Explanation of discrepancies among satellite observations of the aerosol indirect effects

[1] Satellite-based remote sensing instruments for measuring the aerosol indirect effect (IE = −d ln re/d ln τa where re is the cloud drop effective radius and τa is the aerosol optical depth) show large disparities in the magnitude of the effect for similar regions of the globe. Over the oceans, the Advanced Very High Resolution Radiometer (AVHRR) measures an indirect effect twice that measured by the POLarization and Directionality of the Earth Reflectances (POLDER) (0.17 vs. 0.085). We address possible reasons for these disparities. It is argued that AVHRR misses the optically thin and broken clouds, especially over land, while POLDER misses clouds with variable top heights in its field of view. POLDER is also biased to thinner, less turbulent clouds. The sensitivity of the indirect effect to cloud turbulence therefore biases POLDER to lower values. POLDER measures an indirect effect over the ocean that is about twice that over the land (0.085 vs. 0.04). By considering factors such as dynamics, variability in cloud liquid water path, decoupling of the boundary layer, and the effect of salt particles, we argue that this could be an artifact, and that the indirect effect on cloud microstructure may be stronger over land than over the ocean.

[1]  Itamar M. Lensky,et al.  Satellite-Based Insights into Precipitation Formation Processes in Continental and Maritime Convective Clouds , 1998 .

[2]  S. Twomey,et al.  Determining the Susceptibility of Cloud Albedo to Changes in Droplet Concentration with the Advanced Very High Resolution Radiometer , 1994 .

[3]  Yoram J. Kaufman,et al.  Analysis of smoke impact on clouds in Brazilian biomass burning regions: An extension of Twomey's approach , 2001 .

[4]  François-Marie Bréon,et al.  Cloud droplet effective radius from spaceborne polarization measurements , 1998 .

[5]  S. Ghan,et al.  Competition between Sea Salt and Sulfate Particles as Cloud Condensation Nuclei , 1998 .

[6]  F. Bréon,et al.  Aerosol Effect on Cloud Droplet Size Monitored from Satellite , 2002, Science.

[7]  A. H. Woodcock SALT NUCLEI IN MARINE AIR AS A FUNCTION OF ALTITUDE AND WIND FORCE , 1953 .

[8]  Glen Lesins,et al.  Stronger Constraints on the Anthropogenic Indirect Aerosol Effect , 2002, Science.

[9]  George A. Isaac,et al.  Physical and chemical observations in marine stratus during the 1993 North Atlantic Regional Experiment: Factors controlling cloud droplet number concentrations , 1996 .

[10]  Alexander Khain,et al.  The Role of Sea Spray in Cleansing Air Pollution over Ocean via Cloud Processes , 2002, Science.

[11]  Dana E. Veron,et al.  First measurements of the Twomey indirect effect using ground‐based remote sensors , 2003 .

[12]  Harshvardhan,et al.  Influence of anthropogenic aerosol on cloud optical depth and albedo shown by satellite measurements and chemical transport modeling , 2002, Proceedings of the National Academy of Sciences of the United States of America.

[13]  G. Müller,et al.  The Scientific Basis , 1995 .

[14]  S. Twomey The Influence of Pollution on the Shortwave Albedo of Clouds , 1977 .

[15]  Teruyuki Nakajima,et al.  A possible correlation between satellite‐derived cloud and aerosol microphysical parameters , 2001 .

[16]  Annick Bricaud,et al.  The POLDER mission: instrument characteristics and scientific objectives , 1994, IEEE Trans. Geosci. Remote. Sens..

[17]  E. Williams,et al.  The physical origin of the land–ocean contrast in lightning activity , 2002 .