A. V. Duin,et al.  ReaxFF: A Reactive Force Field for Hydrocarbons , 2001 .

[11]  Paolo Vavassori,et al.  Flexible and stretchable polymers with embedded magnetic nanostructures. , 2013, Advanced materials.

[12]  Xiaolin Zheng,et al.  Fabrication of nanowire electronics on nonconventional substrates by water-assisted transfer printing method. , 2011, Nano letters.

[13]  Heung Cho Ko,et al.  Arrays of silicon micro/nanostructures formed in suspended configurations for deterministic assembly using flat and roller-type stamps. , 2011, Small.

[14]  J. Kollár,et al.  The surface energy of metals , 1998 .

[15]  R. Dauskardt,et al.  Fracture of nanoporous thin-film glasses , 2004, Nature materials.

[16]  B. Cho,et al.  Direct measurement of adhesion energy of monolayer graphene as-grown on copper and its application to renewable transfer process. , 2012, Nano letters.

[17]  R. Dauskardt,et al.  Environmentally assisted debonding of copper/barrier interfaces , 2012 .

[18]  Brian Litt,et al.  Flexible, Foldable, Actively Multiplexed, High-Density Electrode Array for Mapping Brain Activity in vivo , 2011, Nature Neuroscience.

[19]  Yonggang Huang,et al.  Transfer printing by kinetic control of adhesion to an elastomeric stamp , 2006 .

[20]  Stephen W. Freiman,et al.  A molecular interpretation of stress corrosion in silica , 1982, Nature.

[21]  S. Wiederhorn Moisture assisted crack growth in ceramics , 1968 .

[22]  John A Rogers,et al.  Imbricate scales as a design construct for microsystem technologies. , 2012, Small.

[23]  Xiaolin Zheng,et al.  Fabricating nanowire devices on diverse substrates by simple transfer-printing methods , 2010, Proceedings of the National Academy of Sciences.

[24]  Huanyu Cheng,et al.  A Physically Transient Form of Silicon Electronics , 2012, Science.

[25]  Audrey M. Bowen,et al.  Transfer Printing Techniques for Materials Assembly and Micro/Nanodevice Fabrication , 2012, Advanced materials.

[26]  R. M. Cannon,et al.  On the physics of moisture-induced cracking in metal-glass (copper-silica) interfaces , 2007 .

[27]  Dirk C. Keene Acknowledgements , 1975 .

[28]  Sheldon M. Wiederhorn,et al.  Influence of Water Vapor on Crack Propagation in Soda‐Lime Glass , 1967 .

[29]  J. Rogers,et al.  GaAs photovoltaics and optoelectronics using releasable multilayer epitaxial assemblies , 2010, Nature.

[30]  M. Kanatzidis,et al.  Low-temperature fabrication of high-performance metal oxide thin-film electronics via combustion processing. , 2011, Nature materials.