Observation of mean path length invariance in light-scattering media

Scattered light, it is all the same Materials can vary from transparent to opaque depending on the density of scatters within the medium. As light propagates through a material, intuition might suggest that the more scatters there are, the shorter the path along which the light can propagate. Savo et al. confirm a recent theoretical proposal that predicts that this is not the case. They shone light through a series of samples of varying scatterer density and found that the average path length that the light traveled was independent of the sample microstructure. This finding should also be applicable to acoustics and matter waves. Science, this issue p. 765 The average path length of light through a disordered medium is independent of the medium’s microstructure. The microstructure of a medium strongly influences how light propagates through it. The amount of disorder it contains determines whether the medium is transparent or opaque. Theory predicts that exciting such a medium homogeneously and isotropically makes some of its optical properties depend only on the medium’s outer geometry. Here, we report an optical experiment demonstrating that the mean path length of light is invariant with respect to the microstructure of the medium it scatters through. Using colloidal solutions with varying concentration and particle size, the invariance of the mean path length is observed over nearly two orders of magnitude in scattering strength. Our results can be extended to a wide range of systems—however ordered, correlated, or disordered—and apply to all wave-scattering problems.

[1]  Otto L Muskens,et al.  Design of light scattering in nanowire materials for photovoltaic applications. , 2008, Nano letters.

[2]  Peidong Yang,et al.  Light trapping in silicon nanowire solar cells. , 2010, Nano letters.

[3]  Salvatore Torquato,et al.  Designer disordered materials with large, complete photonic band gaps , 2009, Proceedings of the National Academy of Sciences.

[4]  V. Ntziachristos Going deeper than microscopy: the optical imaging frontier in biology , 2010, Nature Methods.

[5]  J. Sáenz,et al.  Density of states and extinction mean free path of waves in random media: dispersion relations and sum rules. , 2008, Physical review letters.

[6]  Philipp Ambichl,et al.  Spatiotemporal Control of Light Transmission through a Multimode Fiber with Strong Mode Coupling. , 2016, Physical review letters.

[7]  B. J. Ackerson,et al.  Correlation transfer - Application of radiative transfer solution methods to photon correlation problems , 1992 .

[8]  Ad Lagendijk,et al.  Resonant multiple scattering of light , 1996 .

[9]  S. Blanco,et al.  An invariance property of diffusive random walks , 2019, 1902.07080.

[10]  G. Popescu,et al.  Optical path-length spectroscopy of wave propagation in random media. , 1999, Optics letters.

[11]  G. Cody,et al.  Intensity enhancement in textured optical sheets for solar cells , 1982, IEEE Transactions on Electron Devices.

[12]  Arjun G. Yodh,et al.  Diffuse correlation spectroscopy for non-invasive, micro-vascular cerebral blood flow measurement , 2014, NeuroImage.

[13]  Fabrizio Martelli,et al.  Measurements of optical properties of high-density media. , 2003, Applied optics.

[14]  H. V. Hulst Light Scattering by Small Particles , 1957 .

[15]  S. Skipetrov,et al.  Localization of ultrasound in a three-dimensional elastic network , 2008, 0805.1502.

[16]  Aaswath Raman,et al.  Roadmap on optical energy conversion , 2016 .

[17]  J. Goodman Some fundamental properties of speckle , 1976 .

[18]  David A. Weitz,et al.  Ultralow-angle dynamic light scattering with a charge coupled device camera based multispeckle, multitau correlator , 1999 .

[19]  J. Joannopoulos,et al.  Photonic crystals: putting a new twist on light , 1997, Nature.

[20]  Suman Rana,et al.  Making sense of Brownian motion: colloid characterization by dynamic light scattering. , 2015, Langmuir : the ACS journal of surfaces and colloids.

[21]  P. de Vries,et al.  Observation of Anomalous Transport of Strongly Multiple Scattered Light in Thin Disordered Slabs , 1997 .

[22]  David A. Boas,et al.  PATH-LENGTH-RESOLVED DYNAMIC LIGHT SCATTERING IN HIGHLY SCATTERING RANDOM MEDIA : THE TRANSITION TO DIFFUSING WAVE SPECTROSCOPY , 1998 .

[23]  Anthony B. Davis,et al.  3D Radiative Transfer in Cloudy Atmospheres , 2005 .

[24]  P. Barthelemy,et al.  A Lévy flight for light , 2008, Nature.

[25]  R. Pecora Dynamic Light Scattering , 1985 .

[26]  Zongfu Yu,et al.  Fundamental limit of nanophotonic light trapping in solar cells , 2010, Proceedings of the National Academy of Sciences.

[27]  D. Weitz,et al.  Diffusing wave spectroscopy. , 1988, Physical review letters.

[28]  E. Yablonovitch Statistical ray optics , 1982 .

[29]  G. Maret,et al.  Multiple light scattering from disordered media. The effect of brownian motion of scatterers , 1987 .

[30]  L. Apresyan,et al.  Radiation transfer : statistical and wave aspects , 1996 .

[31]  Jochen Schröder,et al.  Observation of Eisenbud–Wigner–Smith states as principal modes in multimode fibre , 2015, Nature Photonics.

[32]  D. Durian,et al.  Accuracy of diffusing-wave spectroscopy theories. , 1995, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[33]  Matteo Burresi,et al.  Spatio-temporal visualization of light transport in complex photonic structures , 2015, Light: Science & Applications.

[34]  S. Gigan,et al.  Light fields in complex media: Mesoscopic scattering meets wave control , 2017, 1702.05395.

[35]  R. Carminati,et al.  Invariance property of wave scattering through disordered media , 2014, Proceedings of the National Academy of Sciences.

[36]  Vidya Ganapati,et al.  Light Trapping Textures Designed by Electromagnetic Optimization for Subwavelength Thick Solar Cells , 2013, IEEE Journal of Photovoltaics.

[37]  G. Ozin,et al.  Large-scale synthesis of a silicon photonic crystal with a complete three-dimensional bandgap near 1.5 micrometres , 2000, Nature.

[38]  D. Wiersma,et al.  Photon management in two-dimensional disordered media , 2012, 2013 Conference on Lasers & Electro-Optics Europe & International Quantum Electronics Conference CLEO EUROPE/IQEC.

[39]  Thomas F. Krauss,et al.  Enhanced energy storage in chaotic optical resonators , 2013, Nature Photonics.

[40]  R. Carminati,et al.  Beyond the diffusing-wave spectroscopy model for the temporal fluctuations of scattered light. , 2004, Physical review letters.

[41]  D. Wiersma,et al.  Exploiting breakdown of the similarity relation for diffuse light transport: simultaneous retrieval of scattering anisotropy and diffusion constant. , 2012, Optics letters.

[42]  Jaroslav Ricka,et al.  Dead‐time and afterpulsing correction in multiphoton timing with nonideal detectors , 1994 .

[43]  Michael Wahl,et al.  Fast calculation of fluorescence correlation data with asynchronous time-correlated single-photon counting. , 2003, Optics express.

[44]  Douglas J. Durian,et al.  Investigating non-Gaussian scattering processes by using nth-order intensity correlation functions , 1999 .

[45]  H. Atwater,et al.  Photonic design principles for ultrahigh-efficiency photovoltaics. , 2012, Nature materials.

[46]  R. Pierrat Transport equation for the time correlation function of scattered field in dynamic turbid media. , 2008, Journal of the Optical Society of America. A, Optics, image science, and vision.

[47]  B. Ackerson,et al.  Correlation transfer: development and application. , 1994 .