Time-of-flight-photoelectron emission microscopy on plasmonic structures using attosecond extreme ultraviolet pulses

We report on the imaging of plasmonic structures by time-of-flight-photoemission electron microscopy (ToF-PEEM) in combination with extreme ultraviolet (XUV) attosecond pulses from a high harmonic generation source. Characterization of lithographically fabricated Au structures using these ultrashort XUV pulses by ToF-PEEM shows a spatial resolution of ∼200 nm. Energy-filtered imaging of the secondary electrons resulting in reduced chromatic aberrations as well as microspectroscopic identification of core and valence band electronic states have been successfully proven. We also find that the fast valence band electrons are not influenced by space charge effects, which is essentially important for attosecond nanoplasmonic-field microscopy realization.

[1]  Ferenc Krausz,et al.  Time of flight-photoemission electron microscope for ultrahigh spatiotemporal probing of nanoplasmonic optical fields , 2009, Journal of physics. Condensed matter : an Institute of Physics journal.

[2]  Ferenc Krausz,et al.  Attosecond Nanoplasmonic Field Microscope , 2007 .

[3]  S. Sivananthan,et al.  Selective growth of CdTe on patterned CdTe∕Si(211) , 2008 .

[4]  G. Schönhense,et al.  Image enhancement in photoemission electron microscopy by means of imaging time-of-flight analysis , 2004 .

[5]  Martin Aeschlimann,et al.  Time- and energy resolved photoemission electron microscopy-imaging of photoelectron time-of-flight analysis by means of pulsed excitations , 2010 .

[6]  M. Mazzoni,et al.  First-principles investigation of electrochemical properties of gold nanoparticles , 2010, Nanotechnology.

[7]  U. Kleineberg,et al.  Time-of-flight photoelectron emission microscopy TOF-PEEM: first results , 1998 .

[8]  P. Zhou,et al.  Space charge effects in photoemission electron microscopy using amplified femtosecond laser pulses , 2009, Journal of physics. Condensed matter : an Institute of Physics journal.

[9]  M. Aeschlimann,et al.  Space charge effects in photoemission with a low repetition, high intensity femtosecond laser source , 2006 .

[10]  N. V. Smith,et al.  Photoemission spectra and band structures of d -band metals. IV. X-ray photoemission spectra and densities of states in Rh, Pd, Ag, Ir, Pt, and Au , 1974 .

[11]  E. Lundgren,et al.  Photoemission electron microscopy using extreme ultraviolet attosecond pulse trains. , 2009, The Review of scientific instruments.

[12]  U. Kleineberg,et al.  Atomic transient recorder , 2004, Nature.