Manipulating the size distributions of quantum dots associated with strain-renormalized surface energy

Utilizing computer simulations based on a continuity equation model, we propose a strategy for modifying three-dimensional quantum dot size distributions using a two-stage growth and anneal approach. The method simply requires that individual quantum dots have a minimum in their chemical potential as a function of island size, such as those associated with strain-renormalized surface energy. By depositing material for the required time, the island size distribution can be tuned to a desired size before removing the flux to narrow the distribution.

[1]  V. Shchukin,et al.  Tunable metastability of surface nanostructure arrays. , 2004, Physical review letters.

[2]  Nikolai N. Ledentsov,et al.  Epitaxy of Nanostructures , 2003 .

[3]  F. Liu Self-assembly of three-dimensional metal islands: nonstrained versus strained islands. , 2002, Physical Review Letters.

[4]  M. Lagally,et al.  Self-assembly of two-dimensional islands via strain-mediated coarsening. , 2001, Physical review letters.

[5]  Sinclair,et al.  Novel SiGe island coarsening kinetics: ostwald ripening and elastic interactions , 2000, Physical review letters.

[6]  Nikolai N. Ledentsov,et al.  Quantum dot heterostructures , 1999 .

[7]  Juan J. L. Velázquez,et al.  The Becker–Döring Equations and the Lifshitz–Slyozov Theory of Coarsening , 1998 .

[8]  J. Tersoff,et al.  Coarsening of Self-Assembled Ge Quantum Dots on Si(001) , 1998 .

[9]  A. Barabasi,et al.  DISLOCATION-FREE ISLAND FORMATION IN HETEROEPITAXIAL GROWTH : A STUDY AT EQUILIBRIUM , 1997, cond-mat/9710170.

[10]  N. Ledentsov,et al.  Spontaneous ordering of arrays of coherent strained islands. , 1995, Physical review letters.

[11]  Ng,et al.  Stability of periodic domain structures in a two-dimensional dipolar model. , 1995, Physical review. B, Condensed matter.

[12]  D. Vanderbilt Phase segregation and work-function variations on metal surfaces: spontaneous formation of periodic domain structures☆ , 1992 .

[13]  H. Atwater,et al.  Island growth and coarsening in thin films—conservative and nonconservative systems , 1990 .

[14]  B. Chakraverty Grain size distribution in thin films—1. Conservative systems , 1967 .

[15]  I. Lifshitz,et al.  The kinetics of precipitation from supersaturated solid solutions , 1961 .