An Experimental and Modeling Investigation of Al-based Nanocomposites Manufactured via Ultrasonic Cavitation and Solidification Processing

Abstract In the present study, A356 based nano-composites are fabricated by using the ultrasonic stirring technology (UST) in a coreless induction furnace. SiC nanoparticles were used as the reinforcement. Nanoparticles were added into the molten metal and then dispersed by ultrasonic cavitation and acoustic streaming assisted by electromagnetic stirring. The UST was also applied during the solidification process. The microstructure of the nanocomposites has been investigated by optical microscopy and scanning electron microscopy (SEM). The distribution of SiC nanoparticles in the A356 alloy matrix has also been analyzed. The SEM and energy dispersive X-ray spectroscopy (EDS) analyses showed that the matrix microstructure of the A356 alloy and the dispersion of the SiC nanoparticles into the matrix can be significantly improved when ultrasonic cavitation, induction melting and stirring, and solidification processing techniques are used together. Molecular dynamics (MD) simulations were conducted to analyze the complex interactions between the nanoparticle and the liquid/solid interface. The assumption that nanoparticles will be engulfed by the solidification front instead of being pushed was proved through MD simulations.

[1]  Matthew S. Dargusch,et al.  The role of ultrasonic treatment in refining the as-cast grain structure during the solidification of an Al–2Cu alloy , 2014 .

[2]  A. Moitra,et al.  Behavior of ceramic particles at the solid- liquid metal interface in metal matrix composites , 1988, Metallurgical and Materials Transactions A.

[3]  Chang-soo Kim,et al.  Impact of Brownian motion on the particle settling in molten metals , 2014, Metals and Materials International.

[4]  Yang Li,et al.  Effect of ultrasonic treatment on microstructures of hypereutectic Al-Si alloy , 2008 .

[5]  D. Božić,et al.  Influence of SiC particles distribution on mechanical properties and fracture of DRA alloys , 2010 .

[6]  Tersoff Carbon defects and defect reactions in silicon. , 1990, Physical review letters.

[7]  T. Meek,et al.  Effect of power ultrasound on solidification of aluminum A356 alloy , 2005 .

[8]  W. Yoon,et al.  Improved mechanical properties of near-eutectic Al-Si piston alloy through ultrasonic melt treatment , 2016 .

[9]  S. Reihani Processing of squeeze cast Al6061–30vol% SiC composites and their characterization , 2006 .

[10]  Hongge Yan,et al.  Study on the preparation of the SiCp/Al–20Si–3Cu functionally graded material using spray deposition , 2010 .

[11]  L. Nastac,et al.  The role of ultrasonic cavitation in refining the microstructure of aluminum based nanocomposites during the solidification process , 2018, Ultrasonics.

[12]  P. Allison,et al.  Microstructure, mechanical properties and fracture behavior of 6061 aluminium alloy-based nanocomposite castings fabricated by ultrasonic processing , 2016 .

[13]  M. Qian,et al.  High-intensity ultrasonic grain refinement of magnesium alloys: role of solute , 2009 .

[14]  Xiaochun Li,et al.  Study on bulk aluminum matrix nano-composite fabricated by ultrasonic dispersion of nano-sized SiC particles in molten aluminum alloy , 2004 .

[15]  J. Tersoff,et al.  Modeling solid-state chemistry: Interatomic potentials for multicomponent systems. , 1989, Physical review. B, Condensed matter.

[16]  Y. Osawa,et al.  Grain refinement of AZ91 alloy by introducing ultrasonic vibration during solidification , 2008 .

[17]  Michael J. Mehl,et al.  Interatomic potentials for monoatomic metals from experimental data and ab initio calculations , 1999 .

[18]  Xing Ma,et al.  Ultrasonic assisted fabrication of particle reinforced bonds joining aluminum metal matrix composites , 2011 .

[19]  M. Gupta,et al.  Simultaneous enhancement in strength and ductility by reinforcing magnesium with carbon nanotubes , 2006 .

[20]  H. Baharvandi,et al.  Fabrication and study on mechanical properties and fracture behavior of nanometric Al2O3 particle-reinforced A356 composites focusing on the parameters of vortex method , 2013 .

[21]  D. Stefanescu Science and Engineering of Casting Solidification , 2002 .

[22]  L. Nastac,et al.  Experimental and Numerical Analysis of the 6061-Based Nanocomposites Fabricated via Ultrasonic Processing , 2015, Journal of Materials Engineering and Performance.

[23]  Alain Karma,et al.  Atomistic Simulation Methods for Computing the Kinetic Coefficient in Solid-Liquid Systems , 2002 .

[24]  Nanxian Chen,et al.  Interfacial potentials for Al/SiC(111) , 2009, Journal of physics. Condensed matter : an Institute of Physics journal.

[25]  H. Baharvandi,et al.  Fabrication of nano-sized Al2O3 reinforced casting aluminum composite focusing on preparation process of reinforcement powders and evaluation of its properties , 2013 .

[26]  D. Brabazon,et al.  Computational and experimental analysis of particulate distribution during Al-SiC MMC fabrication , 2007 .

[27]  Yung C. Shin,et al.  Molecular dynamics based cohesive zone law for describing Al–SiC interface mechanics , 2011 .

[28]  Y. Xuan,et al.  An experimental and modeling investigation of aluminum-based alloys and nanocomposites processed by ultrasonic cavitation processing , 2016 .