Public Health Costs of Primary PM2.5 and Inorganic PM2.5 Precursor Emissions in the United States.

Current methods of estimating the public health effects of emissions are computationally too expensive or do not fully address complex atmospheric processes, frequently limiting their applications to policy research. Using a reduced-form model derived from tagged chemical transport model (CTM) simulations, we present PM2.5 mortality costs per tonne of inorganic air pollutants with the 36 km × 36 km spatial resolution of source location in the United States, providing the most comprehensive set of such estimates comparable to CTM-based estimates. Our estimates vary by 2 orders of magnitude. Emission-weighted seasonal averages were estimated at $88,000-130,000/t PM2.5 (inert primary), $14,000-24,000/t SO2, $3,800-14,000/t NOx, and $23,000-66,000/t NH3. The aggregate social costs for year 2005 emissions were estimated at $1.0 trillion dollars. Compared to other studies, our estimates have similar magnitudes and spatial distributions for primary PM2.5 but substantially different spatial patterns for precursor species where secondary chemistry is important. For example, differences of more than a factor of 10 were found in many areas of Texas, New Mexico, and New England states for NOx and of California, Texas, and Maine for NH3. Our method allows for updates as emissions inventories and CTMs improve, enhancing the potential to link policy research to up-to-date atmospheric science.

[1]  Daniel J. Jacob,et al.  Correlations between fine particulate matter (PM2.5) and meteorological variables in the United States: implications for the sensitivity of PM2.5 to climate change. , 2010 .

[2]  G. Yarwood,et al.  1.5-Dimensional volatility basis set approach for modeling organic aerosol in CAMx and CMAQ , 2014 .

[3]  Noelle E. Selin,et al.  Air quality resolution for health impact assessment: influence of regional characteristics , 2013 .

[4]  John H. Seinfeld,et al.  Effect of changes in climate and emissions on future sulfate-nitrate-ammonium aerosol levels in the United States: FUTURE INORGANIC AEROSOLS IN THE U.S. , 2009 .

[5]  D. Jacob,et al.  Impact of 2000-2050 climate change on fine particulate matter (PM 2.5 ) air quality inferred from a multi-model analysis of meteorological modes , 2012 .

[6]  Peter J Adams,et al.  Ammonia emission controls as a cost-effective strategy for reducing atmospheric particulate matter in the Eastern United States. , 2007, Environmental science & technology.

[7]  Michelle L Bell,et al.  Assessment of the health impacts of particulate matter characteristics. , 2012, Research report.

[8]  R. Burnett,et al.  Extended follow-up and spatial analysis of the American Cancer Society study linking particulate air pollution and mortality. , 2009, Research report.

[9]  John P. Dawson,et al.  Impacts of climate change on regional and urban air quality in the eastern United States: Role of meteorology , 2009 .

[10]  M. Brauer,et al.  Risk of Nonaccidental and Cardiovascular Mortality in Relation to Long-term Exposure to Low Concentrations of Fine Particulate Matter: A Canadian National-Level Cohort Study , 2012, Environmental health perspectives.

[11]  A. Goldstein,et al.  Known and Unexplored Organic Constituents in the Earth's Atmosphere , 2007 .

[12]  O. Jolliet,et al.  Defining intake fraction. , 2002, Environmental science & technology.

[13]  The use of ambient measurements to identify which precursor species limit aerosol nitrate formation. , 2000, Journal of the Air & Waste Management Association.

[14]  Comparison of Fine Particles and the Relationship between Particle Variations and Meteorology at an Urban Site and a Remote Site in the Eastern United States , 2002, Journal of the Air & Waste Management Association.

[15]  Anu W. Turunen,et al.  Effects of long-term exposure to air pollution on natural-cause mortality: an analysis of 22 European cohorts within the multicentre ESCAPE project , 2014, The Lancet.

[16]  William D. Nordhaus,et al.  Environmental Accounting for Pollution in the United States Economy , 2011 .

[17]  Kristen M. Foley,et al.  A nonlinear regression model estimating single source concentrations of primary and secondarily formed PM2.5 , 2011 .

[18]  Nicholas Z. Muller,et al.  Measuring the damages of air pollution in the United States , 2007 .

[19]  Nicholas Z. Muller Linking Policy to Statistical Uncertainty in Air Pollution Damages , 2011 .

[20]  S. Pandis,et al.  Marginal PM25: Nonlinear Aerosol Mass Response to Sulfate Reductions in the Eastern United States. , 1999, Journal of the Air & Waste Management Association.

[21]  M. Jacobson GATOR-GCMM: A global through urban scale air pollution and weather forecast model , 2001 .

[22]  M. Kleeman,et al.  Evaluating the first‐order effect of intraannual temperature variability on urban air pollution , 2003 .

[23]  Spyros N. Pandis,et al.  Response of Inorganic PM to Precursor Concentrations , 1998 .

[24]  P. Adams,et al.  Temporally resolved ammonia emission inventories: Current estimates, evaluation tools, and measurement needs , 2006 .

[25]  S. F. Wu,et al.  Effect of changes in climate and emissions on future sulfate‐nitrate‐ammonium aerosol levels in the United States , 2009 .

[26]  Jenny L. Hand,et al.  Seasonal composition of remote and urban fine particulate matter in the United States , 2012 .

[27]  James W. Boylan,et al.  Preliminary Evaluation of the Community Multiscale Air Quality Model for 2002 over the Southeastern United States , 2005, Journal of the Air & Waste Management Association.

[28]  Allen L. Robinson,et al.  Effects of gas particle partitioning and aging of primary emissions on urban and regional organic aerosol concentrations , 2008 .

[29]  Georg A. Grell,et al.  Fully coupled “online” chemistry within the WRF model , 2005 .

[30]  Paulina Jaramillo,et al.  Costs of Automobile Air Emissions in U.S. Metropolitan Areas , 2011 .

[31]  L. Chen,et al.  PM2.5 source profiles for black and organic carbon emission inventories. , 2011 .

[32]  Allen L Robinson,et al.  Rethinking Organic Aerosols: Semivolatile Emissions and Photochemical Aging , 2007, Science.

[33]  D. Byun,et al.  Review of the Governing Equations, Computational Algorithms, and Other Components of the Models-3 Community Multiscale Air Quality (CMAQ) Modeling System , 2006 .

[34]  Robin L. Dennis,et al.  NARSTO critical review of photochemical models and modeling , 2000 .

[35]  Peter J. Adams,et al.  Reduced-form modeling of public health impacts of inorganic PM2.5 and precursor emissions , 2016 .

[36]  Bryan J. Hubbell,et al.  The influence of location, source, and emission type in estimates of the human health benefits of reducing a ton of air pollution , 2009, Air quality, atmosphere, & health.

[37]  Neal Fann,et al.  Characterizing the PM₂.₅-related health benefits of emission reductions for 17 industrial, area and mobile emission sectors across the U.S. , 2012, Environment international.

[38]  Jonathan I Levy,et al.  The influence of traffic on air quality in an urban neighborhood: a community-university partnership. , 2009, American journal of public health.

[39]  J. West,et al.  The effect of grid resolution on estimates of the burden of ozone and fine particulate matter on premature mortality in the USA , 2013, Air Quality, Atmosphere & Health.

[40]  Noelle E Selin,et al.  U.S. Air Quality and Health Benefits from Avoided Climate Change under Greenhouse Gas Mitigation. , 2015, Environmental science & technology.

[41]  Nancy J. Brown,et al.  Evaluating Uncertainties in Regional Photochemical Air Quality Modeling , 2003 .

[42]  P. Adams,et al.  Implications of ammonia emissions from post-combustion carbon capture for airborne particulate matter. , 2015, Environmental science & technology.

[43]  Lester B Lave,et al.  The costs, air quality, and human health effects of meeting peak electricity demand with installed backup generators. , 2006, Environmental science & technology.

[44]  A. Russell,et al.  PM and light extinction model performance metrics, goals, and criteria for three-dimensional air quality models , 2006 .

[45]  Jeremy J. Michalek,et al.  Valuation of plug-in vehicle life-cycle air emissions and oil displacement benefits , 2011, Proceedings of the National Academy of Sciences.

[46]  Ari Rabl,et al.  PUBLIC HEALTH IMPACT OF AIR POLLUTION AND IMPLICATIONS FOR THE ENERGY SYSTEM , 2000 .

[47]  Joel Schwartz,et al.  Uncertainty and Variability in Health‐Related Damages from Coal‐Fired Power Plants in the United States , 2009, Risk analysis : an official publication of the Society for Risk Analysis.

[48]  Nicholas Z. Muller Boosting GDP growth by accounting for the environment , 2014, Science.

[49]  S. Pandis,et al.  Exploring summertime organic aerosol formation in the eastern United States using a regional-scale budget approach and ambient measurements , 2010 .

[50]  Petros Koutrakis,et al.  The Role of Particle Composition on the Association Between PM2.5 and Mortality , 2008, Epidemiology.

[51]  R. Burnett,et al.  Overview of the Reanalysis of the Harvard Six Cities Study and American Cancer Society Study of Particulate Air Pollution and Mortality , 2003, Journal of toxicology and environmental health. Part A.

[52]  C. Hogrefe,et al.  Rethinking the Assessment of Photochemical Modeling Systems in Air Quality Planning Applications , 2008, Journal of the Air & Waste Management Association.

[53]  J. Levy,et al.  Evaluation of the Public Health Impacts of Traffic Congestion: A Health Risk Assessment , 2010 .

[54]  Noelle E Selin,et al.  Changes in inorganic fine particulate matter sensitivities to precursors due to large-scale US emissions reductions. , 2015, Environmental science & technology.

[55]  Xinyi Dong,et al.  Using the Community Multiscale Air Quality (CMAQ) model to estimate public health impacts of PM2.5 from individual power plants. , 2014, Environment international.

[56]  Jay Apt,et al.  Regional variations in the health, environmental, and climate benefits of wind and solar generation , 2013, Proceedings of the National Academy of Sciences.

[57]  John H. Seinfeld,et al.  Parameterization of the formation potential of secondary organic aerosols , 1989 .

[58]  Andrew W. Correia,et al.  Chemical Composition of Fine Particulate Matter and Life Expectancy: In 95 US Counties Between 2002 and 2007 , 2015, Epidemiology.

[59]  Bryan J. Hubbell,et al.  Methodological considerations in developing local-scale health impact assessments: balancing national, regional, and local data , 2009 .

[60]  Erik Swietlicki,et al.  Organic aerosol and global climate modelling: a review , 2004 .

[61]  Joel Schwartz,et al.  Chronic Exposure to Fine Particles and Mortality: An Extended Follow-up of the Harvard Six Cities Study from 1974 to 2009 , 2012, Environmental health perspectives.

[62]  A. Horvath,et al.  Intake fraction for particulate matter: recommendations for life cycle impact assessment. , 2011, Environmental science & technology.

[63]  Qi Zhang,et al.  Ubiquity and dominance of oxygenated species in organic aerosols in anthropogenically‐influenced Northern Hemisphere midlatitudes , 2007 .

[64]  A. Robinson,et al.  Unspeciated organic emissions from combustion sources and their influence on the secondary organic aerosol budget in the United States , 2012, Proceedings of the National Academy of Sciences.