Current status and prospects of memristors based on novel 2D materials

As promising non-volatile memory devices, memristors have received extensive attention since they can effectively mimic synapses and enable the fabrication of neuromorphic systems. In recent years, 2D materials have been widely used in memristors because of their unique advantages, which not only improve the performance of memristors, but also promote the applicability of memristors in flexible electronics, low-power high-temperature devices, neuromorphic computing, etc. In this review, we summarize the applications of 2D materials in fabricating memristors and their physical switching mechanisms. The challenges involved are discussed and the corresponding strategies are reviewed.

[1]  E. Reed,et al.  Structural Phase Transitions by Design in Monolayer Alloys. , 2016, ACS nano.

[2]  Jianhui Zhao,et al.  Highly improved performance in Zr0.5Hf0.5O2 films inserted with graphene oxide quantum dots layer for resistive switching non-volatile memory , 2017 .

[3]  Wei Yi,et al.  Biological plausibility and stochasticity in scalable VO2 active memristor neurons , 2018, Nature Communications.

[4]  D. Fan,et al.  Broadband Nonlinear Photoresponse of 2D TiS2 for Ultrashort Pulse Generation and All‐Optical Thresholding Devices , 2018 .

[5]  Thomas Heine,et al.  Influence of quantum confinement on the electronic structure of the transition metal sulfide T S 2 , 2011, 1104.3670.

[6]  Harold S. Park,et al.  Negative poisson’s ratio in single-layer black phosphorus , 2014, Nature Communications.

[7]  Wei Huang,et al.  Preparation of MoS₂-polyvinylpyrrolidone nanocomposites for flexible nonvolatile rewritable memory devices with reduced graphene oxide electrodes. , 2012, Small.

[8]  Weiwei Xia,et al.  Memristor Crossbars with 4.5 Terabits-per-Inch-Square Density and Two Nanometer Dimension , 2018, ArXiv.

[9]  D. Fan,et al.  Broadband Nonlinear Photonics in Few‐Layer MXene Ti3C2Tx (T = F, O, or OH) , 2018 .

[10]  C Jeffrey Brinker,et al.  Chemically exfoliated MoS2 as near-infrared photothermal agents. , 2012, Angewandte Chemie.

[11]  P. Chu,et al.  Biodegradable black phosphorus-based nanospheres for in vivo photothermal cancer therapy , 2016, Nature Communications.

[12]  J. Coleman,et al.  High-yield production of graphene by liquid-phase exfoliation of graphite. , 2008, Nature nanotechnology.

[13]  J. Yang,et al.  Truly Electroforming‐Free and Low‐Energy Memristors with Preconditioned Conductive Tunneling Paths , 2017 .

[14]  Shuangchun Wen,et al.  Mechanically exfoliated black phosphorus as a new saturable absorber for both Q-switching and Mode-locking laser operation. , 2015, Optics express.

[15]  Mario Lanza,et al.  Bimodal Dielectric Breakdown in Electronic Devices Using Chemical Vapor Deposited Hexagonal Boron Nitride as Dielectric , 2018 .

[16]  F. Guinea,et al.  The electronic properties of graphene , 2007, Reviews of Modern Physics.

[17]  Hua Zhang,et al.  A High‐Rate and Stable Quasi‐Solid‐State Zinc‐Ion Battery with Novel 2D Layered Zinc Orthovanadate Array , 2018, Advanced materials.

[18]  J. Slaughter,et al.  Progress and outlook for MRAM technology , 1999, IEEE International Magnetics Conference.

[19]  Hua Zhang,et al.  Non-volatile resistive memory devices based on solution-processed ultrathin two-dimensional nanomaterials. , 2015, Chemical Society reviews.

[20]  Mengchen Zhang,et al.  3D nanoporous crystals enabled 2D channels in graphene membrane with enhanced water purification performance , 2017 .

[21]  D. Fan,et al.  Biocompatible Two-Dimensional Titanium Nanosheets for Multimodal Imaging-Guided Cancer Theranostics. , 2019, ACS applied materials & interfaces.

[22]  Aaron M. Jones,et al.  Electrical tuning of valley magnetic moment through symmetry control in bilayer MoS2 , 2012, 1208.6069.

[23]  Kaiyou Wang,et al.  High‐Performance, Self‐Driven Photodetector Based on Graphene Sandwiched GaSe/WS2 Heterojunction , 2018 .

[24]  William A. Goddard,et al.  Field-effect transistors made from solution-grown two-dimensional tellurene , 2017, 1704.06202.

[25]  M. Yun,et al.  Low‐Power, Electrochemically Tunable Graphene Synapses for Neuromorphic Computing , 2018, Advanced materials.

[26]  S. Wen,et al.  Broadband nonlinear optical response in multi-layer black phosphorus: an emerging infrared and mid-infrared optical material. , 2015, Optics express.

[27]  Weibo Cai,et al.  Iron oxide decorated MoS2 nanosheets with double PEGylation for chelator-free radiolabeling and multimodal imaging guided photothermal therapy. , 2015, ACS nano.

[28]  G. Steele,et al.  Fast and broadband photoresponse of few-layer black phosphorus field-effect transistors. , 2014, Nano letters.

[29]  Eric Pop,et al.  Li Intercalation in MoS2: In Situ Observation of Its Dynamics and Tuning Optical and Electrical Properties. , 2015, Nano letters.

[30]  Miaoqiang Lyu,et al.  Bifunctional resistive switching behavior in an organolead halide perovskite based Ag/CH3NH3PbI3−xClx/FTO structure , 2016 .

[31]  R. Ruoff,et al.  Graphene oxide thin films for flexible nonvolatile memory applications. , 2010, Nano letters.

[32]  Steven G. Louie,et al.  Boron Nitride Nanotubes , 1995, Science.

[33]  K. Choi,et al.  Highly flexible and electroforming free resistive switching behavior of tungsten disulfide flakes fabricated through advanced printing technology , 2017 .

[34]  Suresh C Pillai,et al.  2D nanostructures for water purification: graphene and beyond. , 2016, Nanoscale.

[35]  Shibing Long,et al.  Graphene and Related Materials for Resistive Random Access Memories , 2017 .

[36]  Laurence Eaves,et al.  High electron mobility, quantum Hall effect and anomalous optical response in atomically thin InSe. , 2017, Nature nanotechnology.

[37]  Li Yang,et al.  Strain-Engineering Anisotropic Electrical Conductance of Phosphorene , 2014 .

[38]  Bo Tang,et al.  Electrochemical Ammonia Synthesis via Nitrogen Reduction Reaction on a MoS2 Catalyst: Theoretical and Experimental Studies , 2018, Advanced materials.

[39]  Ling Wen,et al.  One-pot solventless preparation of PEGylated black phosphorus nanoparticles for photoacoustic imaging and photothermal therapy of cancer. , 2016, Biomaterials.

[40]  Wei Huang,et al.  Controllable Multiple Depression in a Graphene Oxide Artificial Synapse , 2017 .

[41]  Gang Liu,et al.  Conjugated‐Polymer‐Functionalized Graphene Oxide: Synthesis and Nonvolatile Rewritable Memory Effect , 2010, Advanced materials.

[42]  S. Lau,et al.  Solution‐Processable Ultrathin Black Phosphorus as an Effective Electron Transport Layer in Organic Photovoltaics , 2016 .

[43]  Alberto Ansaldo,et al.  Exfoliation of Few-Layer Black Phosphorus in Low-Boiling-Point Solvents and Its Application in Li-Ion Batteries , 2018, 1805.02486.

[44]  E. Reed,et al.  Structural phase transitions in two-dimensional Mo- and W-dichalcogenide monolayers , 2014, Nature Communications.

[45]  Claudia Felser,et al.  Topological Quantum Phase Transition and Superconductivity Induced by Pressure in the Bismuth Tellurohalide BiTeI , 2016, Advanced materials.

[46]  Kai Sun,et al.  Tuning Ionic Transport in Memristive Devices by Graphene with Engineered Nanopores. , 2016, ACS nano.

[47]  F. Zhang,et al.  Revealing of the ultrafast third-order nonlinear optical response and enabled photonic application in two-dimensional tin sulfide , 2019, Photonics Research.

[48]  Mustafa Lotya,et al.  Large‐Scale Exfoliation of Inorganic Layered Compounds in Aqueous Surfactant Solutions , 2011, Advanced materials.

[49]  Han Zhang,et al.  A Novel Top‐Down Synthesis of Ultrathin 2D Boron Nanosheets for Multimodal Imaging‐Guided Cancer Therapy , 2018, Advanced materials.

[50]  Yuanjiang Xiang,et al.  2D Tellurium Based High‐Performance All‐Optical Nonlinear Photonic Devices , 2018, Advanced Functional Materials.

[51]  Jing Guo,et al.  Performance Limits of Monolayer Transition Metal Dichalcogenide Transistors , 2011, IEEE Transactions on Electron Devices.

[52]  Xianfan Xu,et al.  Plasmonic Resonance Enhanced Polarization-Sensitive Photodetection by Black Phosphorus in Near Infrared. , 2018, ACS nano.

[53]  D. Wilson,et al.  Sub-Micron Polymeric Stomatocytes as Promising Templates for Confined Crystallization and Diffraction Experiments. , 2017, Small.

[54]  Bing Chen,et al.  Very Low-Programming-Current RRAM With Self-Rectifying Characteristics , 2016, IEEE Electron Device Letters.

[55]  Feng Xing,et al.  Novel concept of the smart NIR-light–controlled drug release of black phosphorus nanostructure for cancer therapy , 2018, Proceedings of the National Academy of Sciences.

[56]  Giuseppe Iannaccone,et al.  Quantum engineering of transistors based on 2D materials heterostructures , 2018, Nature Nanotechnology.

[57]  Yi Xie,et al.  High‐Performance Flexible Broadband Photodetector Based on Organolead Halide Perovskite , 2014 .

[58]  Jianhui Zhao,et al.  Superior resistive switching memory and biological synapse properties based on a simple TiN/SiO2/p-Si tunneling junction structure , 2017 .

[59]  P. Zhou,et al.  Self‐Assembled Networked PbS Distribution Quantum Dots for Resistive Switching and Artificial Synapse Performance Boost of Memristors , 2018, Advanced materials.

[60]  Andres Castellanos-Gomez,et al.  Photovoltaic effect in few-layer black phosphorus PN junctions defined by local electrostatic gating. , 2014, Nature communications.

[61]  Jianxin Zhong,et al.  High‐Performance Photo‐Electrochemical Photodetector Based on Liquid‐Exfoliated Few‐Layered InSe Nanosheets with Enhanced Stability , 2018 .

[62]  George C Schatz,et al.  Covalent functionalization and passivation of exfoliated black phosphorus via aryl diazonium chemistry. , 2016, Nature chemistry.

[63]  Wang Yao,et al.  Optical signature of symmetry variations and spin-valley coupling in atomically thin tungsten dichalcogenides , 2012, Scientific Reports.

[64]  J. Yang,et al.  Memristive switching mechanism for metal/oxide/metal nanodevices. , 2008, Nature nanotechnology.

[65]  Zhongjun Li,et al.  Two-dimensional non-layered selenium nanoflakes: facile fabrications and applications for self-powered photo-detector , 2019, Nanotechnology.

[66]  Z. Yin,et al.  Fabrication of Flexible, All‐Reduced Graphene Oxide Non‐Volatile Memory Devices , 2013, Advanced materials.

[67]  Wei Ji,et al.  High-mobility transport anisotropy and linear dichroism in few-layer black phosphorus , 2014, Nature communications.

[68]  L. Liao,et al.  Metal‐Ion‐Modified Black Phosphorus with Enhanced Stability and Transistor Performance , 2017, Advanced materials.

[69]  Tetsuo Tsutsui,et al.  Organic‐inorganic heterostructure electroluminescent device using a layered perovskite semiconductor (C6H5C2H4NH3)2PbI4 , 1994 .

[70]  C. Lesniak,et al.  Boron nitride (BN) and BN composites for high-temperature applications , 2008 .

[71]  Chaoxing Wu,et al.  Mimicking Classical Conditioning Based on a Single Flexible Memristor , 2017, Advanced materials.

[72]  Z. Hua,et al.  High-performance photodetectors based on two-dimensional tin(II) sulfide (SnS) nanoflakes , 2018 .

[73]  D. Ciudad,et al.  Gate-tunable diode and photovoltaic effect in an organic-2D layered material p-n junction. , 2015, Nanoscale.

[74]  Lianhui Wang,et al.  RGD-QD-MoS2 nanosheets for targeted fluorescent imaging and photothermal therapy of cancer. , 2017, Nanoscale.

[75]  M. Kanatzidis,et al.  High Members of the 2D Ruddlesden-Popper Halide Perovskites: Synthesis, Optical Properties, and Solar Cells of (CH3(CH2)3NH3)2(CH3NH3)4Pb5I16 , 2017 .

[76]  Wei Huang,et al.  Stretchable Ti3C2Tx MXene/Carbon Nanotube Composite Based Strain Sensor with Ultrahigh Sensitivity and Tunable Sensing Range. , 2017, ACS nano.

[77]  P. Chu,et al.  Surface Coordination of Black Phosphorus for Robust Air and Water Stability. , 2016, Angewandte Chemie.

[78]  J. Gracio,et al.  Resistive switching and activity-dependent modifications in Ni-doped graphene oxide thin films , 2012 .

[79]  Jonghwa Eom,et al.  High-mobility and air-stable single-layer WS2 field-effect transistors sandwiched between chemical vapor deposition-grown hexagonal BN films , 2015, Scientific Reports.

[80]  J. Yang,et al.  Anatomy of a Nanoscale Conduction Channel Reveals the Mechanism of a High‐Performance Memristor , 2011, Advanced materials.

[81]  Qian Liu,et al.  Organic Photovoltaic Devices Based on a Novel Acceptor Material: Graphene , 2008 .

[82]  Jianhui Zhao,et al.  Memristor with Ag‐Cluster‐Doped TiO2 Films as Artificial Synapse for Neuroinspired Computing , 2018 .

[83]  Yuchao Yang,et al.  Building Neuromorphic Circuits with Memristive Devices , 2013, IEEE Circuits and Systems Magazine.

[84]  Shuangchun Wen,et al.  The formation of various multi-soliton patterns and noise-like pulse in a fiber laser passively mode-locked by a topological insulator based saturable absorber , 2014 .

[85]  Gang Qiu,et al.  Controlled Growth of a Large-Size 2D Selenium Nanosheet and Its Electronic and Optoelectronic Applications. , 2017, ACS Nano.

[86]  Ruitao Lv,et al.  The role of defects and doping in 2D graphene sheets and 1D nanoribbons , 2012, Reports on progress in physics. Physical Society.

[87]  Jing Zhang,et al.  AgInSbTe memristor with gradual resistance tuning , 2013 .

[88]  X. Qi,et al.  Two-dimensional bismuth nanosheets as prospective photo-detector with tunable optoelectronic performance , 2018, Nanotechnology.

[89]  G. Sun,et al.  Global pattern for the effect of climate and land cover on water yield , 2015, Nature Communications.

[90]  Shimeng Yu,et al.  A Low Energy Oxide‐Based Electronic Synaptic Device for Neuromorphic Visual Systems with Tolerance to Device Variation , 2013, Advanced materials.

[91]  Dingyuan Tang,et al.  Large energy soliton erbium-doped fiber laser with a graphene-polymer composite mode locker , 2009 .

[92]  Shimeng Yu,et al.  Synaptic electronics: materials, devices and applications , 2013, Nanotechnology.

[93]  Feng Zhang,et al.  Two-dimensional tellurium-polymer membrane for ultrafast photonics. , 2019, Nanoscale.

[94]  S. Lau,et al.  Functionalized graphene and other two-dimensional materials for photovoltaic devices: device design and processing. , 2015, Chemical Society reviews.

[95]  Junqing Hu,et al.  Solar‐Inspired Water Purification Based on Emerging 2D Materials: Status and Challenges , 2020 .

[96]  Zhongying Wang,et al.  Environmental Applications of 2D Molybdenum Disulfide (MoS2) Nanosheets. , 2017, Environmental science & technology.

[97]  Likai Li,et al.  Black phosphorus field-effect transistors. , 2014, Nature nanotechnology.

[98]  L. Dai,et al.  Facile Synthesis of Black Phosphorus: an Efficient Electrocatalyst for the Oxygen Evolving Reaction. , 2016, Angewandte Chemie.

[99]  G. Subramanyam,et al.  A Memristor Device Model , 2011, IEEE Electron Device Letters.

[100]  A. Lacaita,et al.  The race of phase change memories to nanoscale storage and applications , 2013 .

[101]  Lin Gan,et al.  Photonic Potentiation and Electric Habituation in Ultrathin Memristive Synapses Based on Monolayer MoS2. , 2018, Small.

[102]  A. Thomas,et al.  Memristor-based neural networks , 2013 .

[103]  Yubing Zhou,et al.  Strong Second-Harmonic Generation in Atomic Layered GaSe. , 2015, Journal of the American Chemical Society.

[104]  Huide Wang,et al.  Recent Developments in Stability and Passivation Techniques of Phosphorene toward Next‐Generation Device Applications , 2019, Advanced Functional Materials.

[105]  Qi Liu,et al.  Resistive switching memory effect of ZrO2 films with Zr+ implanted , 2008 .

[106]  Xiangfan Xu,et al.  Nonvolatile Floating‐Gate Memories Based on Stacked Black Phosphorus–Boron Nitride–MoS2 Heterostructures , 2015 .

[107]  D. Fan,et al.  Conceptually Novel Black Phosphorus/Cellulose Hydrogels as Promising Photothermal Agents for Effective Cancer Therapy , 2018, Advanced healthcare materials.

[108]  O. Farokhzad,et al.  Antimonene Quantum Dots: Synthesis and Application as Near-Infrared Photothermal Agents for Effective Cancer Therapy. , 2017, Angewandte Chemie.

[109]  J. Zhao,et al.  Roles of grain boundary and oxygen vacancies in Ba0.6Sr0.4TiO3 films for resistive switching device application , 2016, 2016 IEEE International Nanoelectronics Conference (INEC).

[110]  Zhengzheng Shao,et al.  Mechanical and electronic properties of monolayer MoS2 under elastic strain , 2012 .

[111]  Yidong Xia,et al.  Effects of the electroforming polarity on bipolar resistive switching characteristics of SrTiO3−δ films , 2010 .

[112]  D. Fan,et al.  Two Dimensional β-InSe with Layer-Dependent Properties: Band Alignment, Work Function and Optical Properties , 2019, Nanomaterials.

[113]  Minbiao Ji,et al.  Layer-Dependent Ultrafast Carrier and Coherent Phonon Dynamics in Black Phosphorus. , 2018, Nano letters.

[114]  Xiaopeng Li,et al.  Supramolecular Kandinsky circles with high antibacterial activity , 2018, Nature Communications.

[115]  S. Mitra,et al.  High-rate and high-energy-density lithium-ion battery anode containing 2D MoS₂ nanowall and cellulose binder. , 2013, ACS applied materials & interfaces.

[116]  Soo Doo Chae,et al.  Transistors with chemically synthesized layered semiconductor WS2 exhibiting 105 room temperature modulation and ambipolar behavior , 2012, 1204.0474.

[117]  Meng Liu,et al.  Dual-Wavelength Harmonically Mode-Locked Fiber Laser With Topological Insulator Saturable Absorber , 2014, IEEE Photonics Technology Letters.

[118]  Biqin Dong,et al.  Ultrasmall Bismuth Quantum Dots: Facile Liquid-Phase Exfoliation, Characterization, and Application in High-Performance UV–Vis Photodetector , 2017 .

[119]  Jiagen Li,et al.  Black-phosphorus-analogue tin monosulfide: an emerging optoelectronic two-dimensional material for high-performance photodetection with improved stability under ambient/harsh conditions , 2018 .

[120]  Chao Wang,et al.  Photothermal cancer immunotherapy by erythrocyte membrane‐coated black phosphorus formulation , 2019, Journal of controlled release : official journal of the Controlled Release Society.

[121]  T. Fujiwara,et al.  Removal of mercury in flue gas by the reaction with sulfide compounds , 1999 .

[122]  H. Tam,et al.  Induced solitons formed by cross-polarization coupling in a birefringent cavity fiber laser. , 2008, Optics letters.

[123]  Meng Qiu,et al.  Graphene oxide/black phosphorus nanoflake aerogels with robust thermo-stability and significantly enhanced photothermal properties in air. , 2017, Nanoscale.

[124]  A. Splendiani,et al.  Emerging photoluminescence in monolayer MoS2. , 2010, Nano letters.

[125]  T. Prodromakis,et al.  High Density Crossbar Arrays with Sub- 15 nm Single Cells via Liftoff Process Only , 2016, Scientific Reports.

[126]  K. Allakhverdiev,et al.  Photoluminescence frequency up-conversion in GaSe single crystals as studied by confocal microscopy , 2002 .

[127]  Jianhui Zhao,et al.  Flexible memristors as electronic synapses for neuro-inspired computation based on scotch tape-exfoliated mica substrates , 2018, Nano Research.

[128]  K. Sun,et al.  Memristive Behavior and Ideal Memristor of 1T Phase MoS2 Nanosheets. , 2016, Nano letters.

[129]  Limin Tong,et al.  High‐Speed and High‐Responsivity Hybrid Silicon/Black‐Phosphorus Waveguide Photodetectors at 2 µm , 2018, Laser & Photonics Reviews.

[130]  D. K. Sang,et al.  Black Phosphorous/Indium Selenide Photoconductive Detector for Visible and Near‐Infrared Light with High Sensitivity , 2019, Advanced Optical Materials.

[131]  H. Hamann,et al.  Ultra-high-density phase-change storage and memory , 2006, Nature materials.

[132]  Peng Zhou,et al.  The mechanism of the asymmetric SET and RESET speed of graphene oxide based flexible resistive switching memories , 2012 .

[133]  A. Bessonov,et al.  Layered memristive and memcapacitive switches for printable electronics. , 2015, Nature materials.

[134]  Mohammad Javad Sharifi,et al.  General SPICE Models for Memristor and Application to Circuit Simulation of Memristor-Based Synapses and Memory Cells , 2010, J. Circuits Syst. Comput..

[135]  D. Fan,et al.  Black phosphorus analogue tin sulfide nanosheets: synthesis and application as near-infrared photothermal agents and drug delivery platforms for cancer therapy. , 2018, Journal of materials chemistry. B.

[136]  Shinhyun Choi,et al.  Comprehensive physical model of dynamic resistive switching in an oxide memristor. , 2014, ACS nano.

[137]  Nam-Gyu Park,et al.  Organolead Halide Perovskite: New Horizons in Solar Cell Research , 2014 .

[138]  P. Miró,et al.  An atlas of two-dimensional materials. , 2014, Chemical Society reviews.

[139]  Qi Liu,et al.  Eliminating Negative‐SET Behavior by Suppressing Nanofilament Overgrowth in Cation‐Based Memory , 2016, Advanced materials.

[140]  Jae Hyuck Jang,et al.  Atomic structure of conducting nanofilaments in TiO2 resistive switching memory. , 2010, Nature nanotechnology.

[141]  Zhong Lin Wang,et al.  Piezoelectricity of single-atomic-layer MoS2 for energy conversion and piezotronics , 2014, Nature.

[142]  D. K. Sang,et al.  Current progress in black phosphorus materials and their applications in electrochemical energy storage. , 2017, Nanoscale.

[143]  Dianyuan Fan,et al.  2D Nonlayered Selenium Nanosheets: Facile Synthesis, Photoluminescence, and Ultrafast Photonics , 2017 .

[144]  F. Zhuge,et al.  Nonvolatile resistive switching in graphene oxide thin films , 2009 .

[145]  Transport properties of pristine few-layer black phosphorus by van der Waals passivation in an inert atmosphere. , 2014, Nature communications.

[146]  Jianhui Zhao,et al.  Vacancy-Induced Synaptic Behavior in 2D WS2 Nanosheet-Based Memristor for Low-Power Neuromorphic Computing. , 2019, Small.

[147]  Zhongjun Li,et al.  Graphene/phosphorene nano-heterojunction: facile synthesis, nonlinear optics, and ultrafast photonics applications with enhanced performance , 2017 .

[148]  J Joshua Yang,et al.  Memristive devices for computing. , 2013, Nature nanotechnology.

[149]  M. Green,et al.  The emergence of perovskite solar cells , 2014, Nature Photonics.

[150]  D. Stewart,et al.  The missing memristor found , 2008, Nature.

[151]  Siddharth Gaba,et al.  Nanoscale resistive memory with intrinsic diode characteristics and long endurance , 2010 .

[152]  SUPARNA DUTTASINHA,et al.  Graphene: Status and Prospects , 2009, Science.

[153]  L. Chu,et al.  Quasi‐Monolayer Black Phosphorus with High Mobility and Air Stability , 2018, Advanced materials.

[154]  Tze Chien Sum,et al.  Synthesis of Organic–Inorganic Lead Halide Perovskite Nanoplatelets: Towards High‐Performance Perovskite Solar Cells and Optoelectronic Devices , 2014 .

[155]  Lain‐Jong Li,et al.  Epitaxial Growth of Two-Dimensional Layered Transition-Metal Dichalcogenides: Growth Mechanism, Controllability, and Scalability. , 2017, Chemical reviews.

[156]  M. Ostling,et al.  A graphene-based hot electron transistor. , 2012, Nano letters.

[157]  Zhixing Wang,et al.  Electrochemical analysis graphite/electrolyte interface in lithium-ion batteries: p-Toluenesulfonyl isocyanate as electrolyte additive , 2017 .

[158]  Yuchao Yang,et al.  Oxide Resistive Memory with Functionalized Graphene as Built‐in Selector Element , 2014, Advanced materials.

[159]  Jinlan Wang,et al.  Passivation of Black Phosphorus via Self‐Assembled Organic Monolayers by van der Waals Epitaxy , 2017, Advanced materials.

[160]  M. Terrones,et al.  Defect engineering of two-dimensional transition metal dichalcogenides , 2016 .

[161]  J. Yang,et al.  Memristor crossbar arrays with 6-nm half-pitch and 2-nm critical dimension , 2018, Nature Nanotechnology.

[162]  Wei Yang Lu,et al.  Nanoscale memristor device as synapse in neuromorphic systems. , 2010, Nano letters.

[163]  G. Duscher,et al.  Pulsed Laser Deposition of Photoresponsive Two‐Dimensional GaSe Nanosheet Networks , 2014 .

[164]  M. Johnston,et al.  Charge-carrier dynamics in vapour-deposited films of the organolead halide perovskite CH3NH3PbI3-xClx , 2014 .

[165]  G. Guo,et al.  Enabling Colloidal Synthesis of Edge-Oriented MoS2 with Expanded Interlayer Spacing for Enhanced HER Catalysis. , 2017, Nano letters.

[166]  S. Porro,et al.  Memristive behaviour in inkjet printed graphene oxide thin layers , 2015 .

[167]  L. Chua Memristor-The missing circuit element , 1971 .

[168]  Fei Gao,et al.  Doxorubicin-loaded Fe3O4@MoS2-PEG-2DG nanocubes as a theranostic platform for magnetic resonance imaging-guided chemo-photothermal therapy of breast cancer , 2018, Nano Research.

[169]  Wilman Tsai,et al.  Chloride molecular doping technique on 2D materials: WS2 and MoS2. , 2014, Nano letters.

[170]  Xubing Lu,et al.  Flexible, Semitransparent, and Inorganic Resistive Memory based on BaTi0.95Co0.05O3 Film , 2017, Advanced materials.

[171]  Fei Meng,et al.  Enhanced hydrogen evolution catalysis from chemically exfoliated metallic MoS2 nanosheets. , 2013, Journal of the American Chemical Society.

[172]  Giacomo Indiveri,et al.  Integration of nanoscale memristor synapses in neuromorphic computing architectures , 2013, Nanotechnology.

[173]  Jihan Kim,et al.  Metallic Ti3C2Tx MXene Gas Sensors with Ultrahigh Signal-to-Noise Ratio. , 2018, ACS nano.

[174]  E. Akturk,et al.  Mechanical and Electronic Properties of MoS2 Nanoribbons and Their Defects , 2010, 1009.5488.

[175]  Dianyuan Fan,et al.  Broadband Nonlinear Optical Response in Few‐Layer Antimonene and Antimonene Quantum Dots: A Promising Optical Kerr Media with Enhanced Stability , 2017 .

[176]  S. Kim,et al.  Analysis on switching mechanism of graphene oxide resistive memory device , 2011 .

[177]  J. Cheon,et al.  Synthesis and structural transformations of colloidal 2D layered metal chalcogenide nanocrystals. , 2013, Chemical Society reviews.

[178]  X. Duan,et al.  High-Performance Black Phosphorus Field-Effect Transistors with Long-Term Air Stability. , 2018, Nano letters.

[179]  Yuting Luo,et al.  Preparation of 2D material dispersions and their applications. , 2018, Chemical Society reviews.

[180]  Yuliang Zhao,et al.  Functionalized Nano-MoS2 with Peroxidase Catalytic and Near-Infrared Photothermal Activities for Safe and Synergetic Wound Antibacterial Applications. , 2016, ACS nano.

[181]  Junle Qu,et al.  Ultrathin 2D Nonlayered Tellurium Nanosheets: Facile Liquid‐Phase Exfoliation, Characterization, and Photoresponse with High Performance and Enhanced Stability , 2018 .

[182]  A. Kis,et al.  2D transition metal dichalcogenides , 2017 .

[183]  P. Zhou,et al.  A New Memristor with 2D Ti3 C2 Tx MXene Flakes as an Artificial Bio-Synapse. , 2019, Small.

[184]  Takeshi Fujita,et al.  Covalent functionalization of monolayered transition metal dichalcogenides by phase engineering. , 2015, Nature chemistry.

[185]  Jing Guo,et al.  Atomically Thin Femtojoule Memristive Device , 2017, Advanced materials.

[186]  Nathan Youngblood,et al.  Waveguide-integrated black phosphorus photodetector with high responsivity and low dark current , 2014, Nature Photonics.

[187]  R. Williams,et al.  Sub-nanosecond switching of a tantalum oxide memristor , 2011, Nanotechnology.

[188]  Tae Whan Kim,et al.  Resistive switching memory based on organic/inorganic hybrid perovskite materials , 2016 .

[189]  Jie Yu,et al.  High-throughput synthesis of single-layer MoS2 nanosheets as a near-infrared photothermal-triggered drug delivery for effective cancer therapy. , 2014, ACS nano.

[190]  A. Pirovano,et al.  Electronic switching in phase-change memories , 2004, IEEE Transactions on Electron Devices.

[191]  Jian-Gang Zhu,et al.  Magnetoresistive Random Access Memory: The Path to Competitiveness and Scalability , 2008, Proceedings of the IEEE.

[192]  S. Lau,et al.  Wafer-Scale Synthesis of High-Quality Semiconducting Two-Dimensional Layered InSe with Broadband Photoresponse. , 2017, ACS nano.

[193]  G. Lay 2D materials: Silicene transistors , 2015 .

[194]  Jian Qin,et al.  2D Space-Confined Synthesis of Few-Layer MoS2 Anchored on Carbon Nanosheet for Lithium-Ion Battery Anode. , 2015, ACS nano.

[195]  Kai Yan,et al.  Epitaxy and photoresponse of two-dimensional GaSe crystals on flexible transparent mica sheets. , 2014, ACS nano.

[196]  L. Lauhon,et al.  Gate-tunable memristive phenomena mediated by grain boundaries in single-layer MoS2. , 2015, Nature nanotechnology.

[197]  Jack C. Lee,et al.  Thinnest Nonvolatile Memory Based on Monolayer h‐BN , 2019, Advanced materials.

[198]  Qiang Zhang,et al.  Exceptional catalytic effects of black phosphorus quantum dots in shuttling-free lithium sulfur batteries , 2018, Nature Communications.

[199]  Haiming Xie,et al.  Electrochemical Activity of Black Phosphorus as an Anode Material for Lithium-Ion Batteries , 2012 .

[200]  B. Liu,et al.  GaS and GaSe Ultrathin Layer Transistors , 2012, Advanced materials.

[201]  Jianhua Hao,et al.  Three-terminal memtransistors based on two-dimensional layered gallium selenide nanosheets for potential low-power electronics applications , 2019, Nano Energy.

[202]  W. Lu,et al.  AsP/InSe Van der Waals Tunneling Heterojunctions with Ultrahigh Reverse Rectification Ratio and High Photosensitivity , 2019, Advanced Functional Materials.

[203]  Xiaobing Yan,et al.  The Rise of 2D Photothermal Materials beyond Graphene for Clean Water Production , 2020, Advanced science.

[204]  Pu Huang,et al.  Enhanced Photodetection Properties of Tellurium@Selenium Roll-to-Roll Nanotube Heterojunctions. , 2019, Small.

[205]  Huaqiang Wu,et al.  Graphene Oxide Quantum Dots Based Memristors with Progressive Conduction Tuning for Artificial Synaptic Learning , 2018, Advanced Functional Materials.

[206]  Qinghua Zhao,et al.  Biocompatible PEGylated MoS2 nanosheets: controllable bottom-up synthesis and highly efficient photothermal regression of tumor. , 2015, Biomaterials.

[207]  A. Knorr,et al.  Dark and bright exciton formation, thermalization, and photoluminescence in monolayer transition metal dichalcogenides , 2017, 1703.03317.

[208]  Liang Cheng,et al.  Drug Delivery with PEGylated MoS2 Nano‐sheets for Combined Photothermal and Chemotherapy of Cancer , 2014, Advanced materials.

[209]  Taojian Fan,et al.  Black phosphorus: A novel nanoplatform with potential in the field of bio-photonic nanomedicine , 2018, Journal of Innovative Optical Health Sciences.

[210]  Wenhui Wang,et al.  All-Optical Switching of Two Continuous Waves in Few Layer Bismuthene Based on Spatial Cross-Phase Modulation , 2017 .

[211]  M. Hersam,et al.  Multi-terminal memtransistors from polycrystalline monolayer molybdenum disulfide , 2018, Nature.

[212]  F. Wen,et al.  Liquid‐Exfoliated Black Phosphorous Nanosheet Thin Films for Flexible Resistive Random Access Memory Applications , 2016 .

[213]  Huan Pang,et al.  MoS2‐Based Nanocomposites for Electrochemical Energy Storage , 2016, Advanced science.

[214]  Xiaodong Xu,et al.  Valleytronics in 2D materials , 2016 .

[215]  Xi Zhu,et al.  Engineering Lateral Heterojunction of Selenium‐Coated Tellurium Nanomaterials toward Highly Efficient Solar Desalination , 2019, Advanced science.

[216]  Jundong Shao,et al.  From Black Phosphorus to Phosphorene: Basic Solvent Exfoliation, Evolution of Raman Scattering, and Applications to Ultrafast Photonics , 2015 .

[217]  Xiaohui Li,et al.  Few-layer bismuthene for ultrashort pulse generation in a dissipative system based on an evanescent field. , 2018, Nanoscale.

[218]  Linghai Xie,et al.  Temperature dependence of resistive switching behaviors in resistive random access memory based on graphene oxide film , 2014, Nanotechnology.

[219]  R. W. Dave,et al.  A 4-Mb toggle MRAM based on a novel bit and switching method , 2005, IEEE Transactions on Magnetics.

[220]  Zhen Zhang,et al.  Field Test of Measurement-Device-Independent Quantum Key Distribution , 2014, IEEE Journal of Selected Topics in Quantum Electronics.

[221]  F. Zhang,et al.  Electric-field induced structural transition in vertical MoTe2- and Mo1–xWxTe2-based resistive memories , 2018, Nature Materials.

[222]  Jianhua Ji,et al.  Few-layer antimonene decorated microfiber: ultra-short pulse generation and all-optical thresholding with enhanced long term stability , 2017 .

[223]  Chi Jung Kang,et al.  Resistive Switching Behavior in Organic–Inorganic Hybrid CH3NH3PbI3−xClx Perovskite for Resistive Random Access Memory Devices , 2015, Advanced materials.

[224]  Zhipei Sun Optical modulators with two-dimensional layered materials , 2016, 2016 Progress in Electromagnetic Research Symposium (PIERS).

[225]  F. Xia,et al.  Rediscovering black phosphorus as an anisotropic layered material for optoelectronics and electronics. , 2014, Nature communications.

[226]  Photodetectors based on junctions of two-dimensional transition metal dichalcogenides* , 2017, 1702.02260.

[227]  Li Yang,et al.  Strain-engineering the anisotropic electrical conductance of few-layer black phosphorus. , 2014, Nano letters.

[228]  R. Waser,et al.  Coexistence of Grain‐Boundaries‐Assisted Bipolar and Threshold Resistive Switching in Multilayer Hexagonal Boron Nitride , 2017 .

[229]  S. Lau,et al.  Layer-dependent nonlinear optical properties and stability of non-centrosymmetric modification in few-layer GaSe sheets. , 2015, Angewandte Chemie.

[230]  Qiyuan He,et al.  Recent Advances in Ultrathin Two-Dimensional Nanomaterials. , 2017, Chemical reviews.

[231]  Chongwu Zhou,et al.  Mechanical and Electrical Anisotropy of Few-Layer Black Phosphorus. , 2015, ACS nano.

[232]  J. Yang,et al.  Robust memristors based on layered two-dimensional materials , 2018, 1801.00530.

[233]  Jang‐Sik Lee,et al.  Flexible Hybrid Organic-Inorganic Perovskite Memory. , 2016, ACS nano.

[234]  J. Coleman,et al.  Two-Dimensional Nanosheets Produced by Liquid Exfoliation of Layered Materials , 2011, Science.

[235]  J. Coleman,et al.  Liquid Exfoliation of Layered Materials , 2013, Science.

[236]  Hong Wang,et al.  Characteristic investigation of a flexible resistive memory based on a tunneling junction of Pd/BTO/LSMO on mica substrate , 2018, Applied Physics Letters.

[237]  Yu Pang,et al.  Interface Engineering with MoS2 -Pd Nanoparticles Hybrid Structure for a Low Voltage Resistive Switching Memory. , 2018, Small.

[238]  Long Ye,et al.  Highly Efficient 2D-Conjugated Benzodithiophene-Based Photovoltaic Polymer with Linear Alkylthio Side Chain , 2014 .

[239]  L. Lauhon,et al.  Effective passivation of exfoliated black phosphorus transistors against ambient degradation. , 2014, Nano letters.

[240]  Warren Robinett,et al.  Memristor-CMOS hybrid integrated circuits for reconfigurable logic. , 2009, Nano letters.

[241]  A S Rodin,et al.  Strain-induced gap modification in black phosphorus. , 2014, Physical review letters.

[242]  C. Toumazou,et al.  A Versatile Memristor Model With Nonlinear Dopant Kinetics , 2011, IEEE Transactions on Electron Devices.

[243]  Dianyuan Fan,et al.  Few‐layer Bismuthene: Sonochemical Exfoliation, Nonlinear Optics and Applications for Ultrafast Photonics with Enhanced Stability , 2018 .

[244]  John A Rogers,et al.  CVD-grown monolayer MoS2 in bioabsorbable electronics and biosensors , 2018, Nature Communications.

[245]  Chao Gao,et al.  Ultrathin Graphene Nanofiltration Membrane for Water Purification , 2013 .

[246]  Byung Joon Choi,et al.  High‐Speed and Low‐Energy Nitride Memristors , 2016 .

[247]  Gerhard Klimeck,et al.  Complementary Black Phosphorus Tunneling Field-Effect Transistors. , 2018, ACS nano.

[248]  Peng Chen,et al.  Tunable Electroluminescence in Planar Graphene/SiO2 Memristors , 2013, Advanced materials.

[249]  Teresa J. Feo,et al.  Structural absorption by barbule microstructures of super black bird of paradise feathers , 2018, Nature Communications.

[250]  SUPARNA DUTTASINHA,et al.  Van der Waals heterostructures , 2013, Nature.

[251]  Jong-Hyun Ahn,et al.  Degradation behaviors and mechanisms of MoS2 crystals relevant to bioabsorbable electronics , 2018, NPG Asia Materials.

[252]  Guofa Cai,et al.  Hexagonal Boron Nitride Thin Film for Flexible Resistive Memory Applications , 2016 .

[253]  Xiaobing Yan,et al.  Highly Transparent Bipolar Resistive Switching Memory in Zr0.5Hf0.5O2 Films With Amorphous Semiconducting In–Ga–Zn–O as Electrode , 2015, IEEE Transactions on Electron Devices.

[254]  Georg Kresse,et al.  Structure, energetics, and electronic properties of the surface of a promoted MoS2 catalyst : An ab initio local density functional study , 2000 .

[255]  Meng Qiu,et al.  Fluorinated Phosphorene: Electrochemical Synthesis, Atomistic Fluorination, and Enhanced Stability. , 2017, Small.

[256]  Andre K. Geim,et al.  Electric Field Effect in Atomically Thin Carbon Films , 2004, Science.

[257]  G. Wallace,et al.  Self‐Assembly of Flexible Free‐Standing 3D Porous MoS2‐Reduced Graphene Oxide Structure for High‐Performance Lithium‐Ion Batteries , 2017 .

[258]  F. Besenbacher,et al.  Size-dependent structure of MoS2 nanocrystals. , 2007, Nature nanotechnology.

[259]  Lifeng Wang,et al.  Synthesis of few-layer GaSe nanosheets for high performance photodetectors. , 2012, ACS nano.

[260]  Bernard Dieny,et al.  Magnetoresistive Random Access Memory , 2016, Proceedings of the IEEE.

[261]  Kunnyun Kim,et al.  A High‐On/Off‐Ratio Floating‐Gate Memristor Array on a Flexible Substrate via CVD‐Grown Large‐Area 2D Layer Stacking , 2017, Advanced materials.

[262]  Kai Zhang,et al.  Selenium-Doped Black Phosphorus for High-Responsivity 2D Photodetectors. , 2016, Small.

[263]  Gyu-Tae Kim,et al.  Few-layer black phosphorus field-effect transistors with reduced current fluctuation. , 2014, ACS nano.

[264]  J. Shan,et al.  Electrical control of the valley Hall effect in bilayer MoS2 transistors. , 2015, Nature nanotechnology.

[265]  Jie Yu,et al.  Smart MoS2/Fe3O4 Nanotheranostic for Magnetically Targeted Photothermal Therapy Guided by Magnetic Resonance/Photoacoustic Imaging , 2015, Theranostics.

[266]  Wei Lu,et al.  Short-term Memory to Long-term Memory Transition in a Nanoscale Memristor , 2022 .

[267]  Shimeng Yu,et al.  An Electronic Synapse Device Based on Metal Oxide Resistive Switching Memory for Neuromorphic Computation , 2011, IEEE Transactions on Electron Devices.

[268]  Takashi Taniguchi,et al.  Air-stable transport in graphene-contacted, fully encapsulated ultrathin black phosphorus-based field-effect transistors. , 2014, ACS Nano.

[269]  M. Ashokkumar,et al.  Recent advances in MoS2 nanostructured materials for energy and environmental applications – A Review , 2017 .

[270]  Xiaoling Luo,et al.  Advances in nanomaterials for photodynamic therapy applications: Status and challenges. , 2020, Biomaterials.

[271]  E. Sargent,et al.  Halide-Dependent Electronic Structure of Organolead Perovskite Materials , 2015 .

[272]  H.-S. Philip Wong,et al.  Phase Change Memory , 2010, Proceedings of the IEEE.

[273]  Leslie Y Yeo,et al.  Ultrafast Acoustofluidic Exfoliation of Stratified Crystals , 2018, Advanced materials.

[274]  Meng Qiu,et al.  Omnipotent phosphorene: a next-generation, two-dimensional nanoplatform for multidisciplinary biomedical applications. , 2018, Chemical Society reviews.

[275]  Jinhua Ye,et al.  Targeted Synthesis of 2H‐ and 1T‐Phase MoS2 Monolayers for Catalytic Hydrogen Evolution , 2016, Advanced materials.

[276]  Zhenhua Ni,et al.  Broadband graphene polarizer , 2011 .