Advances in the scintillation performance of LSO:Ce single crystals

We investigated the scintillation characteristics of 2186 LSO crystals that were cut from over 400 crystal boules. We measured the light output and energy resolution of all crystals, and also measured the decay times of a broad sampling of the crystals. We observed a significant reduction in the variation of both light output and decay time in this population of crystals compared to the results previously published in 1998. The reduced variation in scintillation properties may be attributed to better control of the populations of the two Ce scintillation centers in LSO, as well as better control of the effect of quenching centers, and the effects of Ce segregation during crystal growth.

[1]  Z. Zhang,et al.  Crystal growth. , 1999, Proceedings of the National Academy of Sciences of the United States of America.

[2]  G. G. Stokes "J." , 1890, The New Yale Book of Quotations.

[3]  M. Dahlbom,et al.  Investigation of LSO crystals for high spatial resolution positron emission tomography , 1996, 1996 IEEE Nuclear Science Symposium. Conference Record.

[4]  C. Brandle CHAPTER 7 – Crystal Pulling , 1980 .

[5]  R. Reisfeld Spectra and energy transfer of rare earths in inorganic glasses , 1973 .

[6]  C. Melcher,et al.  Czochralski growth of rare earth oxyorthosilicate single crystals , 1993 .

[7]  J. D. Valentine,et al.  Scintillator light yield nonproportionality: calculating photon response using measured electron response , 1997 .

[8]  Charles L. Melcher,et al.  Scintillation properties of LSO:Ce boules , 1998 .

[9]  J. D. Valentine,et al.  Light yield nonproportionality of CsI(Tl), CsI(Na), and YAP , 1997 .

[10]  J. D. Valentine,et al.  The measured electron response nonproportionalities of CaF/sub 2/, BGO, and LSO , 1997 .

[11]  G. E. Thomas,et al.  Measurement of the Time Dependence of Scintillation Intensity by a Delayed‐Coincidence Method , 1961 .

[12]  G. Blasse Influence of crystal structure on luminescence , 1968 .

[13]  Non-linear Response In The Scintillation Yield Of Lu/sub 2/ SiO/sub 5/ O:Ce/sup 3+/ , 1993 .

[14]  R. Lecomte,et al.  Scintillation light emission studies of LSO scintillators , 1998, 1998 IEEE Nuclear Science Symposium Conference Record. 1998 IEEE Nuclear Science Symposium and Medical Imaging Conference (Cat. No.98CH36255).

[15]  Li-Ji Lyu,et al.  Radiative and nonradiative relaxation measurements in Ce3+ doped crystals☆ , 1991 .

[16]  Non-proportional response in the light yield of inorganic scintillators , 1994, Proceedings of 1994 IEEE Nuclear Science Symposium - NSS'94.

[17]  J. Valentine,et al.  Light yield nonproportionality of CsI(Tl), CsI(Na), and YAP , 1997, 1997 IEEE Nuclear Science Symposium Conference Record.

[18]  Charles L. Melcher,et al.  Light emission mechanism of Lu/sub 2/(SiO/sub 4/)O:Ce , 1992 .