Assessment of natural radioactivity and associated radiation hazards in some Cameroonian building materials

Abstract The concentration of 238 U, 232 Th and 40 K in 13 building materials obtained from factories and collected in field in Cameroon were investigated by γ -ray spectrometry. The activity ranged from 1.76 to 49.84 Bq kg - 1 , 0.32 to 147 Bq kg - 1 and 18 to 1226 Bq kg - 1 for 238 U, 232 Th and 40 K, respectively. The highest 238 U activity was found in compressed red soil brick type I ( 49.6 ± 0.3 Bq kg - 1 ) produced by a local manufacturer while the highest 232 Th ( 139 ± 13 Bq kg - 1 ) and 40 K ( 1162 ± 108 Bq kg - 1 ) activities were found in gravel collected from an exploitation site in Logbadjeck. The activities are compared with available data from other investigations and with the world average value for soils. The radium equivalent activity Ra eq , the external hazard index H ex , the indoor absorbed dose rate D ˙ in air and the annual effective dose equivalent E ˙ were evaluated to assess the radiation hazard for people living in dwellings made of the materials studied. All building materials have shown Ra eq (range from 10 to 313 Bq kg - 1 ) lower than the limit of 370 Bq kg - 1 set in the Organization for Economic Cooperation and Development [OECD, 1979. Exposure to radiation from the natural radioactivity in building materials. OECD, Paris] report which is equivalent to a γ -dose of 1.5 mSv yr - 1 . Except for the gravel from Logbadjeck, all the materials examined are acceptable for use as building materials as defined by the OECD criterion.

[1]  M. Iqbal,et al.  Measurement of environmental radioactivity for estimation of radiation exposure from saline soil of Lahore, Pakistan , 2005 .

[2]  M. Sharaf,et al.  Natural radioactivity and radon exhalation rates in building materials used in Egypt , 1999 .

[3]  E. Borham,et al.  A study of the radon emitted from various building materials using alpha track detectors , 1997 .

[4]  F. Bou-Rabee,et al.  Natural radioactivity in building materials utilized in the State of Kuwait , 1996 .

[5]  Stelios Christofides,et al.  Gamma radiation measurements and dose rates in commercially-used natural tiling rocks (granites). , 2002, Journal of environmental radioactivity.

[6]  S. Rizzo,et al.  Gamma activity and geochemical features of building materials: estimation of gamma dose rate and indoor radon levels in Sicily. , 2001, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[7]  W. Arafa Specific activity and hazards of granite samples collected from the Eastern Desert of Egypt. , 2004, Journal of environmental radioactivity.

[8]  S. Stoulos,et al.  Assessment of natural radiation exposure and radon exhalation from building materials in Greece. , 2003, Journal of environmental radioactivity.

[9]  M. S. Bawa'aneh,et al.  Exposure to radiation from the natural radioactivity in Jordanian building materials. , 2006, Radiation protection dosimetry.

[10]  N.Ahmad Matiullah,et al.  Natural radioactivity in Jordanian soil and building materials and the associated radiation hazards , 1998 .

[11]  D. Amrani,et al.  Natural radioactivity in Algerian building materials. , 2001, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[12]  N. M. Rasheed,et al.  A study of radon and thoron release from Egyptian building materials using polymeric nuclear track detectors. , 2001, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[13]  Noorddin Ibrahim,et al.  Natural activities of 238U, 232Th and 40K in building materials , 1999 .

[14]  A. Malanca,et al.  Natural radioactivity in building materials from the Brazilian state of Espírito Santo , 1995 .

[15]  M. Alam,et al.  Concentration of radionuclides in building and ceramic materials of Bangladesh and evaluation of radiation hazard , 1998 .

[16]  岩崎 民子 SOURCES AND EFFECTS OF IONIZING RADIATION : United Nations Scientific Committee on the Effects of Atomic Radiation UNSCEAR 2000 Report to the General Assembly, with Scientific Annexes , 2002 .

[17]  P. Hayumbu,et al.  Natural radioactivity in Zambian building materials collected from Lusaka , 1995 .

[18]  Lei Wang,et al.  Radioactivity concentrations in soils of the Xiazhuang granite area, China. , 2005, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[19]  M. G. Kwato Njock,et al.  Radioactivity level and soil radon measurement of a volcanic area in Cameroon. , 2008, Journal of environmental radioactivity.

[20]  Stefano Magnoni,et al.  Natural radioactivity and radon exhalation in stony materials , 1997 .

[21]  M. A. Misdaq,et al.  A new method for evaluating the influence of building materials on radon emanation in marrakechi Dwellings , 1997 .

[22]  F. Ahmed,et al.  Natural radioactivity and radon exhalation rate of soil in southern Egypt. , 2001, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[23]  R. H. Higgy,et al.  NATURAL RADIOACTIVITY IN DIFFERENT TYPES OF BRICKS FABRICATED AND USED IN THE CAIRO REGION , 1995 .

[24]  Fazal-ur-Rehman,et al.  Determination of radon exhalation rates from tiles using active and passive techniques , 2001 .

[25]  Nour Khalifa Ahmed,et al.  Measurement of natural radioactivity in building materials in Qena city, Upper Egypt. , 2005, Journal of environmental radioactivity.

[26]  Surinder Singh,et al.  Natural activities of , and in some Indian building materials , 2003 .

[27]  A. El-Shershaby,et al.  Measurement of radioactivity and radon exhalation rate in different kinds of marbles and granites. , 2001, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[28]  M. Iqbal,et al.  Measurement of natural radioactivity in marble found in Pakistan using a NaI(Tl) gamma-ray spectrometer , 2000 .

[29]  Henry I. Kohn,et al.  Sources, Effects and Risks of Ionizing Radiation , 1989 .

[30]  Konstantin Kovler,et al.  Natural radionuclides in building materials available in Israel , 2002 .

[31]  C. Raptis,et al.  Study of natural radionuclides and radon emanation in bricks used in the Attica region, Greece , 1996 .

[32]  M. Anagnostakis,et al.  Photon attenuation, natural radioactivity content and radon exhalation rate of building materials. , 2002, Journal of environmental radioactivity.