Predicting Particulate (PM10) Personal Exposure Distributions Using a Random Component Superposition Statistical Model

ABSTRACT This paper presents a new statistical model designed to extend our understanding from prior personal exposure field measurements of urban populations to other cities where ambient monitoring data, but no personal exposure measurements, exist. The model partitions personal exposure into two distinct components: ambient concentration and nonambient concentration. It is assumed the ambient and nonambient concentration components are uncorrelated and add together; therefore, the model is called a random component superposition (RCS) model. The 24-hr ambient outdoor concentration is multiplied by a dimensionless “attenuation factor” between 0 and 1 to account for deposition of particles as the ambient air infiltrates indoors. The RCS model is applied to field PM10 measurement data from three large-scale personal exposure field studies: THEES (Total Human Environmental Exposure Study) in Phillipsburg, NJ; PTEAM (Particle Total Exposure Assessment Methodology) in Riverside, CA; and the Ethyl Corporation study in Toronto, Canada. Because indoor sources and activities (smoking, cooking, cleaning, the personal cloud, etc.) may be similar in similar populations, it was hypothesized that the statistical distribution of nonambient personal exposure is invariant across cities.

[1]  L. Wallace,et al.  A decade of studies of human exposure: what have we learned? , 1993, Risk analysis : an official publication of the Society for Risk Analysis.

[2]  J. Waldman,et al.  The Total Human Environmental Exposure Study (THEES) to benzo(a)pyrene: comparison of the inhalation and food pathways. , 1988, Archives of environmental health.

[3]  C A Clayton,et al.  Particle Total Exposure Assessment Methodology (PTEAM) 1990 study: method performance and data quality for personal, indoor, and outdoor monitoring. , 1993, Journal of exposure analysis and environmental epidemiology.

[4]  N. Klepeis A Total Human Exposure Model (THEM) for Respirable Suspended Particles (RSP) , 1994 .

[5]  P. L. Jenkins,et al.  Activity patterns of Californians: Use of and proximity to indoor pollutant sources , 1992 .

[6]  H Ozkaynak,et al.  A population-based exposure model for benzene. , 1995, Journal of exposure analysis and environmental epidemiology.

[7]  W. Ott,et al.  Human exposure assessment: the birth of a new science. , 1995, Journal of exposure analysis and environmental epidemiology.

[8]  W. Ott,et al.  Total human exposure: basic concepts, EPA field studies, and future research needs. , 1990, Journal of the Air & Waste Management Association.

[9]  Lance Wallace,et al.  VALIDATION OF THE SIMULATION OF HUMAN ACTIVITY AND POLLUTANT EXPOSURE (SHAPE) MODEL USING PAIRED DAYS FROM THE DENVER, CO, CARBON MONOXIDE FIELD STUDY , 1988 .

[10]  P. Lioy,et al.  The personal, indoor and outdoor concentrations of PM-10 measured in an industrial community during the winter , 1990 .

[11]  V. Hasselblad,et al.  Assessment of human exposure to ambient particulate matter. , 1999, Journal of the Air & Waste Management Association.

[12]  J. Thomas,et al.  Comparison of microenvironmental CO concentrations in two cities for human exposure modeling. , 1992, Journal of exposure analysis and environmental epidemiology.

[13]  T McCurdy Estimating human exposure to selected motor vehicle pollutants using the NEM series of models: lessons to be learned. , 1995, Journal of exposure analysis and environmental epidemiology.

[14]  Roy Whitmore,et al.  Measuring human exposure to carbon monoxide in Washington, DC, and Denver, Colorado during the Winter of 1982-1983 , 1985 .

[15]  Lance Wallace,et al.  The TEAM Study: Personal Exposures to Toxic Substances in Air, Drinking Water, and Breath of 400 Residents of , 1987 .

[16]  W R Ott,et al.  Exposure estimates based on computer generated activity patterns. , 1983, Journal of toxicology. Clinical toxicology.

[17]  J D Spengler,et al.  Particle Total Exposure Assessment Methodology (PTEAM) study: distributions of aerosol and elemental concentrations in personal, indoor, and outdoor air samples in a southern California community. , 1993, Journal of exposure analysis and environmental epidemiology.

[18]  R W Whitmore,et al.  The influence of personal activities on exposure to volatile organic compounds. , 1989, Environmental research.

[19]  Donald D. Rosebrook,et al.  Total exposure assessment methodology (team) study: Personal exposures, indoor-outdoor relationships, and breath levels of volatile organic compounds in New Jersey , 1993 .

[20]  G. D. Pfeifer,et al.  Particulate matter and manganese exposures in Toronto, Canada , 1999 .

[21]  R. G. Lewis,et al.  Non-occupational exposures to pesticides for residents of two U.S. cities , 1994, Archives of environmental contamination and toxicology.

[22]  A. Watson,et al.  Assessment of Human Exposure to Air Pollution: Methods, Measurements, and Models , 1988 .

[23]  T R Johnson Recent advances in the estimation of population exposure to mobile source pollutants. , 1995, Journal of exposure analysis and environmental epidemiology.

[24]  Wayne R. Ott,et al.  ENVIRONMENTAL STATISTICS and DATA ANALYSIS , 1995 .

[25]  L. Wallace,et al.  Indoor particles: a review. , 1996, Journal of the Air & Waste Management Association.

[26]  S. Miller,et al.  Exposure to toxic air contaminants in environmental tobacco smoke: an assessment for California based on personal monitoring data. , 1998, Journal of exposure analysis and environmental epidemiology.

[27]  P. Lioy,et al.  Calibration, Intersampler Comparison, and Field Application of a New PM-10 Personal Air-Sampling Impactor , 1991 .

[28]  Johnson Tr Recent advances in the estimation of population exposure to mobile source pollutants. , 1995 .

[29]  L. L. Piper,et al.  Estimating distributions of long-term particulate matter and manganese exposures for residents of Toronto, Canada , 1999 .

[30]  L. A. Wallace Human exposure to environmental pollutants: a decade of experience , 1995, Clinical and experimental allergy : journal of the British Society for Allergy and Clinical Immunology.

[31]  P. Stolpman,et al.  Environmental Protection Agency , 2020, The Grants Register 2022.

[32]  J. Xue,et al.  Personal exposure to airborne particles and metals: results from the Particle TEAM study in Riverside, California. , 1996, Journal of exposure analysis and environmental epidemiology.

[33]  R. Kamens,et al.  The Significance and Characteristics of the Personal Activity Cloud on Exposure Assessment Measurements for Indoor Contaminants , 1991 .

[34]  P. Switzer,et al.  Investigations of the proximity effect for pollutants in the indoor environment , 1999, Journal of Exposure Analysis and Environmental Epidemiology.

[35]  J. M. Hammersley,et al.  Basic Concepts of Probability and Statistics , 1964 .

[36]  N. Duan,et al.  Stochastic microenvironment models for air pollution exposure. , 1991, Journal of exposure analysis and environmental epidemiology.

[37]  Richard F. Gunst,et al.  Applied Regression Analysis , 1999, Technometrics.

[38]  L. Wallace Correlations of Personal Exposure to Particles with Outdoor Air Measurements: A Review of Recent Studies , 2000 .

[39]  D. Rosebrook,et al.  Personal exposures, indoor-outdoor relationships, and breath levels of toxic air pollutants measured for 355 persons in New Jersey , 1993 .