Dynamics of a colloidal particle coupled to a Gaussian field: from a confinement-dependent to a non-linear memory

The effective dynamics of a colloidal particle immersed in a complex medium is often described in terms of an overdamped linear Langevin equation for its velocity with a memory kernel which determines the effective (time-dependent) friction and the correlations of fluctuations. Recently, it has been shown in experiments and numerical simulations that this memory may depend on the possible optical confinement the particle is subject to, suggesting that this description does not capture faithfully the actual dynamics of the colloid, even at equilibrium. Here, we propose a different approach in which we model the medium as a Gaussian field linearly coupled to the colloid. The resulting effective evolution equation of the colloidal particle features a non-linear memory term which extends previous models and which explains qualitatively the experimental and numerical evidence in the presence of confinement. This non-linear term is related to the correlations of the effective noise via a novel fluctuation-dissipation relation which we derive.

[1]  D. Venturelli,et al.  Nonequilibrium relaxation of a trapped particle in a near-critical Gaussian field. , 2022, Physical review. E.

[2]  J. Fournier Field-mediated interactions of passive and conformation-active particles: multibody and retardation effects. , 2021, Soft matter.

[3]  J. Caspers,et al.  Barrier Crossing in a Viscoelastic Bath. , 2021, Physical Review Letters.

[4]  M. Gross Dynamics and steady states of a tracer particle in a confined critical fluid , 2021, Journal of Statistical Mechanics: Theory and Experiment.

[5]  Juan Ruben Gomez-Solano,et al.  Fluid Viscoelasticity Triggers Fast Transitions of a Brownian Particle in a Double Well Optical Potential. , 2020, Physical review letters.

[6]  C. Bechinger,et al.  Properties of a nonlinear bath: experiments, theory, and a stochastic Prandtl–Tomlinson model , 2019, New Journal of Physics.

[7]  F. van Wijland,et al.  Spatial organization of active particles with field-mediated interactions. , 2019, Physical review. E.

[8]  D. Beysens Brownian motion in strongly fluctuating liquid , 2019, Thermodynamique des interfaces et mécanique des fluides.

[9]  É. Fodor,et al.  Driven probe under harmonic confinement in a colloidal bath , 2018, Journal of Statistical Mechanics: Theory and Experiment.

[10]  Giovanni Volpe,et al.  Controlling the dynamics of colloidal particles by critical Casimir forces. , 2018, Soft matter.

[11]  R. Netz,et al.  External Potential Modifies Friction of Molecular Solutes in Water , 2017 .

[12]  Artyom Petrosyan,et al.  Energy Transfer between Colloids via Critical Interactions , 2017, Entropy.

[13]  Clemens Bechinger,et al.  Transient dynamics of a colloidal particle driven through a viscoelastic fluid , 2015, 1505.06674.

[14]  Uwe C. Täuber,et al.  Critical Dynamics: A Field Theory Approach to Equilibrium and Non-Equilibrium Scaling Behavior , 2014 .

[15]  Hugo Jacquin,et al.  Generalized Langevin equations for a driven tracer in dense soft colloids: construction and applications , 2014, 1401.5515.

[16]  Shamik Gupta,et al.  Dynamics of a tagged monomer: effects of elastic pinning and harmonic absorption. , 2013, Physical review letters.

[17]  Y. Fujitani,et al.  Drag coefficient of a rigid spherical particle in a near-critical binary fluid mixture, beyond the regime of the Gaussian model , 2013, Journal of Fluid Mechanics.

[18]  Hajime Tanaka,et al.  Nonequilibrium critical Casimir effect in binary fluids. , 2013, Physical review letters.

[19]  Valentin L. Popov,et al.  Prandtl‐Tomlinson model: History and applications in friction, plasticity, and nanotechnologies , 2012 .

[20]  L. Forró,et al.  Resonances arising from hydrodynamic memory in Brownian motion , 2011, Nature.

[21]  D. Dean,et al.  Perturbative path-integral study of active- and passive-tracer diffusion in fluctuating fields. , 2011, Physical review. E, Statistical, nonlinear, and soft matter physics.

[22]  G. Biroli,et al.  Symmetries of generating functionals of Langevin processes with colored multiplicative noise , 2010, 1007.5059.

[23]  P. Dommersnes,et al.  Fluctuations of the Casimir-like force between two membrane inclusions. , 2010, Physical review. E, Statistical, nonlinear, and soft matter physics.

[24]  C Bechinger,et al.  Critical Casimir effect in classical binary liquid mixtures. , 2009, Physical review. E, Statistical, nonlinear, and soft matter physics.

[25]  Denis Wirtz,et al.  Particle-tracking microrheology of living cells: principles and applications. , 2009, Annual review of biophysics.

[26]  S. Dietrich,et al.  Direct measurement of critical Casimir forces , 2008, Nature.

[27]  F. MacKintosh,et al.  Nonequilibrium Mechanics of Active Cytoskeletal Networks , 2007, Science.

[28]  D. Mizuno,et al.  Electrophoretic microrheology in a dilute lamellar phase of a nonionic surfactant. , 2001, Physical review letters.

[29]  R. Zwanzig Nonequilibrium statistical mechanics , 2001, Physics Subject Headings (PhySH).

[30]  Mason,et al.  Optical measurements of frequency-dependent linear viscoelastic moduli of complex fluids. , 1995, Physical review letters.

[31]  E. Hernández Nonequilibrium Statistical Mechanics , 1990 .

[32]  J. L. D. Rio-Correa,et al.  The fluctuation-dissipation theorem for non-Markov processes and their contractions: The role of the stationarity condition , 1987 .

[33]  Bertrand I. Halperin,et al.  Theory of dynamic critical phenomena , 1977, Physics Today.

[34]  M. Grunwald Principles Of Condensed Matter Physics , 2016 .

[35]  Y. Gliklikh The Langevin Equation , 1997 .

[36]  Jan K. G. Dhont,et al.  An introduction to dynamics of colloids , 1996 .

[37]  R. Kubo The fluctuation-dissipation theorem , 1966 .

[38]  L. Prandtl,et al.  Ein Gedankenmodell zur kinetischen Theorie der festen Körper , 1928 .