Oscillating bubble concentration and its size distribution using acoustic emission spectra.

New method has been proposed for the estimation of size and number density distribution of oscillating bubbles in a sonochemical reactor using acoustic emission spectra measurements. Bubble size distribution has been determined using Minnaert's equation [M. Minnaert, On musical air bubbles and sound of running water, Philanthr. Mag. 16 (1933) 235], i.e., size of oscillating bubble is inversely related to the frequency of its volume oscillations. Decomposition of the pressure signal measured by the hydrophone in frequency domain of FFT spectrum and then inverse FFT reconstruction of the signal at each frequency level has been carried out to get the information about each of the bubble/cavity oscillation event. The number mean radius of the bubble size is calculated to be in the range of 50-80 microm and it was not found to vary much with the spatial distribution of acoustic field strength of the ultrasound processor used in the work. However, the number density of the oscillating bubbles and the nature of the distribution were found to vary in different horizontal planes away from the driving transducer surface in the ultrasonic bath. A separate set of experiments on erosion assessment studies were carried out using a thin aluminium foil, revealing a phenomena of active region of oscillating bubbles at antinodal points of the stationary waves, identical to the information provided by the acoustic emission spectra at the same location in the ultrasonic bath.

[1]  Andrea Prosperetti,et al.  Linear pressure waves in bubbly liquids: Comparison between theory and experiments , 1989 .

[2]  A. E. Crawford The measurement of cavitation , 1964 .

[3]  W. Lauterborn,et al.  EXPERIMENTAL APPROACH TO A COMPLEX ACOUSTIC SYSTEM , 1993 .

[4]  Aniruddha B. Pandit,et al.  Mapping the cavitation intensity in an ultrasonic bath using the acoustic emission , 2000 .

[5]  Clive Temperton Implementation of a self-sorting in-place prime factor FFT algorithm , 1985 .

[6]  L. Rayleigh VIII. On the pressure developed in a liquid during the collapse of a spherical cavity , 1917 .

[7]  M. Minnaert XVI.On musical air-bubbles and the sounds of running water , 1933 .

[8]  Andrea Prosperetti,et al.  Nonlinear bubble dynamics , 1988 .

[9]  C. Bruneel,et al.  Ultrasonic cavitation monitoring by acoustic noise power measurement , 2000, The Journal of the Acoustical Society of America.

[10]  J. Varley,et al.  Sound measurement as a means of gas‐bubble sizing in aerated agitated tanks , 1998 .

[11]  P. Gogate,et al.  Cavity cluster approach for quantification of cavitational intensity in sonochemical reactors. , 2003, Ultrasonics sonochemistry.

[12]  M. Ashokkumar,et al.  Determination of the size distribution of sonoluminescence bubbles in a pulsed acoustic field. , 2005, Journal of the American Chemical Society.

[13]  John M. Killen,et al.  An Evaluation of Acoustic Techniques for Measuring Gas Bubble Size Distributions in Cavitation Research , 1971 .

[14]  A. Pandit,et al.  Steam bubble cavitation , 2008 .

[15]  F. R. Schiebe The Influence of Gas Nuclei Size Distribution on Transient Cavitation Near Inception , 1969 .

[16]  V. S. Moholkar,et al.  Hydrodynamic cavitation for sonochemical effects. , 1999, Ultrasonics sonochemistry.

[17]  A. Prosperetti,et al.  Bubble Dynamics and Cavitation , 1977 .

[18]  M. Longuet-Higgins,et al.  Monopole emission of sound by asymmetric bubble oscillations. Part 1. Normal modes , 1989, Journal of Fluid Mechanics.

[19]  A. V. Tolkachev,et al.  Fiber optics LDA and laser knife simultaneous use for flow investigation , 1993, Other Conferences.

[20]  Z. Derouiche,et al.  Acoustic Signature Estimation Of The Cavitation Noise. , 1993 .

[21]  Aniruddha B. Pandit,et al.  Measurement of bubble size distribution: an acoustic technique , 1992 .

[22]  N. A. Tsochatzidis,et al.  Determination of velocity, size and concentration of ultrasonic cavitation bubbles by the phase-Doppler technique , 2001 .

[23]  M. Strasberg,et al.  Gas Bubbles as Sources of Sound in Liquids , 1956 .