Development and validation of transport models for the study of regional acid deposition require improved observations of pollutant transport and dispersion processes. No suitable method for air-parcel tracking along nonconstant density surfaces is available. The feasibility of using an airborne lidar system to observe atmospheric transport and dispersion of fluorescent-dye-particle (FDP) tracers was demonstrated for various meteorological conditions and FDP-release scenarios in the general area of the Cross-Appalachian Tracer Experiment (CAPTEX) during October 1983. This paper presents some of the results obtained on six case studies, each of which illustrates a unique application of the technique.