A large‐eddy model for cirrus clouds with explicit aerosol and ice microphysics and Lagrangian ice particle tracking

We introduce a novel large-eddy model for cirrus clouds with explicit aerosol and ice microphysics, and validate its central components. A combined Eulerian/Lagrangian approach is used to simulate the formation and evolution of cirrus. While gas and size-resolved aerosol phases are treated over a fixed Eulerian grid similar to the dynamical and thermodynamical variables, the ice phase is treated by tracking a large number of simulation ice particles. The macroscopic properties of the ice phase are deduced from statistically analysing large samples of simulation ice particle properties. The new model system covers non-equilibrium growth of liquid supercooled aerosol particles, their homogeneous freezing, heterogeneous ice nucleation in the deposition or immersion mode, growth of ice crystals by deposition of water vapour, sublimation of ice crystals and their gravitational sedimentation, aggregation between ice crystals due to differential sedimentation, the effect of turbulent dispersion on ice particle trajectories, diabatic latent and radiative heating or cooling, and radiative heating or cooling of ice crystals. This suite of explicitly resolved physical processes enables the detailed simulation and analysis of the dynamical–microphysical–radiative feedbacks characteristic of cirrus. We draw special attention to the ice aggregation process which redistributes large ice crystals vertically and changes the ice particle size distributions accordingly. We find that aggregation of ice crystals is the key process to generate precipitation-sized ice crystals in stratiform cirrus. A process-oriented algorithm is developed for ice aggregation based on the trajectories and sedimentation velocities of simulation ice particles for use in the dynamically and microphysically complex, multi-dimensional large-eddy approach. By virtue of an idealized model set-up, designed to isolate the effect of aggregation on the cirrus development, we show that aggregation and its effect on the ice crystal size distribution in the model is consistent with a theoretical scaling relation, which was found to be in good agreement with in situ measurements. Copyright c � 2010 Royal Meteorological Society

[1]  M. Schnaiter,et al.  Supplementary information for ‘ Heterogeneous nucleation of ice particles on glassy aerosols under cirrus conditions ’ , 2010 .

[2]  P. Smolarkiewicz,et al.  A multiscale anelastic model for meteorological research , 2002 .

[3]  Christopher P. Woods,et al.  The Occurrence of “Irregular” Ice Particles in Stratiform Clouds , 2007 .

[4]  J. Marsham,et al.  On the importance of the diffusional uptake of water vapour for the development and radiative properties of high altitude clouds: a large eddy model sensitivity study , 2007 .

[5]  P. Minnis,et al.  Factors controlling contrail cirrus optical depth , 2009 .

[6]  B. Kärcher,et al.  A cirrus cloud scheme for general circulation models , 2008 .

[7]  E. Jensen,et al.  Implications of persistent ice supersaturation in cold cirrus for stratospheric water vapor , 2005 .

[8]  Q. Fu,et al.  On the correlated k-distribution method for radiative transfer in nonhomogeneous atmospheres , 1992 .

[9]  Christian D. Kummerow,et al.  The Remote Sensing of Clouds and Precipitation from Space: A Review , 2007 .

[10]  B. Kärcher,et al.  Cloud-controlling factors of cirrus , 2009 .

[11]  D. Mitchell Evolution of Snow-Size Spectra in Cyclonic Storms. Part II: Deviations from the Exponential Form , 1991 .

[12]  Patrick Minnis,et al.  An Intercomparison of Microphysical Retrieval Algorithms for Upper-Tropospheric Ice Clouds , 2007 .

[13]  Thomas Koop,et al.  Heterogeneous nucleation of ice on surrogates of mineral dust , 2006 .

[14]  I. Sednev,et al.  Simulation of hydrometeor size spectra evolution by water-water, ice-water and ice-ice interactions , 1995 .

[15]  The capacitance of solid and hollow hexagonal ice columns , 2005 .

[16]  T. Elperin,et al.  Critical comments to results of investigations of drop collisions in turbulent clouds , 2007 .

[17]  Evolution of Snow-Size Spectra in Cyclonic Storms. Part I: Snow Growth by Vapor Deposition and Aggregation , 1988 .

[18]  K. K. Lo,et al.  The Growth of Snow in Winter Storms:. An Airborne Observational Study , 1982 .

[19]  B. Finlayson‐Pitts,et al.  Chemistry of the Upper and Lower Atmosphere , 2000 .

[20]  B. Kärcher,et al.  The roles of dynamical variability and aerosols in cirrus cloud formation , 2003 .

[21]  Bernd Kärcher,et al.  Trapping of trace gases by growing ice surfaces including surface-saturated adsorption , 2009 .

[22]  Paul A. Vaillancourt,et al.  Statistics and Parameterizations of the Effect of Turbulence on the Geometric Collision Kernel of Cloud Droplets , 2007 .

[23]  L. Margolin,et al.  MPDATA: A Finite-Difference Solver for Geophysical Flows , 1998 .

[24]  P. Field,et al.  Theory of growth by differential sedimentation, with application to snowflake formation. , 2004, Physical review. E, Statistical, nonlinear, and soft matter physics.

[25]  Kenneth Sassen,et al.  Cirrus Cloud Simulation Using Explicit Microphysics and Radiation. Part II: Microphysics, Vapor and Ice Mass Budgets, and Optical and Radiative Properties , 1998 .

[26]  E. James Davis,et al.  Breakup of levitated frost particles , 1998 .

[27]  J. Reichardt,et al.  Nucleation in synoptically forced cirrostratus , 2005 .

[28]  T. Ackerman,et al.  A simple formulation of the delta-four-stream approximation for radiative transfer parameterizations , 1988 .

[29]  S. Hayashida,et al.  Analysis of ozone loss in the Arctic stratosphere during the late winter and spring of 1997 using the Chemical Species Mapping on Trajectories (CSMT) technique , 2003 .

[30]  K. Gierens The influence of radiation on the diffusional growth of ice crystals , 1994 .

[31]  U. Schumann,et al.  Water vapour measurements inside cirrus clouds in Northern and Southern hemispheres during INCA , 2002 .

[32]  Mahoney,et al.  In situ measurements of organics, meteoritic material, mercury, and other elements in aerosols at 5 to 19 kilometers , 1998, Science.

[33]  ndrea,et al.  Development of a Detailed Microphysics Cirrus Model Tracking Aerosol Particles’ Histories for Interpretation of the Recent INCA Campaign , 2004 .

[34]  Paul R. Field,et al.  Aircraft Observations of Ice Crystal Evolution in an Altostratus Cloud , 1999 .

[35]  E. Fetzer,et al.  Cloudy and clear‐sky relative humidity in the upper troposphere observed by the A‐train , 2009 .

[36]  R. Rauber Characteristics of Cloud Ice and Precipitation during Wintertime Storms over the Mountains of Northern Colorado , 1987 .

[37]  Len G. Margolin,et al.  On Forward-in-Time Differencing for Fluids: an Eulerian/Semi-Lagrangian Non-Hydrostatic Model for Stratified Flows , 1997 .

[38]  B. Kärcher,et al.  Numerical simulations of homogeneous freezing processes in the aerosol chamber AIDA , 2002 .

[39]  B. Stevens,et al.  Elements of the microphysical structure of numerically simulated nonprecipitating stratocumulus , 1996 .

[40]  R. Hogan,et al.  The Capacitance of Pristine Ice Crystals and Aggregate Snowflakes , 2006, physics/0610038.

[41]  Ulrike Lohmann,et al.  A parameterization of cirrus cloud formation: Heterogeneous freezing , 2003 .

[42]  Matthew Bailey,et al.  Growth Rates and Habits of Ice Crystals between −20° and −70°C , 2004 .

[43]  J. Hallett,et al.  Production of secondary ice particles during the riming process , 1974, Nature.

[44]  Sonia Lasher-Trapp,et al.  Broadening of droplet size distributions from entrainment and mixing in a cumulus cloud , 2005 .

[45]  G. Shutts,et al.  A numerical modelling study of the geostrophic adjustment process following deep convection , 1994 .

[46]  C. Hosler,et al.  The aggregation of small ice crystals , 1960 .

[47]  J. Iaquinta,et al.  A general approach for deriving the properties of cirrus and stratiform ice cloud particles , 2002 .

[48]  A. Mangold,et al.  Experimental investigation of homogeneous freezing of sulphuric acid particles in the aerosol chamber AIDA , 2002 .

[49]  S. Solomon,et al.  On the composition and optical extinction of particles in the tropopause region , 1999 .

[50]  Bernd Kärcher,et al.  Process‐oriented large‐eddy simulations of a midlatitude cirrus cloud system based on observations , 2011 .

[51]  D. Mitchell,et al.  A new snow growth model with application to radar precipitation estimates , 2006 .

[52]  G. Stephens The Influence of Radiative Transfer on the Mass and Heat Budgets of Ice Crystals Failing in the Atmosphere , 1983 .

[53]  Bernd Kärcher,et al.  Atmospheric Chemistry and Physics The role of organic aerosols in homogeneous ice formation , 2005 .

[54]  Ernst Strüngmann Forum,et al.  Clouds in the perturbed climate system : their relationship to energy balance, atmospheric dynamics, and precipitation , 2009 .

[55]  K. D. Beheng,et al.  A two-moment cloud microphysics parameterization for mixed-phase clouds. Part 1: Model description , 2006 .

[56]  U. Lohmann,et al.  Freezing thresholds and cirrus cloud formation mechanisms inferred from in situ measurements of relative humidity , 2003 .

[57]  M. Petters,et al.  Observations of ice nucleation by ambient aerosol in the homogeneous freezing regime , 2010 .

[58]  R. Lawson,et al.  The 2D-S (Stereo) Probe: Design and Preliminary Tests of a New Airborne, High-Speed, High-Resolution Particle Imaging Probe , 2006 .

[59]  D. Mitchell Use of Mass- and Area-Dimensional Power Laws for Determining Precipitation Particle Terminal Velocities , 1996 .

[60]  P. Hobbs The Aggregation of Ice Particles in Clouds and Fogs at Low Temperatures , 1965 .

[61]  K. Liou Influence of Cirrus Clouds on Weather and Climate Processes: A Global Perspective , 1986 .

[62]  G. Kattawar,et al.  Scattering and absorption property database for nonspherical ice particles in the near- through far-infrared spectral region. , 2005, Applied optics.

[63]  K. Sassen,et al.  Cirrus Cloud Simulation Using Explicit Microphysics and Radiation. Part I: Model Description , 1998 .

[64]  Steven Platnick,et al.  Interactive comment on “On the importance of small ice crystals in tropical anvil cirrus” by E. J. Jensen et al , 2009 .

[65]  H. Morrison,et al.  A Novel Approach for Representing Ice Microphysics in Models: Description and Tests Using a Kinematic Framework , 2007 .

[66]  Pao K. Wang,et al.  Ventilation coefficients for falling ice crystals in the atmosphere at low-intermediate Reynolds numbers , 1999 .

[67]  D. M. Murphy,et al.  Measurements of the concentration and composition of nuclei for cirrus formation , 2003, Proceedings of the National Academy of Sciences of the United States of America.

[68]  S. Siano,et al.  Dispersion of aircraft emissions due to wake vortices in stratified shear flows : A two-dimensional numerical study , 1996 .

[69]  A. Petzold,et al.  Aerosol states in the free troposphere at northern midlatitudes , 2002 .

[70]  W. Cotton,et al.  New primary ice-nucleation parameterizations in an explicit cloud model , 1992 .

[71]  M. Bailey,et al.  A Comprehensive Habit Diagram for Atmospheric Ice Crystals: Confirmation from the Laboratory, AIRS II, and Other Field Studies , 2009 .

[72]  Richard Cotton,et al.  Efficiency of the deposition mode ice nucleation on mineral dust particles , 2006 .

[73]  Thomas Koop,et al.  Review of the vapour pressures of ice and supercooled water for atmospheric applications , 2005 .

[74]  S. Kreidenweis,et al.  The susceptibility of ice formation in upper tropospheric clouds to insoluble aerosol components , 1997 .

[75]  Sonia M. Kreidenweis,et al.  Observations of organic species and atmospheric ice formation , 2004 .

[76]  Kenneth Sassen,et al.  Cirrus Cloud Microphysical Property Retrieval Using Lidar and Radar Measurements. Part I: Algorithm Description and Comparison with In Situ Data , 2002 .

[77]  R. Shaw PARTICLE-TURBULENCE INTERACTIONS IN ATMOSPHERIC CLOUDS , 2003 .

[78]  Pao K. Wang,et al.  A Numerical Study of Cirrus Clouds. Part I: Model Description , 2003 .

[79]  Steven D. Miller,et al.  Comparison of GOES Cloud Classification Algorithms Employing Explicit and Implicit Physics , 2009 .

[80]  J. Klett,et al.  Microphysics of Clouds and Precipitation , 1978, Nature.

[81]  A. Heymsfield On measurements of small ice particles in clouds , 2007 .

[82]  Andrew J. Heymsfield,et al.  Refinements in the Treatment of Ice Particle Terminal Velocities, Highlighting Aggregates , 2005 .

[83]  W. D. Keith,et al.  The collection efficiency of a cylindrical target for ice crystals , 1989 .

[84]  A. Heymsfield Cirrus Uncinus Generating Cells and the Evolution of Cirriform Clouds. Part I: Aircraft Observations of the Growth of the Ice Phase , 1975 .

[85]  Stephen K. Cox,et al.  Cirrus Clouds. Part I: A Cirrus Cloud Model , 1985 .

[86]  William B. Rossow,et al.  Radiative Effects of Cloud-Type Variations , 2000 .

[87]  A. Heymsfield Cirrus Uncinus Generating Cells and the Evolution of Cirriform Clouds. Part III: Numerical Computations of the Growth of the Ice Phase , 1975 .

[88]  A. Khain,et al.  Collisions of Cloud Droplets in a Turbulent Flow. Part V: Application of Detailed Tables of Turbulent Collision Rate Enhancement to Simulation of Droplet Spectra Evolution , 2008 .

[89]  Richard Cotton,et al.  Parametrization of ice‐particle size distributions for mid‐latitude stratiform cloud , 2005 .

[90]  Ulrich Schumann,et al.  Subgrid length-scales for large-eddy simulation of stratified turbulence , 1991 .

[91]  S. Kinne,et al.  Microphysical modeling of cirrus: 1. Comparison with 1986 FIRE IFO measurements , 1994 .

[92]  Yu G Ua,et al.  Interactions of Radiation, Microphysics, and Turbulence in the Evolution of Cirrus Clouds , 2000 .

[93]  C. Westbrook (www.interscience.wiley.com) DOI: 10.1002/qj.000 The fall speeds of sub-100µm ice crystals , 2022 .

[94]  Q. Fu An Accurate Parameterization of the Infrared Radiative Properties of Cirrus Clouds for Climate Models , 1996 .

[95]  W. Hall,et al.  The Survival of Ice Particles Falling from Cirrus Clouds in Subsaturated Air , 1976 .

[96]  B. Luo,et al.  vapour pressures of H2SO4/HNO3/HCl/HBr/H2O solutions to low stratospheric temperatures , 1995 .

[97]  Andrew J. Heymsfield,et al.  Aggregation and Scaling of Ice Crystal Size Distributions , 2003 .

[98]  K. Gierens,et al.  Modelling of cirrus clouds – Part 1a: Model description and validation , 2008 .

[99]  F. X. Kneizys,et al.  AFGL atmospheric constituent profiles (0-120km) , 1986 .

[100]  K. Sassen,et al.  Cirrus Cloud Microphysical Property Retrieval Using Lidar and Radar Measurements. Part II: Midlatitude Cirrus Microphysical and Radiative Properties , 2002 .

[101]  H. Kapitza,et al.  3D mesoscale numerical studies of cirrus and stratus clouds by their time and space evolution , 1992 .

[102]  P. Field,et al.  A Test of Ice Self-Collection Kernels Using Aircraft Data , 2006 .

[103]  B. Luo,et al.  Water activity as the determinant for homogeneous ice nucleation in aqueous solutions , 2000, Nature.

[104]  A. Heymsfield,et al.  PRODUCTION OF ICE IN TROPOSPHERIC CLOUDS A Review , 2005 .

[105]  B. Kärcher Supersaturation, dehydration, and denitrification in Arctic cirrus , 2005 .

[106]  B. Kärcher Simulating gas-aerosol-cirrus interactions: Process-oriented microphysical model and applications , 2003 .

[107]  Ulrike Lohmann,et al.  Oxalic acid as a heterogeneous ice nucleus in the upper troposphere and its indirect aerosol effect , 2006 .

[108]  V. Ramaswamy,et al.  Interdependence of Radiation and Microphysics in Cirrus Clouds , 1986 .