A set of prompt partial γ -ray production cross sections from thermal neutron-capture were measured for the 139 La( n, γ ) reaction using a guided beam of subthermal (thermal and cold) neutrons incident upon a nat La 2 O 3 target at the Prompt Gamma Activation Analysis facility of the Budapest Research Reactor. Absolute 140 La cross sections were determined relative to the well-known comparator 35 Cl( n, γ ) cross sections from the irradiation of a stoichiometric nat LaCl 3 sample. The total cross section for radiative thermal neutron-capture on 139 La from the sum of experimentally measured cross sections observed to directly feed the 140 La ground state was determined to be σ expt0 = 8 . 58(50) b. To assess completeness of the decay scheme and as a consistency check, the measured cross sections for transitions feeding the ground state from levels below a critical energy of E c = 285 keV were combined with a modeled contribution accounting for ground-state feeding from the quasicontinuum to arrive at a total cross section of σ 0 = 9 . 36(74) b. In addition, a neutron-separation energy of S n = 5161 . 005(21) keV was determined from a least-squares fit of the measured primary γ -ray energies to the low-lying levels of the 140 La decay scheme. Furthermore, several nuclear structure improvements are proposed for the decay scheme. The measured cross-section and separation-energy results are comparable to earlier measurements of these quantities.
[1]
R. Sarpong,et al.
Bio-inspired synthesis of xishacorenes A, B, and C, and a new congener from fuscol† †Electronic supplementary information (ESI) available. See DOI: 10.1039/c9sc02572c
,
2019,
Chemical science.
[2]
F. Kondev,et al.
Nuclear Data Needs and Capabilities for Applications
,
2015,
1511.07772.
[3]
Said F. Mughabghab,et al.
Atlas of Neutron Resonances: Resonance Parameters and Thermal Cross Sections. Z=1-100
,
2006
.
[4]
S. Landsberger.
Handbook of Prompt Gamma Activation Analysis with Neutron Beams
,
2005
.
[5]
Z. Révay,et al.
Database of prompt gamma rays from slow neutron capture for elemental analysis
,
2004
.
[6]
P. Obložinský,et al.
Handbook for calculations of nuclear reaction data, RIPL-2 (Reference Input Parameter Library-2)
,
2006
.