Electronic structure of FeS

Here we report the electronic structure of FeS, a recently identified iron-based superconductor. Our high-resolution angle-resolved photoemission spectroscopy studies show two hole-like ($\alpha$ and $\beta$) and two electron-like ($\eta$ and $\delta$) Fermi pockets around the Brillouin zone center and corner, respectively, all of which exhibit moderate dispersion along $k_z$. However, a third hole-like band ($\gamma$) is not observed, which is expected around the zone center from band calculations and is common in iron-based superconductors. Since this band has the highest renormalization factor and is known to be the most vulnerable to defects, its absence in our data is likely due to defect scattering --- and yet superconductivity can exist without coherent quasiparticles in the $\gamma$ band. This may help resolve the current controversy on the superconducting gap structure of FeS. Moreover, by comparing the $\beta$ bandwidths of various iron chalcogenides, including FeS, FeSe$_{1-x}$S$_x$, FeSe, and FeSe$_{1-x}$ Te$_x$, we find that the $\beta$ bandwidth of FeS is the broadest. However, the band renormalization factor of FeS is still quite large, when compared with the band calculations, which indicates sizable electron correlations. This explains why the unconventional superconductivity can persist over such a broad range of isovalent substitution in FeSe$_{1-x}$Te$_{x}$ and FeSe$_{1-x}$S$_{x}$.

[1]  W. Hager,et al.  and s , 2019, Shallow Water Hydraulics.

[2]  Thomas Wolf,et al.  Superconductivity‐enhanced nematicity and “s+d” gap symmetry in Fe(Se1−xSx) , 2016, 1607.01288.

[3]  T. Terashima,et al.  Upper critical field and quantum oscillations in tetragonal superconducting FeS , 2016, 1608.01043.

[4]  S. Blundell,et al.  Robustness of superconductivity to competing magnetic phases in tetragonal FeS , 2016, 1607.00953.

[5]  C. Krellner,et al.  Impurity scattering effects on the superconducting properties and the tetragonal-to-orthorhombic phase transition in FeSe , 2016 .

[6]  J. Tian,et al.  Critical current density and vortex pinning in tetragonal FeS1-xSex(x = 0,0.06) , 2016, 1605.09791.

[7]  Xiyu Zhu,et al.  Strong-coupling superconductivity revealed by scanning tunneling microscope in tetragonal FeS , 2016, 1605.05184.

[8]  M. Abdel-Hafiez,et al.  Highly Anisotropic and Twofold Symmetric Superconducting Gap in Nematically Ordered FeSe_{0.93}S_{0.07}. , 2016, Physical review letters.

[9]  Wan-Sheng Wang,et al.  Electronic structure and d x 2 -y 2 -wave superconductivity in FeS , 2016 .

[10]  M. Fang,et al.  A unifying phase diagram with correlation-driven superconductor-to-insulator transition for the 122 series of iron chalcogenides , 2016 .

[11]  C. Baines,et al.  Coexistence of low-moment magnetism and superconductivity in tetragonal FeS and suppression of T-c under pressure , 2016, 1602.01987.

[12]  J. Q. Yan,et al.  Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe , 2015, Nature Communications.

[13]  Yufeng Li,et al.  Nodal superconducting gap in tetragonal FeS , 2015, 1512.04074.

[14]  M. X. Wang,et al.  Nodal superconductivity in FeS: Evidence from quasiparticle heat transport , 2015, 1511.07717.

[15]  D. Johrendt,et al.  Structural transition and superconductivity in hydrothermally synthesized FeX (X = S, Se). , 2015, Chemical communications.

[16]  X. H. Chen,et al.  Evolution of High-Temperature Superconductivity from a Low-T_{c} Phase Tuned by Carrier Concentration in FeSe Thin Flakes. , 2015, Physical review letters.

[17]  X. Lou,et al.  Anomalous correlation effects and unique phase diagram of electron-doped FeSe revealed by photoemission spectroscopy , 2015, Nature Communications.

[18]  M. Abdel-Hafiez,et al.  Strong interplay between stripe spin fluctuations, nematicity and superconductivity in FeSe. , 2015, Nature materials.

[19]  T. Wolf,et al.  Suppression of orbital ordering by chemical pressure in FeSe1-xSx , 2015, 1508.05016.

[20]  Fuqiang Huang,et al.  Observation of Superconductivity in Tetragonal FeS. , 2015, Journal of the American Chemical Society.

[21]  Yulin Chen,et al.  Experimental observation of incoherent-coherent crossover and orbital-dependent band renormalization in iron chalcogenide superconductors , 2015, 1505.03074.

[22]  D. Knyazev,et al.  Superconducting properties of sulfur-doped iron selenide , 2015, 1501.07346.

[23]  H. Yang,et al.  Significant contribution of As 4 p orbitals to the low-lying electronic structure of the 112-type iron-based superconductor Ca 0.9 La 0.1 FeAs 2 , 2014, 1411.5525.

[24]  D. Feng Extraordinary Doping Effects on Quasiparticle Scattering and Bandwidth in Iron-Based Superconductors , 2014 .

[25]  Z. K. Liu,et al.  Interfacial mode coupling as the origin of the enhancement of Tc in FeSe films on SrTiO3 , 2013, Nature.

[26]  B. Buchner,et al.  Unusual band renormalization in the simplest iron-based superconductor FeSe 1 − x , 2013, 1307.1280.

[27]  T. Xiang,et al.  Interface-induced superconductivity and strain-dependent spin density waves in FeSe/SrTiO3 thin films. , 2013, Nature materials.

[28]  T. Qian,et al.  Three dimensionality and orbital characters of the Fermi surface in (Tl,Rb)(y)Fe(2-x)Se2. , 2012, Physical review letters.

[29]  Q. Xue,et al.  High temperature superconductivity in single unit-cell FeSe films on SrTiO$_{3}$ , 2014 .

[30]  X. Dai,et al.  Orbital characters determined from Fermi surface intensity patterns using angle-resolved photoemission spectroscopy , 2012, 1201.3655.

[31]  Q. Ge,et al.  Nodal superconducting-gap structure in ferropnictide superconductor BaFe2(As0.7P0.3)2 , 2011, Nature Physics.

[32]  Jiangping Hu,et al.  Local antiferromagnetic exchange and collaborative Fermi surface as key ingredients of high temperature superconductors , 2011, Scientific Reports.

[33]  M. Fang,et al.  Superconductivity close to magnetic instability in Fe ( Se 1 − x Te x ) 0.82 , 2008, 0807.4775.

[34]  David J. Singh,et al.  Density functional study of FeS, FeSe and FeTe: Electronic structure, magnetism, phonons and superconductivity , 2008, 0807.4312.

[35]  F. Hsu,et al.  Superconductivity in the PbO-type structure α-FeSe , 2008, Proceedings of the National Academy of Sciences.

[36]  J. M. Luttinger FERMI SURFACE AND SOME SIMPLE EQUILIBRIUM PROPERTIES OF A SYSTEM OF INTERACTING FERMIONS , 1960 .