A two-atom electron pump

With the development of single-atom transistors, consisting of single dopants, nanofabrication has reached an extreme level of miniaturization. Promising functionalities for future nanoelectronic devices are based on the possibility of coupling several of these dopants to each other. This already allowed to perform spectroscopy of the donor state by d.c. electrical transport. The next step, namely manipulating a single electron over two dopants, remains a challenge. Here we demonstrate electron pumping through two phosphorus donors in series implanted in a silicon nanowire. While quantized pumping is achieved in the low-frequency adiabatic regime, we observe remarkable features at higher frequency when the charge transfer is limited either by the tunnelling rates to the electrodes or between the two donors. The transitions between quantum states are modelled involving a Landau–Zener transition, allowing to reproduce in detail the characteristic signatures observed in the non-adiabatic regime.

[1]  B. Kaestner,et al.  Universal decay cascade model for dynamic quantum dot initialization. , 2009, Physical review letters.

[2]  Johnson,et al.  Quantized current in a quantum-dot turnstile using oscillating tunnel barriers. , 1991, Physical review letters.

[3]  D. Moraru,et al.  Single-electron transport through single dopants in a dopant-rich environment. , 2010, Physical review letters.

[4]  X Jehl,et al.  Detection of a large valley-orbit splitting in silicon with two-donor spectroscopy. , 2012, Physical review letters.

[5]  H. Inokawa,et al.  Pauli-spin-blockade transport through a silicon double quantum dot , 2007, 0707.3513.

[6]  Michel Devoret,et al.  Single-Electron Pump Based on Charging Effects , 1992 .

[7]  Takahiro Shinada,et al.  Enhancing semiconductor device performance using ordered dopant arrays , 2005, Nature.

[8]  Floquet scattering theory of quantum pumps , 2002, cond-mat/0208356.

[9]  X Jehl,et al.  Single-donor ionization energies in a nanoscale CMOS channel. , 2010, Nature nanotechnology.

[10]  Andrew D. Greentree,et al.  Coherent electronic transfer in quantum dot systems using adiabatic passage , 2004 .

[11]  M. Y. Simmons,et al.  A single atom transistor , 2012, 2012 IEEE Silicon Nanoelectronics Workshop (SNW).

[12]  John M. Martinis,et al.  Accuracy of electron counting using a 7‐junction electron pump , 1996 .

[13]  E. Abrahams,et al.  Impurity Conduction at Low Concentrations , 1960 .

[14]  S. Chorley,et al.  Quantized charge pumping through a carbon nanotube double quantum dot , 2012, 1204.1044.

[15]  Andrew S. Dzurak,et al.  A single-atom electron spin qubit in silicon , 2012, Nature.

[16]  Yu. A. Pashkin,et al.  Single-electron current sources: towards a refined definition of ampere , 2012, 1208.4030.

[17]  Gert-Ludwig Ingold,et al.  Charge Tunneling Rates in Ultrasmall Junctions , 1992 .

[18]  E. Tosatti,et al.  Crossover from adiabatic to antiadiabatic quantum pumping with dissipation. , 2011, Physical review letters.

[19]  Marc Kastner,et al.  Single Charge Tunneling: Coulomb Blockade Phenomena in Nanostructures , 1993 .

[20]  A. Fujiwara,et al.  Donor-based single electron pumps with tunable donor binding energy. , 2012, Nano letters.

[21]  G. Hein,et al.  Single-parameter nonadiabatic quantized charge pumping , 2007, 0707.0993.

[22]  M Jurczak,et al.  Transport spectroscopy of a single dopant in a gated silicon nanowire. , 2006, Physical review letters.

[23]  M. Flatté,et al.  Single dopants in semiconductors. , 2011, Nature materials.

[24]  C. Zener Non-Adiabatic Crossing of Energy Levels , 1932 .

[25]  D. Thouless,et al.  Quantization of particle transport , 1983 .

[26]  Andrew Alves,et al.  Transport spectroscopy of single phosphorus donors in a silicon nanoscale transistor. , 2009, Nano letters.

[27]  Mark A. Eriksson,et al.  Embracing the quantum limit in silicon computing , 2011, Nature.

[28]  W. V. D. Wiel,et al.  Electron transport through double quantum dots , 2002, cond-mat/0205350.

[29]  Nazarov,et al.  Resonant tunneling through two discrete energy states. , 1995, Physical review letters.